Quantum opto-mechanics is a fast moving, broad research field which aims to investigate and control the interaction of light and the quantized motion of mechanical objects and the coupling between them. This allows one to engineer the mechanical quantum state by controlling and measuring the electromagnetic field, and conversely, to control the dynamical evolution of the optical field via its interaction with a mechanical system. Mechanical resonators are accessible in many different shapes and sizes, from kilogram scales in experiments that test gravitational theories to micro- and nano-scales in resolved sideband regime, where the frequency of the mechanical resonator is larger than the bandwidth of the optical cavity. In this regime, it is possible to cool the mechanical object to the ground state which allows a high degree of control and the ability to prepare interesting non-classical states, states that could aid in investigating the quantum dynamics of macroscopic objects. The field of quantum opto-mechanics is a promising testbed for quantum control technologies, such as fundamental tests of quantum mechanics, ultra-sensitive quantum sensors for precise measurements, phonon lasing, mechanical memories with long lifetime and quantum information processing. Furthermore, experiments are progressing toward strong opto-mechanical coupling regimes with single photons. This creates a platform that can take advantage of the nonlinear optical interactions to generate highly non-classical states in such light-matter interfaces. Photonic systems working in the single photon regime will be promising for low power applications and also for implementations of quantum information and computation. Motivated by these applications, this thesis consists of theoretical studies in the context of single photonics. This includes investigating non-classical mechanical state generation and mechanically controlling the dynamical evolution of optical fields in the strong coupling regime single photon opto-mechanics and furthermore, proposing a quantum sensor using single photonics. In this regard, we employ three important formalisms to treat and measure open quantum systems with non-Gaussian input fields: the conditional and unconditional cascaded master equations, Fock-state master equations and input-output Langevin equations. In the context of opto-mechanics, the system to be investigated is composed of two optical cavities with a coupling modulated via a mechanical resonator. In one case, a sequence of single photons are irreversibly sent to one of the optical cavities. After photons go through the opto-mechanical interaction, photon counting measurements are performed on the cavity output, conditionally steering the mechanical state to a highly non-classical Fock state. Numerical calculations are performed to predict the experimental parameters needed to generate a mechanical Fock state before the mechanical object is thermalized. In another case, the same opto-mechanical scheme is employed to conversely modify the state of the optical mode by engineering the state of the mechanical degree of freedom. In this case, it is shown that the opto-mechanical system operates as an effective beam splitter for the input single photons, with a transmission that can be controlled by tuning the number of excitations in the bulk mechanical resonator. When the mechanical resonator has a small coherent amplitude it acts as a quantum control, entangling the optical and mechanical degrees of freedom. As the coherent amplitude of the resonator increases, it acts as a classical control for the input photons. Finally, we propose a novel multi-purpose sensor architecture that can be used for force, refractive index and possibly local temperature detection. In this scheme, two coupled cavities behave as an effective beam splitter. This sensor is based on fourth order interference (the Hong-Ou-Mandel effect) and requires a sequence of single photon pulses and consequently has low pulse power. Changes in the parameter to be measured induce variations in the effective beam splitter reflectivity and result in changes to the visibility of interference. We propose that this generic scheme could be implemented with coupled L3 photonic crystal cavities and find that this system, which only relies on photon coincidence detection and does not need any spectral resolution, can estimate forces as small as 10-7 Newtons and can measure one part per million change in refractive index using a very low input power of 10-10 W.
