The field of Quantum Optics has transitioned from the original study of the coherences of light, to its present day focus on the treatment of the interactions of matter with various quantum states of lights. This transition was spurred, in part, by the predicted potential of Quantum Information Processing protocols. These protocols take advantage of the coherent nature of quantum states and have been shown to be useful in numerous settings. However, the delicate nature of these coherences make scalability a real concern in realistic systems. Quantum Control is one particular tool to address this facet of Quantum Information Processing and has been used in experiments to great effect. In this thesis, we present our study of the use of Quantum Optics in Quantum Information and Quantum Control. We first introduce some results of InputOutput Theory, which is an elegant formalism to treat open quantum systems. Following which, we expound on work done in collaboration with colleagues from Brazil on a proposal for a loophole-free Bell test. This builds on the results derived using Input-Output theory and includes a semi-analytical formalism to perform the optimization of the Bell inequality. The treatment of this problem is then used to show that with existing optical cavity setups, one is able to produce the required states with a fidelity sufficient to violate a Bell inequality. Next, we present a description of an experiment to produce entangled photon pairs using four-wave mixing, done in collaboration with the experimental group in CQT. Finally, we present a study of quantum optimal control which highlights non-intuitive concepts of Optimal Control Theory.
The field of Quantum Optics has transitioned from the original study of the coherences of light, to its present day focus on the treatment of the interactions of matter with various quantum states of lights. This transition was spurred, in part, by the predicted potential of Quantum Information Processing protocols. These protocols take advantage of the coherent nature of quantum states and have been shown to be useful in numerous settings. However, the delicate nature of these coherences make scalability a real concern in realistic systems. Quantum Control is one particular tool to address this facet of Quantum Information Processing and has been used in experiments to great effect. In this thesis, we present our study of the use of Quantum Optics in Quantum Information and Quantum Control. We first introduce some results of InputOutput Theory, which is an elegant formalism to treat open quantum systems. Following which, we expound on work done in collaboration with colleagues from Brazil on a proposal for a loophole-free Bell test. This builds on the results derived using Input-Output theory and includes a semi-analytical formalism to perform the optimization of the Bell inequality. The treatment of this problem is then used to show that with existing optical cavity setups, one is able to produce the required states with a fidelity sufficient to violate a Bell inequality. Next, we present a description of an experiment to produce entangled photon pairs using four-wave mixing, done in collaboration with the experimental group in CQT. Finally, we present a study of quantum optimal control which highlights non-intuitive concepts of Optimal Control Theory.
In this thesis, I present experimental and theoretical work which assesses and develops a range of tools that are required for performing quantum information processing, particularly in photonic systems. I investigate the three degrees of freedom of a single photon—its polarisation, spatialmomentum and time-frequency distributions. For polarisation, I show that using wave plates to implement arbitrary, single-qubit rotations is more complicated than is commonly appreciated. In the spatial-momentum and time-frequency domains, I develop ways to perform tomographic analysis of quantum states, and I report the first demonstrations of these techniques. In the time-frequency domain, the tomography technique utilises entanglement in the photon polarisation as a resource to store and provide access to the time-frequency information. In my first two experiments, I use spontaneous parametric down-conversion to produce entanglement between pairs of single photons in all three degrees of freedom. I demonstrate the first characterisation of entanglement in spatial modes and the time-frequency domain, the first quantitative measurement of entangled qutrit states, and the highest quality entangled states yet measured in both polarisation and spatial modes. I also report the first realisation of complete hyperentanglement, and a full, black-box tomography of a 36-dimensional two-photon state—the largest system to be characterised in this way to date. In my final experiment, I model and implement a new architecture for a controlled-Z gate which is much simpler to align than previous implementations. This gate requires only one non-classical interference condition, the visibility of which is the main limitation to its performance. I show that the gate operates effectively as a means of both creating entanglement and discriminating between the four elements in a basis of maximally entangled, Bell-type states. Indeed, its observed performance as a Bell analyser would be sufficient to