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Advances in Optical Sciences Congress

Material slow light does not enhance Beer-Lambert absorption

Sanghoon Chin, Isabelle Dicaire, Jean‐Charles Beugnot, Stella Foaleng Mafang, M. G. Herraez, Luc Thévenaz A

Published Jan 1, 2009• 12 citations
Publisher

Abstract

We experimentally demonstrate that material slow light does not enhance Beer-Lambert absorption. A 26% group velocity reduction induced by stimulated Brillouin scattering in a gas-filled microstructured fiber caused no observable change in the measured absorption.
DOI
10.1364/sl.2009.sma3

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The absorption of light by a gas molecule has been measured comparatively using light propagating in normal conditions and in a slow light regime. The experiment is designed to make the 2 measurements possible without modifying the interaction conditions, so that the sole effect of slow light is unambiguously observed. A 26% group velocity reduction induced by stimulated Brillouin scattering in a gas-filled microstructured fiber caused no observable change in the measured absorption, so that it is proved that material slow light does not enhance Beer-Lambert absorption and has a null impact on gas sensing or spectroscopic applications.
The group velocity at which light pulses propagate through a dispersive material system is very different from the vacuum speed of light c, One refers to light as being "slow" for v g << c (Boyd & Gauthier, 2009) or "fast" for v g > c or v g <0 (Stenner et al, 2003 ).For v g <0, the pulse envelope appears to travel backward in the material (Gehring et al, 2006), and hence it is sometimes referred to as "backward light."The subject of slow light has caused keen interest in the past decade or more, and it is possible to control the group velocity of light pulses in the dispersive materials.Interest in slow and fast light dates back to the early days of the 20th century.Sommerfeld and Brillouin (Sommerfeld & Brillouin, 1960) were intrigued by the fact that theory predicts that v g can exceed c, which leads to apparent inconsistencies with Einstein's special theory of relativity.Experimental investigations of extreme propagation velocities were performed soon after the invention of the laser (Faxvog and et al, 1970).In 1999, Harris's group research work greatly stimulated researchers' interests, which showed that light could be slowed down to 17m/s.The result was obtained in ultra cold atom clouds with the use of electromagnetically induced transparency (EIT), which induces transparency in a material while allowing it to retain strong linear and nonlinear optical properties (Hau et al, 1999).Slow light can also be obtained through the use of the optical response of hot atomic vapors (Philips et al, 2001).These early research works require hard conditions and the slow light cannot operate in room temperature.Recently, researchers found ways to realize slow light operating in room temperature and solid-state materials, which are more suited for many practical applications, namely slow light via stimulated Brillouin scattering(SBS), slow light via coherent population oscillations (CPO), tunable time delays based on group velocity dispersion or conversion/ dispersion(C/D), slow light in fiber Bragg gratings and so on.In this chapter, we describe some of the physical mechanisms that can be used to induce slow and fast light effects in room-temperature solids (Bigelow et al, 2003) and some of the exotic propagation effects that can thereby be observed.We also survey some applications of slow and fast light within the fields of quantum electronics and photonics. Fundamentals of slow and fast lightSlow and fast light refer to the group velocity of a light wave.The group velocity is the velocity most closely related to the velocity at which the peak of a light pulse moves through an optical dispersive material (Milonni, 2005), and is given by the standard result www.intechopen.comRecent Progress in Optical Fiber Research 82where n is the refractive (phase) index and ω is the angular frequency of the carrier wave of the light field.One refers to light as being slow light for v g << c, fast light for for v g > c, and backwards light for v g <0 or v g is negative.Extreme values of the group velocity invariably rely on the dominance of the second contribution to the group index of Equation ( 1).This contribution of course results from the frequency dependence of the refractive index, and for this reason extreme values of the group velocity are usually associated with the resonant or near-resonant response of material systems.According to this theory, slow light is expected in the wings of an absorption line and fast light is expected near line center, and the spatial dispersion, that is, the non-locality in space of the medium response, is another mechanism that can lead to slow light, as has been predicted (Kocharovskaya et al,2001) and observed (Strekalov et al, 2001).We catalogue the main methods to realize slow light in room temperature solid, namely slow light via stimulated Brillouin scattering(SBS), slow light via coherent population oscillations (CPO), tunable time delays based on group velocity dispersion or conversion/ dispersion(C/D), slow light in fiber Bragg gratings and so on.We will describe CPO and SBS slow light in more details.