Using the model of the DM interaction in
XY antiferromagnetic spin chain with spin-phonon coupling, the nonadiabatic effects on the DM interaction have been studied by developing a nonadiabatic analytical approach. The results show that in the nonadiabatic case, to a certain finite phonon frequency, there exists a finite critical value of spin-phonon coupling. As the spin-phonon coupling decreases to the critical value, the system becomes gapless and the spin dimerization is destroyed. The DM interaction leads the system to have a finite critical value of spin-phonon coupling even in the adiabatic limit. The increase in staggered DM interaction will decrease the critical value of spin-phonon coupling, but increase that of phonon frequency, therefore, favors the dimerization. The nonadiabaticity plays an important role in suppressing the enhancement effects of the DM interaction to the dimerization. The dimerized ground state when DM interaction is present can be destroyed by the quantum lattice fluctuations. The threshold value of $\ensuremath{\beta}$ changing the effect of the DM interaction on the dimerization from suppression to promotion is not simply a constant but a crossover. For appropriate fixed values of spin-phonon coupling, phonon frequency and $\ensuremath{\beta}$, as
D increases, the system undergoes a reentry of phase between spin-dimer state and gapless state.
Spin-phonon interactions have a dual role in emerging spin-based quantum technologies. While they can be a limitation to device performance through decoherence, they also serve as a critical resource for coherent spin control, detection, and the realization of spin-based quantum networks. However, their direct characterization remains a challenge and is usually material-dependent. Here, we introduce a technique to probe spin-phonon coupling at millikelvin temperatures and gigahertz frequencies, using high-overtone bulk acoustic wave resonators (HBARs) integrated with arbitrary crystals via visco-elastic transfer of thin-film lithium niobate transducers. By tuning the Larmor frequency of dilute spin ensembles into resonance with HBAR modes, we extract the anisotropy and strength of spin-phonon interactions from acoustic dispersion and dissipation measurements. We demonstrate this approach in calcium tungstate (CaWO4) and yttrium orthosilicate (Y2SiO5), achieving cooperativities up to 0.5 for erbium dopant ensembles. Our method enables the study of spin-phonon interactions in complex crystalline materials, with minimal fabrication constraints. These results will facilitate the design of hybrid quantum systems and the quest for ion-matrix combination with enhanced spin-phonon coupling.