build a quantum state teleporter which would guarantee that the recipient would be left with a better copy of an unknown input state than any eavesdropper. In a series of numerical simulations, I investigate some of the practicalities that arise when using tomographic reconstruction techniques, including how to estimate errors, which measurements to make and what is actually the optimal reconstruction. In particular, I show that tomographies perform better when based on the results from over-complete sets of measurements. Finally, I discuss the important issue of how to compare two processes, particularly when trying to assess the quality of a measured process by comparing it to some expected ideal. Judging possible candidate measures against a set of experimentally and theoretically motivated
Quantum opto-mechanics is a fast moving, broad research field which aims to investigate and control the interaction of light and the quantized motion of mechanical objects and the coupling between them. This allows one to engineer the mechanical quantum state by controlling and measuring the electromagnetic field, and conversely, to control the dynamical evolution of the optical field via its interaction with a mechanical system. Mechanical resonators are accessible in many different shapes and sizes, from kilogram scales in experiments that test gravitational theories to micro- and nano-scales in resolved sideband regime, where the frequency of the mechanical resonator is larger than the bandwidth of the optical cavity. In this regime, it is possible to cool the mechanical object to the ground state which allows a high degree of control and the ability to prepare interesting non-classical states, states that could aid in investigating the quantum dynamics of macroscopic objects. The field of quantum opto-mechanics is a promising testbed for quantum control technologies, such as fundamental tests of quantum mechanics, ultra-sensitive quantum sensors for precise measurements, phonon lasing, mechanical memories with long lifetime and quantum information processing. Furthermore, experiments are progressing toward strong opto-mechanical coupling regimes with single photons. This creates a platform that can take advantage of the nonlinear optical interactions to generate highly non-classical states in such light-matter interfaces. Photonic systems working in the single photon regime will be promising for low power applications and also for implementations of quantum information and computation. Motivated by these applications, this thesis consists of theoretical studies in the context of single photonics. This includes investigating non-classical mechanical state generation and mechanically controlling the dynamical evolution of optical fields in the strong coupling regime single photon opto-mechanics and furthermore, proposing a quantum sensor using single photonics. In this regard, we employ three important formalisms to treat and measure open quantum systems with non-Gaussian input fields: the conditional and unconditional cascaded master equations, Fock-state master equations and input-output Langevin equations. In the context of opto-mechanics, the system to be investigated is composed of two optical cavities with a coupling modulated via a mechanical resonator. In one case, a sequence of single photons are irreversibly sent to one of the optical cavities. After photons go through the opto-mechanical interaction, photon counting measurements are performed on the cavity output, conditionally steering the mechanical state to a highly non-classical Fock state. Numerical calculations are performed to predict the experimental parameters needed to generate a mechanical Fock state before the mechanical object is thermalized. In another case, the same opto-mechanical scheme is employed to conversely modify the state of the optical mode by engineering the state of the mechanical degree of freedom. In this case, it is shown that the opto-mechanical system operates as an effective beam splitter for the input single photons, with a transmission that can be controlled by tuning the number of excitations in the bulk mechanical resonator. When the mechanical resonator has a small coherent amplitude it acts as a quantum control, entangling the optical and mechanical degrees of freedom. As the coherent amplitude of the resonator increases, it acts as a classical control for the input photons. Finally, we propose a novel multi-purpose sensor architecture that can be used for force, refractive index and possibly local temperature detection. In this scheme, two coupled cavities behave as an effective beam splitter. This sensor is based on fourth order interference (the Hong-Ou-Mandel effect) and requires a sequence of single photon pulses and consequently has low pulse power. Changes in the parameter to be measured induce variations in the effective beam splitter reflectivity and result in changes to the visibility of interference. We propose that this generic scheme could be implemented with coupled L3 photonic crystal cavities and find that this system, which only relies on photon coincidence detection and does not need any spectral resolution, can estimate forces as small as 10-7 Newtons and can measure one part per million change in refractive index using a very low input power of 10-10 W.