Quantum opto-mechanics is a fast moving, broad research field which aims to investigate and control the interaction of light and the quantized motion of mechanical objects and the coupling between them. This allows one to engineer the mechanical quantum state by controlling and measuring the electromagnetic field, and conversely, to control the dynamical evolution of the optical field via its interaction with a mechanical system. Mechanical resonators are accessible in many different shapes and sizes, from kilogram scales in experiments that test gravitational theories to micro- and nano-scales in resolved sideband regime, where the frequency of the mechanical resonator is larger than the bandwidth of the optical cavity. In this regime, it is possible to cool the mechanical object to the ground state which allows a high degree of control and the ability to prepare interesting non-classical states, states that could aid in investigating the quantum dynamics of macroscopic objects. The field of quantum opto-mechanics is a promising testbed for quantum control technologies, such as fundamental tests of quantum mechanics, ultra-sensitive quantum sensors for precise measurements, phonon lasing, mechanical memories with long lifetime and quantum information processing. Furthermore, experiments are progressing toward strong opto-mechanical coupling regimes with single photons. This creates a platform that can take advantage of the nonlinear optical interactions to generate highly non-classical states in such light-matter interfaces. Photonic systems working in the single photon regime will be promising for low power applications and also for implementations of quantum information and computation. Motivated by these applications, this thesis consists of theoretical studies in the context of single photonics. This includes investigating non-classical mechanical state generation and mechanically controlling the dynamical evolution of optical fields in the strong coupling regime single photon opto-mechanics and furthermore, proposing a quantum sensor using single photonics. In this regard, we employ three important formalisms to treat and measure open quantum systems with non-Gaussian input fields: the conditional and unconditional cascaded master equations, Fock-state master equations and input-output Langevin equations. In the context of opto-mechanics, the system to be investigated is composed of two optical cavities with a coupling modulated via a mechanical resonator. In one case, a sequence of single photons are irreversibly sent to one of the optical cavities. After photons go through the opto-mechanical interaction, photon counting measurements are performed on the cavity output, conditionally steering the mechanical state to a highly non-classical Fock state. Numerical calculations are performed to predict the experimental parameters needed to generate a mechanical Fock state before the mechanical object is thermalized. In another case, the same opto-mechanical scheme is employed to conversely modify the state of the optical mode by engineering the state of the mechanical degree of freedom. In this case, it is shown that the opto-mechanical system operates as an effective beam splitter for the input single photons, with a transmission that can be controlled by tuning the number of excitations in the bulk mechanical resonator. When the mechanical resonator has a small coherent amplitude it acts as a quantum control, entangling the optical and mechanical degrees of freedom. As the coherent amplitude of the resonator increases, it acts as a classical control for the input photons. Finally, we propose a novel multi-purpose sensor architecture that can be used for force, refractive index and possibly local temperature detection. In this scheme, two coupled cavities behave as an effective beam splitter. This sensor is based on fourth order interference (the Hong-Ou-Mandel effect) and requires a sequence of single photon pulses and consequently has low pulse power. Changes in the parameter to be measured induce variations in the effective beam splitter reflectivity and result in changes to the visibility of interference. We propose that this generic scheme could be implemented with coupled L3 photonic crystal cavities and find that this system, which only relies on photon coincidence detection and does not need any spectral resolution, can estimate forces as small as 10-7 Newtons and can measure one part per million change in refractive index using a very low input power of 10-10 W.
