The absorption of light by a gas molecule has been measured comparatively using light propagating in normal conditions and in a slow light regime. The experiment is designed to make the 2 measurements possible without modifying the interaction conditions, so that the sole effect of slow light is unambiguously observed. A 26% group velocity reduction induced by stimulated Brillouin scattering in a gas-filled microstructured fiber caused no observable change in the measured absorption, so that it is proved that material slow light does not enhance Beer-Lambert absorption and has a null impact on gas sensing or spectroscopic applications.
The absorption of light by a gas molecule has been measured comparatively using light propagating in normal conditions and in a slow light regime. The experiment is designed to make the 2 measurements possible without modifying the interaction conditions, so that the sole effect of slow light is unambiguously observed. A 26% group velocity reduction induced by stimulated Brillouin scattering in a gas-filled microstructured fiber caused no observable change in the measured absorption, so that it is proved that material slow light does not enhance Beer-Lambert absorption and has a null impact on gas sensing or spectroscopic applications.
The group velocity at which light pulses propagate through a dispersive material system is very different from the vacuum speed of light c, One refers to light as being "slow" for v g << c (Boyd & Gauthier, 2009) or "fast" for v g > c or v g <0 (Stenner et al, 2003 ).For v g <0, the pulse envelope appears to travel backward in the material (Gehring et al, 2006), and hence it is sometimes referred to as "backward light."The subject of slow light has caused keen interest in the past decade or more, and it is possible to control the group velocity of light pulses in the dispersive materials.Interest in slow and fast light dates back to the early days of the 20th century.Sommerfeld and Brillouin (Sommerfeld & Brillouin, 1960) were intrigued by the fact that theory predicts that v g can exceed c, which leads to apparent inconsistencies with Einstein's special theory of relativity.Experimental investigations of extreme propagation velocities were performed soon after the invention of the laser (Faxvog and et al, 1970).In 1999, Harris's group research work greatly stimulated researchers' interests, which showed that light could be slowed down to 17m/s.The result was obtained in ultra cold atom clouds with the use of electromagnetically induced transparency (EIT), which induces transparency in a material while allowing it to retain strong linear and nonlinear optical properties (Hau et al, 1999).Slow light can also be obtained through the use of the optical response of hot atomic vapors (Philips et al, 2001).These early research works require hard conditions and the slow light cannot operate in room temperature.Recently, researchers found ways to realize slow light operating in room temperature and solid-state materials, which are more suited for many practical applications, namely slow light via stimulated Brillouin scattering(SBS), slow light via coherent population oscillations (CPO), tunable time delays based on group velocity dispersion or conversion/ dispersion(C/D), slow light in fiber Bragg gratings and so on.In this chapter, we describe some of the physical mechanisms that can be used to induce slow and fast light effects in room-temperature solids (Bigelow et al, 2003) and some of the exotic propagation effects that can thereby be observed.We also survey some applications of slow and fast light within the fields of quantum electronics and photonics. Fundamentals of slow and fast lightSlow and fast light refer to the group velocity of a light wave.The group velocity is the velocity most closely related to the velocity at which the peak of a light pulse moves through an optical dispersive material (Milonni, 2005), and is given by the standard result www.intechopen.comRecent Progress in Optical Fiber Research 82where n is the refractive (phase) index and ω is the angular frequency of the carrier wave of the light field.One refers to light as being slow light for v g << c, fast light for for v g > c, and backwards light for v g <0 or v g is negative.Extreme values of the group velocity invariably rely on the dominance of the second contribution to the group index of Equation ( 1).This contribution of course results from the frequency dependence of the refractive index, and for this reason extreme values of the group velocity are usually associated with the resonant or near-resonant response of material systems.According to this theory, slow light is expected in the wings of an absorption line and fast light is expected near line center, and the spatial dispersion, that is, the non-locality in space of the medium response, is another mechanism that can lead to slow light, as has been predicted (Kocharovskaya et al,2001) and observed (Strekalov et al, 2001).We catalogue the main methods to realize slow light in room temperature solid, namely slow light via stimulated Brillouin scattering(SBS), slow light via coherent population oscillations (CPO), tunable time delays based on group velocity dispersion or conversion/ dispersion(C/D), slow light in fiber Bragg gratings and so on.We will describe CPO and SBS slow light in more details.