Precisely characterizing and controlling the dynamics of realistic open quantum systems has emerged in recent years as a key challenge across contemporary quantum sciences and technologies, with implications ranging from physics, chemistry and applied mathematics to quantum information processing (QIP) and quantum engineering. Quantum control theory aims to provide both a general dynamical-system framework and a constructive toolbox to meet this challenge. The purpose of this special issue of Journal of Physics B: Atomic, Molecular and Optical Physics is to present a state-of-the-art account of recent advances and current trends in the field, as reflected in two international meetings that were held on the subject over the last summer and which motivated in part the compilation of this volume—the Topical Group: Frontiers in Open Quantum Systems and Quantum Control Theory , held at the Institute for Theoretical Atomic, Molecular and Optical Physics (ITAMP) in Cambridge, Massachusetts (USA), from 1–14 August 2010, and the Safed Workshop on Quantum Decoherence and Thermodynamics Control , held in Safed (Israel), from 22–27 August 2010. Initial developments in quantum control theory date back to (at least) the early 1980s, and have been largely inspired by the well-established mathematical framework for classical dynamical systems. As the above-mentioned meetings made clear, and as the burgeoning body of literature on the subject testifies, quantum control has grown since then well beyond its original boundaries, and has by now evolved into a highly cross-disciplinary field which, while still fast-moving, is also entering a new phase of maturity, sophistication, and integration. Two trends deserve special attention: on the one hand, a growing emphasis on control tasks and methodologies that are specifically motivated by QIP, in addition and in parallel to applications in more traditional areas where quantum coherence is nevertheless vital (such as, for instance, quantum control of chemical reactions or high-resolution magnetic resonance spectroscopy); on the other hand, an unprecedented demand for close coupling between theory and experiment , with theoretical developments becoming more and more attuned to and driven by experimental advances as different quantum technologies continue to evolve at an impressive pace in the laboratory. Altogether, these two trends account for several of the recurrent themes in this volume, as well as in the current quantum control literature as a whole: namely, the quest for control strategies that can attain the highest degree of precision and robustness possible, while striving for efficiency and, ultimately, optimality in achieving the intended control task under realistic operational constraints. From a theory standpoint, this makes it imperative to take into account increasingly more realistic control settings; to assess the quantitative impact of limited control resources and/or system knowledge; and to provide a rigorous and general foundation for existing experimental approaches in order to further enhance applicability and performance. From an experimental standpoint, renewed emphasis is in turn placed on validating theoretical predictions and benchmarking performance, so that the limiting constraints can be singled out for additional theoretical analysis and guidance. This ongoing cross-talk is clearly reflected in this collection, which brings together theoreticians and experimentalists, with a significant fraction of the papers reporting on combined quantum control theory–experiment efforts. While a precise categorization would neither be possible nor desirable, contributions to this volume have been loosely grouped into five broad sections. This grouping has been made in the hope that connections between different problems and/or technical approaches will become more transparent, facilitating the transfer of concepts and methods. The special issue opens with a section devoted to open-loop control methods, with special emphasis on dynamical decoupling (DD), which is becoming an increasingly important tool for decoherence control at the physical 'quantum firmware' level. In addition to including original research results, the first two articles, by Brion et al and Biercuk et al , also serve to pedagogically review some background in their respective subjects. In particular, Brion et al revisit one of the conceptually simplest approaches to open-loop manipulation of both closed and open quantum systems, nonholonomic control , motivated by its broad applicability to QIP settings. A special instance of open-loop control based on sequences of (nearly) instantaneous `bang-bang' pulses is addressed by Biercuk et al , who reformulate the simplest DD scenario, suppression of phase decoherence in a single qubit, as a filter-design problem. Peng et al report on the implementation of 'concatenated' DD for arbitrary single-qubit decoherence in the context