Non-relativistic quantum mechanics have proven to be a significant framework to understand the non-classical behaviour of light and the microcosmos. Perhaps, one of the first technological revolutions within quantum theory came with the invention of the transistor, whereby a purely quantum mechanical description was required. Currently, another outstanding revolution is taking place in a crossroad where information science meets quantum mechanics (this being the quantum information field). Such an area of work contemplates both the fascinating theoretical aspect of quantum correlations, as well as implementations towards quantum tasks performed by a universal quantum computer; tasks that cannot be realised (or they are hard to implement) within the classical domain. This Thesis is devoted to study the dynamics of quantum entanglement in spin-optomechanics systems. In particular, we explore the quantum stabilization of quantum entanglement, a quantum concentration scheme in opto-mechanics and an interfacing of matter and light towards quantum networking applications. Additionally, we also investigate theoretical aspects of quantum correlations within thermal environments, as well as the topical area of quantum sudden transitions. In Chapter 1, we provide a brief summary of quantum information and of the quantum optics framework to cover elementary concepts and techniques used subsequently in this work. Subsequently, in Chapter 2 we present the stabilization of quantum entanglement in a non-linear qubit-oscillator system. The inclusion of a modest nonlinearity gives three results, i) the loss of periodicity of the system, ii) the occurrence of quadrature squeezing appearing for a short time, and iii) the quantum entanglement reaches higher values in contrast to the case without non-linearity. In Chapter 3, a technique to concentrate/distill a two-mode vacuum state in optomechanics via unsharp measurements is presented. Here, one of the optical modes is injected into a cavity at first, and thereafter, it is nonlinearly coupled to a mechanical oscillator. Afterwards, the position of the oscillator is measured using pulsed optomechanics and homodyne detection. The results show that this measurement can conditionally increase the initial entanglement. Next, in Chapter 4, stimulated by optomechanical transducers and quantum networking, a light-matter system is constructed where a qubit is coupled to a cavity mode mediated through a mechanical oscillator. The qubit-oscillator conditionally displaced Hamiltonian and the oscillator-cavity radiation-pressure interaction generate a maximal qubit-cavity entanglement. Additionally, we consider the case in which the cavity mode is coupled to a waveguide, numerical calculations show a promising qubit-fibre entanglement under a weak matter-light coupling. For the quantum network case, we coupled a generic qubit in the first node to a second qubit-cavity distant Jaynes-Cummings system coupled through an optical fibre, where qubit-qubit correlations can be achieved in the quantum open systems scenario. In Chapter 5, we study the evolution of an open quantum system within the Born-Markov microscopic master equation (MME). Essentially, two distant two-level atoms are trapped in fibre-coupled cavities. Under the approximation of one-excitation allowed in the atom-cavity-fibre basis, we can obtain quantum correlations induced by thermal fluctuations from the environments. Lastly, in Chapter 6, we bring together previously elements explored in this Thesis. The system is a hybrid atomic-mechanical system formed from two remote qubits interacting with individual harmonic oscillators. This system, as in Chapter 4, explores interesting applications in quantum networking schemes. The two qubits are initially prepared in a Bell-diagonal state, and consequently the two-qubit correlations exhibit few interesting effects such as freezing, sudden changes and revivals in the evolution of the quantum entropic discord. To conclude, I summarize my findings in Chapter 7.
In a nutshell, a cavity optomechanical system consists of a mechanical oscillator inside an optical cavity. Cavity optomechanics studies the interplay between the light-matter radiation-pressure interaction and the change in the cavity frequency induced by mechanical motion. By leveraging the tools of quantum optics and quantum measurement, cavity quantum optomechanics enables the engineering of nonclassical quantum states of bulk matter. In this thesis, I present protocols for engineering such nonclassical quantum states in Part II. First, I introduce a scheme to ‘grow’ a quantum kitten state of a mechanical oscillator into a macroscopic Schrödinger cat state using a series of nonlinear pulsed optomechanical interactions. Next, I detail our proposed schemes to generate and verify entanglement between two mechanical oscillators. Moving on from pulsed optomechanics, I describe the theory behind an experiment that achieved multi-phonon subtraction from a mechanical oscillator in a continuously driven Brillouin optomechanical system. In the final chapter of Part II, I provide a theoretical preview of an experiment that investigates the behaviour of the mechanical oscillator when no light is detected at the output. In Part III, I introduce a new framework for nonlinear cavity quantum optomechanics that incorporates the intrinsic nonlinearity of the radiation-pressure interaction, the nonlinearity from the cavity enhancement, and higher-order mechanical position terms in the expansion of the cavity frequency. I then propose a scheme for measuring mechanical position using general-dyne detection, applicable to pulsed and continuous measurements. This predicts a new regime of operation, the “stochastic Gaussian” regime. Finally, I discuss a protocol for deterministic mechanical squeezing that utilizes the cavity response.