Dynamic control of the speed of a light signal, based on stimulated Brillouin scattering in optical fibers, was theoretically studied and also experimentally demonstrated as the core object of this thesis. To date, slow light based on stimulated Brillouin scattering has shown the unmatched flexibility to offer an efficient timing tool for the development of all-optical future router. Nevertheless, the seeming perfect Brillouin slow light suffered from three major obstacles: naturally narrow signal bandwidth, strong change of signal amplitude, and significant signal distortion. The essential contribution of this work has been mostly dedicated to resolve all those impairments so as to make Brillouin slow light a completely operating all-optical delay line for practical applications. Actually, high capability of tailoring the spectral distribution of the effective Brillouin resonance makes possible to resolve partially or completely all those problems. First of all, a broadband spectral window was passively obtained in between two Brillouin gain/loss resonances by simply appending two segments of fibers showing different Brillouin frequency shifts. The global Brillouin gain of the concatenated fibers manifests a gain/loss doublet resonance showing a broad window in between gain/loss peaks. In practice, this configuration has a crucial advantage that it removes the need of the pump modulation, generally used to create a polychromatic pump source. Therefore, a broadband Brillouin slow and fast light was simple realized with a reduced distortion. Secondly, the signal amplification or attenuation associated to the signal delay was completely compensated by superposing Brillouin gain and loss resonances with identical depth but different width. As a result, the Brillouin gain led to effectively a spectral hole in the center of the broadband absorption and opened a transparent window while the sharp change in the refractive index was preserve. This way it makes possible to realize zero-gain Brillouin slow light. This configuration was also exploited to produce Brillouin fast light with a total absence of signal loss, simply by swapping the spectral position of the two pumps. At last, a signal was continuously delayed through a Brillouin fiber delay line without any distortion. Due to the strong induced dispersion, pulse broadening is a major difficulty in all slow light systems and it is impossible to compensate such broadening using a linear system. Therefore, a conventional Brillouin slow light system was combined with a nonlinear optical fiber loop mirror that gives a nonlinear quadratic transmission. Using this configuration, the inevitable pulse broadening was completely compensated at the output of the loop and a signal was delayed up to one symbol without any distortion. Brillouin slow light systems were further studied in the spectral domain. For a given Brillouin resonance the spectrum of a light pulse was optimized to better match the Brillouin bandwidth. When the time envelope of a pulse was properly shaped, it was clearly observed that the spectral width of the pulse became minimized while preserving the pulse duration. This way the maximum time delay through Brillouin slow light could be enhanced for a fixed pulse width. Brillouin fast light was even realized in total absence of any pump source, which is a plain requirement for the generation of Brillouin slow or fast light. This self-generated delay line, key contribution of this thesis, relies on both spontaneous and stimulated Brillouin scattering in optical fibers. In this implementation, a light signal was strongly boosted above the so-called Brillouin threshold, so that most power of the signal was transferred to a backward propagating wave, namely the generation of amplified spontaneous Stokes wave. Since the center frequency of the intense Stokes wave is below the signal frequency by exactly Brillouin shift of the fiber used, this wave led to a Brillouin loss band centered at the signal frequency. Consequently, the signal experienced fast light propagation and the propagation velocity of the signal was self-controlled, simply by varying the signal input power. This technique has many practical advantages such as its high simplicity of the configuration and an invariant signal power in the output of this delay line. Additionally, this system self-adapts the signal bandwidth as the spectrum of the amplified Stokes wave matches the spectral distribution of the signal. An alternative method to generate all-optical delay line was proposed instead of slow light. This scheme makes use of the combination of wavelength conversion and group velocity dispersion. This type of delay line was mainly aimed at improving the storage capability of delaying element. The wavelength of a signal was simply and efficiently converted at a desired wavelength using cross gain modulation in semiconductor optical amplifiers. Then the converted signal was delivered to a high dispersive medium and arrived at the end of the medium with relative time delay due to the group velocity dispersion. A fractional delay of 140 was continuously produced through this delay line for a signal with a duration of 100 ps, preserving signal bandwidth and wavelength. The effect of slow light on linear interactions between light and matter was experimentally investigated to clarify the current scientific argument regarding slow light-enhanced Beer-Lambert absorption. It was predicted that real slowing of the light group velocity could enhance the molecular linear absorptions so as to improve the sensitivity of this type of sensing. However, the experimental results unambiguously show that material slow light (slow light in traveling wave media) does not enhance the Beer-Lambert absorption.