of nuclear magnetic resonance QIP. A dedicated analysis of the performance of different DD schemes in the presence of realistic pulse errors is given by Wang and Dobrovitski. DD is also one of the strategies used by Lucamarini et al to reduce polarization decoherence in a photon qubit. These authors additionally report on the use of active feedback to counter transmission noise, effectively setting the stage for the second section, which is centered on closed-loop control. Unlike in open-loop control, measurement is an essential ingredient in closed-loop schemes aimed at both reliably identifying features of the target quantum system and further modifying its dynamics. The importance of directly measuring the spectrum of the underlying system-environment coupling is stressed by Almog et al , who show how this knowledge is crucial, in particular, for predicting the performance of DD sequences in experiments and for optimizing performance. Riofrio et al address a weak-measurement protocol for implementing quantum state tomography , which is a necessary 'primitive' for inferring the target quantum state and thereby diagnosing the control performance. Next, the impact of realistic control and system imperfections in continuous-time Markovian feedback strategies for rapid state preparation is analyzed by Combes and Wiseman. A prominent role is played in the special issue by optimal control (OC) approaches, reflecting their central importance for quantum control and QIP. The OC contributions have been divided into two separate sections, depending on whether the target dynamics is modeled as Hamiltonian (section 3) or dissipative (section 4), respectively. The contribution by Beltrani et al deals with `control landscapes', which provide a foundation for analyzing the performance of numerical OC algorithms and their robustness against control errors. Specifically, this paper characterizes geometric properties of the control landscape, relevant to the optimal control of state-to-state transitions. Application of OC theory to the problem of population transfer and coherence enhancement in Λ-systems is studied by Kumar et al , whereas Goerz et al report on the OC-design of a high-fidelity controlled phase-gate in atomic qubits. The robustness of an OC solution is specifically addressed by Negretti et al , along with an approach for identifying easily implementable while still 'close-to-optimal' control pulses. Powerful relaxation-optimized OC schemes (based on so-called opengrape algorithms) for generating unitary target gates in the presence of known dissipation parameters are discussed by Schulte-Herbrüggen et al . Next, Lapert et al report on the problem of time-optimal control of spin-1/2 systems undergoing Bloch relaxation dynamics, highlighting the crucial role played by singular extremals in the control synthesis. Alternative approaches for optimized control of qubits exposed to various decoherence processes are developed by Esher et al and Xue et al , based on a perturbative 'bath-optimized' formalism and on numerical optimization via a genetic algorithm, respectively. Testifying to the richness of the field, the volume concludes with four contributions that address a diverse range of problems. The exploitation of properties of adiabatic quantum evolutions is common to the first two papers. In particular, Legthtas et al offer a rigorous explanation for the robustness of a control protocol, chirped pulsing , that is widely employed in 'adiabatic rapid passage' experiments, while Han et al present a theoretical framework for adiabatic Raman photo-association schemes relevant to ultracold atomic systems. In the context of cavity quantum electrodynamics, Montenegro and Orszag describe how to engineer a system of two atoms coupled to distant lossy cavities so that stable atomic entanglement is generated. Finally, still very little is known about the physical mechanisms that are responsible for and control the experimentally observed 'coherent' features of transport phenomena in biological systems. The last contribution by Alicki and Giraldi analyzes energy transport in dynamical systems that can be modeled as 'quantum networks', and points to this fascinating emerging frontier. It is our hope that the above papers may help readers to gain an overview of some of the main trends in current quantum control efforts, both theoretical and experimental. In closing, we take the opportunity to thank the organizations which sponsored the above-mentioned ITAMP Topical Group (the United States National Science Foundation and Harvard University) and the Safed Workshop (the Israeli Science Foundation, the Safed Scientific Workshop program, CECAM and ACAM). Last but not least our sincere gratitude goes to all of the contributors to the volume and the reviewers as well as the J. Phys. B staff, for their respective efforts in preparing the papers and ensuring the overall quality of this special issue.