The coupling of nanomechanical resonators to controllable quantum systems represents a growing and promising area of research. Recent advances in this field have brought to astonishing results, such as the initialization of a mechanical resonator into its quantum ground state and even the preparation of non-classical coherent states of motion. These achievements open up appealing scenarios to quantum information technologies and to the exploration of the quantum-classical boundary. From an application perspective, such quantum-mechanical hybrid systems provide a versatile and attractive tool for a variety of precision measurements, like ultra-sensitive detection of force, mass, and displacement. \n \nQuantum control over a mechanical resonator, or, conversely, the prospect of using resonator's motion for probing quantum states, both involve some tight requirements. First of all, the interaction between the mechanics and its quantum partner has to be large on the scale of the decoherence rates of the coupled systems. In most cases, the coupling mechanism has to be activated by engineering the resonator with electrodes, magnets, or mirrors, or by using tailored laser fields. For this reason, the search for a strong coupling typically competes with the requirement of overcoming decoherence effects. In addition, for quantum effects to be observable, strong coupling has to be accompanied by the preparation of zero entropy initial states, for instance by cooling the resonator into its ground state of motion. \n \nThe motivation pursued by this thesis is to contribute to the inspiring field of hybrid systems by walking through each of the aforementioned directions. We in fact demonstrate a promising system in which optically active quantum dots, embedded in fully self-assembled core-shell nanowires, are coupled to the nanowire motion. Mechanical vibrations of the nanowire modulate the quantum dot emission energy over a broad range exceeding 14 meV, by means of deformation potential coupling. In our system, therefore, both the coupling mechanism and the quantum states themselves are intrinsic to the resonator's structure. Besides revealing unusually strong, such a built-in opto-mechanical interaction produces a hybrid system whose inherent coherence is unspoiled by any functionalization or external field and whose fabrication is simpler than top-down techniques. \n \nWe further demonstrate the use of a quantum point contact as a displacement transducer to measure and control the low-temperature thermal motion of a nearby micromechanical cantilever. We show that by including the QPC in a suitable feedback loop, we are able to cool the cantilever's fundamental mechanical mode down to the level of the measurement noise, achieving a squashing of the QPC noise at high gain. Due to its off-board design, our system is particularly versatile and suitable to force-sensing applications. Since the QPC transducer is sensitive to local modifications of the nearby electric field, our approach is in principle compatible with any nanoscale resonator, without requiring any functionalization to activate the coupling. By improving the performance of the QPC as a one-dimensional conductor and the cantilever-QPC capacitive coupling, our system has the potential to achieve quantum-limited displacement resolution and ground state cooling. We then report on some ongoing attempts to overcome the current limitations of our system and couple mechanical motion to different mesoscopic transport devices. \n \nWe remark that our demonstration of an as-grown quantum-dot-in-nanowire hybrid system opens up bright prospects on future experiments, as also testified by the very recent ferment of the scientific community around this topic. We find that the opto-mechanical coupling rate is not far from the nanowire mechanical frequency. This fact makes our system particularly promising for the quantum non-demolition readout of a quantum dot state through a measurement of the nanowire position. On the other hand, we show that the coupling can be further optimized, and the nanowire mechanical heating rate reduced, thus disclosing the captivating perspective of using quantum dots to probe and control the mechanical state of a nanowire. In this context, it would be important to investigate a possible spin-oscillator coupling in our system, given the long coherence time offered by a spin state in a quantum dot. The wide range of control over the quantum dots emission energy and the ability to tune two neighboring dots into resonance pave the way to mechanically induced emitter-emitter coupling. In addition, our monolithic opto-mechanical system constitutes a good candidate for recent proposals of a tripartite hybrid system, which would integrate an optical cavity, a quantum two-level system and a mechanical resonator. The intrinsically strong coupling between the quantum dots and the nanowire motion would enhance the interaction between the mechanics and the cavity field, leading for instance to efficient cooling of the resonator to the ground state. Finally, the quantum dot sensitivity to the nanowire resonant vibration could also support the use of our system as an integrated force probe or as a nanomechanical mass sensor. In other words, the results reported in this dissertation constitute not only a relevant proof-of-principle, moreover they open up intriguing challenges for future research.
