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Bulletin of the American Physical Society

Detecting and manipulating the rotational states of trapped polyatomic molecules

Alexander Prehn, Rosa Gl ockner, Martin Ibr ugger, Martin Zeppenfeld, Gerhard Rempe

Published Jun 11, 2015• 0 citations
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Polyatomic molecules offer many applications in quantum science once the wealth of internal and external degrees of freedom can be controlled. A widely applicable approach for controlling the rotational states of trapped polyatomic molecules is presented in this thesis. It includes the development of a rotational-state detection method, rotational-state cooling via optical pumping, and the preparation of a motionally cold (~30 mK) ensemble of 10 6 trapped CH 3 F molecules in a single rotational state.

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Polyatomic molecules offer many applications in quantum science once the wealth of internal and external degrees of freedom can be controlled. A widely applicable approach for controlling the rotational states of trapped polyatomic molecules is presented in this thesis. It includes the development of a rotational-state detection method, rotational-state cooling via optical pumping, and the preparation of a motionally cold (~30 mK) ensemble of 10 6 trapped CH 3 F molecules in a single rotational state.