Quantum information processing opens up completely new possibilities in communication and computation, that would be impossible in the realms of classical physics. While the benefits of quantum information processing are well understood in theory, it remains a formidable challenge to experimentally implement even simple quantum information processing tasks. Numerous physical architectures have been proposed for preparing and coherently manipulating quantum information. Amongst these, quantum optics has been identified as a particularly promising candidate. In particular this arises from the long decoherence times of single photon states, which can be used to encode logical qubits in a variety of ways. Nonetheless, there remain formidable challenges to implementing large scale quantum information processing using optical qubits. Most notably these include: the preparation of pure indistinguishable photons; efficient number-resolving photo-detection; mode-matching; photon loss; and the non-determinism of entangling gates. Any future large scale implementation of optical quantum information processing protocols will require significant advances on most, if not all these fronts. In this thesis we aim to present a comprehensive overview of the major requirements for optical quantum information processing, understand the effects they have, and how they can be modeled. From this we aim to understand what the realistic technological requirements are to achieve scalable optical quantum information processing, and, where possible, suggest means by which to help achieve these goals.
The violation of Bell inequalities where both detection and locality loopholes are closed is crucial for device-independent assessments of quantum information. While of a technological nature, the simultaneous closing of both loopholes still remains a challenge. In Teo et al. [Nat. Commun. 4, 2104 (2013)], a realistic setup to produce an atom-photon entangled state that could reach a loophole-free Bell inequality violation within current experimental technology is proposed. Here we improve the analysis of this proposal by giving an analytical treatment that shows that the state proposed in Teo et al. [Nat. Commun. 4, 2104 (2013)] can violate a Bell inequality for arbitrarily low photodectection efficiency, when all other losses are ignored. Moreover, it is also able to violate a Bell inequality considering only atomic and homodyne measurements eliminating the need to consider inefficient photocounting measurements. In this case, the maximum Clauser-Horne-Shimony-Holt inequality violation achievable is 2.29, and the minimum transmission required for violation is about 68%. Finally, we show that by postselecting on an atomic measurement, one can engineer superpositions of coherent states for various coherent state amplitudes.
Optimization of a Pulsed Source of Entangled Photons for the Violation of the CHSH Inequality
This thesis focuses on my work carried out in the Quantum Communications laboratory with the Quantum Future research group of the Department of Information Engeneering, in which I worked on the creation and optimization of a pulsed source of polarization entangled photons. The main focus in the laboratory was to optimize the experimental setup to prove the entangled nature of the photons produced. This was done by violating the Bell inequality in the form presented by Clauser, Horne, Shimony and Holt (CHSH) in 1969. The present work's objective is to provide an overview of all the crucial physical phenomena exploited in the experiment to obtain the wanted results.
In section 1 a presentation of the phenomenon of entanglement and of Bell's argument proving the incapability to describe its properties with a both real and local theory is given, along with the derivation of the ``CHSH inequality and the possibility to violate it with polarization entangled photons. Sections 2 and 3 focus on the properties of the Gaussian beam used in the experiment and its source: the mode-locked Mira laser. A brief discussion about mode-locked lasers and their properties is provided. In section 4 the nonlinear optical phenomena of second harmonic generation and spontaneous parametric down conversion are discussed, the former from a classical standpoint and the latter with a few quantum mechanical considerations. Section 5 focuses on polarization optics and the both classical and quantum mechanical formalism of the Jones vectors. A discussion of the effects of the birefringent devices used in the experiment on the photons' state is provided. Finally, sections 6 and 7 display a complete overview of the experimental setup and the results obtained for the violation of the inequality. A systematic explanation of the experimental optimization procedure is provided in section 6 as it may be useful for the future experimenters, since it proved to be tricky.
Throughout all the work, various characteristics of the devices used in the experimental setup are given, hopefully making the most important and peculiar aspects of the experiment clear.