Quantum entanglement and quantum superposition are fundamental properties of quantum mechanics, which underline quantum information and quantum computation. Preparing quantum states in the macroscopic level is both conceptually interesting for extending quantum physics to a broader sense and fundamentally important for testing the validity of quantum mechanics. In this dissertation, schemes of preparing macroscopic entanglement and macroscopic superposition states in cavity optomechanics are studied using the unitary evolution method in the nonlinear regime or Lyapunov equation in the linearized regime. Quantum entanglement and quantum superposition states can be realized using experimentally feasible parameters with the proposals in this dissertation.\nFirstly, a scheme of entangling two movable end mirrors in a Fabry-Perot cavity that are coupled to a common single photon superposition state is studied. It is shown that strong entanglement can be obtained either in the single-photon strong coupling regime deterministically or in the single-photon weak coupling regime conditionally.\nSecondly, a scheme of entangling two movable end mirrors, that are coupled to two-mode entangled fields generated from a correlated-emission laser is investigated. By tuning the input driving laser frequencies at the Stokes sidebands of the cavity, the radiation-pressure coupling can be linearized as an effective beam-splitter-like interaction. Hence entanglement can be transferred from the two-mode fields to the two mechanical mirrors. Macroscopic entanglement between macroscopic mirrors persists at temperature ~ 1K.\nThirdly, a scheme of creating macroscopic quantum superpositions of a mechanical mirror via periodically flipping a photonic qubit is proposed. Quantum superposition states of a mechanical mirror can be obtained via the nonlinear radiation coupling with a single-photon superposition state. However, the difference between two superposed mechanical states is very small due to the weak single-photon coupling rate available in experiment. By periodically flipping the photonic qubit state, the difference can be magnified. It is shown in detail that this scheme is experimentally feasible under current technology.
In this dissertation, I theoretically investigate the open system dynamics of cavity optomechanical systems in the quantum limit, where a mechanical resonator couples to a cavity mode via radiation pressure force. Recent developments in nano-fabrication and cooling techniques make it possible to optically control and manipulate the motion of micro- and nano-mechanical resonator. Several experiments have demonstrated the possibility of preparing macroscopic mechanical resonators into their quantum ground state, which makes optomechanical systems an ideal candidate for studying the quantum behavior of macroscopic objects. One important direction in quantum optomechanics is the study of the decoherence of optomechanical system due to the interaction with their external environments. This dissertation explores the decoherence effects by considering the influence of the radiation pressure coupling on the interaction between optomechanical system and its environments. Because the effects of the nonlinear interaction vary with the optomechanical coupling strength, three different interaction regimes are fully studied here: the weak coupling, the intermediate coupling and the strong coupling.
Cavity optomechanics originated from the research of interferometric detection of gravitational waves, and later became a fast-growing area of techniques and approaches ranging from the fields of atomic, molecular, and optical physics to nano-science and condensed matter physics as well. Recently, it focused on the exploration of operating mechanical oscillators deep in the quantum regime, with an interest ranging from quantum-classical interface tests to high-precision quantum metrology. In this paper, recent theoretical work of our group in the field of quantum measurement with cavity optomechanical systems is reviewed. We explore the quantum measurement theory and its applications with several unconventional cavity optomechanical schemes working in the quantum regime. This review covers the basics of quantum noises in the cavity optomechanical setups and the resulting standard quantum limit of precision displacement and force measurement. Three novel quantum measurement proposals based on the hybrid optomechanical system are introduced. First, we describe a quantum back-action insulated weak force sensor. It is realized by forming a quantum-mechanics-free subsystem with two optomechanical oscillators of reversed effective mass. Then we introduce a role-reversed atomic optomechanical system which enables the preparation and the quantum tomography of a variety of non-classical states of atoms. In this system, the cavity field acts as a mechanical oscillator driven by the radiation pressure force from an ultracold atomic field. In the end, we recommend a multimode optomechanical transducer that can detect intensities significantly below the single-photon level via adiabatic transfer of the microwave signal to the optical frequency domain. These proposals demonstrate the possible applications of optomechanical devices in understanding of quantum-classical crossover and in achieving quantum measurement limit.