Optical frequency references are devices providing well-defined and stable optical frequency responses to incoming radiation for applications such as high-precision spectroscopy and optical fibre communications. To stabilise the emission frequency of lasers, which drifts with time mostly because of fluctuations in temperature and mechanical vibrations, atomic and molecular optical transitions can be used since they show precise and well-defined frequency responses to incoming radiation. However from a practical standpoint conventional gas cell devices cannot be easily integrated into existing optical systems because of their bulky dimensions. To replace conventional absorption cells, photonic crystal fibres filled with gas-phase material are promising devices owing to their robustness, reliability, and portable characteristics. In addition they can be directly embedded into existing optical systems and they perform well in harsh environments. In this experimental study, optical gas-phase frequency references based on photonic crystal technology are realised. The gas-sensing properties of different photonic crystal fibre samples are studied and the long-term stability and reliability of fibre gas cells are demonstrated. In addition an analytical model predicting the gas-filling time in photonic crystal fibres (PCF) is developed and can be applied to any type of fibre, fibre geometry, or length. Then fibre gas cells filled with acetylene gas, a recognised frequency reference gas-phase material, have been prepared to conduct fundamental research on slow & fast light generation in optical fibres to verify the possibilities of slow light in enhancing light-matter interaction. The group velocity of light is controlled by modifying the material and structural dispersive properties of the PCF absorption cells through stimulated Brillouin scattering and cavity ring resonators, respectively. We could demonstrate that material slow light has no impact on the molecular absorption effect whereas structural slow light has an impact on the absorption efficiency scaling linearly with the group index. Such radically different responses to slow light suggest that group velocity is not the universal physical quantity scaling light-matter interaction, and that the optical absorption of molecules is more closely related to the velocity of the electromagnetic energy. Finally the impact of slow light on the molecular absorption efficiency is also evaluated in dispersion-engineered photonic crystal waveguides. We demonstrate that in planar photonic crystal waveguides the field enhancement and its evanescent fraction have more impact on the absorption efficiency than the reduction of the group velocity of light.
The manipulation of the group velocity of optical signals (slow and fast light) has many possible applications in telecommunications, sensing, nonlinear optics, and so on. The exploitation of the effect of stimulated Brillouin scattering (SBS) is of special interest for the alteration of the group velocity in optical fibers, since it just requires standard telecom equipment and low-to-moderate optical power. However, each delay in one single, low-gain SBS-based slow-light system is accompanied by a pulse broadening. This is a result of the inherent Kramers–Kronig relations among the gain, the phase change, and the accompanied group velocity. For an ideal flat gain, the phase change is nonideal, and for an ideal phase change the gain curve leads to a broadening. Furthermore, if the gain bandwidth is adapted to the signal by broadening, the delay will be reduced. Thus the signal broadening can be reduced by several methods for one single low-gain slow-light system, but it cannot be zero. Here, we will show how a zero-broadening SBS-based slow light can be achieved with several methods. The basic idea is a reshaping of the original pulse in a second stage by saturation of the SBS system, or by the superposition of two gains. As will be shown, all of these systems show an almost ideal overall gain and phase function over the bandwidth of the pulses. Thus, SBS-based slow light with a delay bandwidth product of 1 bit and zero distortion is possible.