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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Dipole-dipole interactions experiment with a few cold Rb Rydberg atoms

Vasily M. Entin, Denis B. Tretyakov, Ilya I. Beterov, I. I. Ryabtsev

Published Jun 1, 2009• 0 citations
Publisher

Abstract

The aim of this paper is to realize excitation in a small volume, development of diagnostic methods for cold Rydberg atoms, spectroscopy of the microwave transitions between Rydberg states in the presence of the magneto-optical trap (MOT) quadrupole magnetic field, as well as observation of dipole-dipole interaction of a small number of Rydberg atoms.

DOI
10.1109/cleoe-eqec.2009.5191655

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The aim of this paper is to realize excitation in a small volume, development of diagnostic methods for cold Rydberg atoms, spectroscopy of the microwave transitions between Rydberg states in the presence of the magneto-optical trap (MOT) quadrupole magnetic field, as well as observation of dipole-dipole interaction of a small number of Rydberg atoms.
This paper reports on the results of experiments with cold rubidium Rydberg atoms in a magneto-optical trap. The specific feature of the experiments is the excitation of Rydberg atoms in a small volume within a cloud of cold atoms and the sorting of measured signals and spectra according to the number of detected Rydberg atoms. The effective lifetime of the 37 P Rydberg state and its polarizability in a weak electric field are measured. The results obtained are in good agreement with theoretical calculations. It is demonstrated that the localization of the excitation volume in the vicinity of the zero-magnetic-field point makes it possible to improve the spectral resolution and to obtain narrow microwave resonances in Rydberg atoms without switching off the quadrupole magnetic field of the trap. The dependence of the amplitude of dipole-dipole interaction resonances in Rydberg atoms on the number of atoms is measured. This dependence exhibits a linear behavior and agrees with the theory for a weak dipole-dipole interaction.
I hereby declare that I am the sole author of this thesis. This is a true copy of the thesis, including any required final revisions, as accepted by my examiners. I understand that my thesis may be made electronically available to the public. ii This thesis reports the first observation of the resonant electric dipole-dipole interaction between cold Rydberg atoms using microwave spectroscopy, the observation of the magnetic field suppression of resonant interactions, and the development of a unique technique for precise magnetic field measurements. ARydbergstate(46d 5/2) of laser cooled 85 Rb atoms has been optically excited. A fraction of these atoms has been transferred to another Rydberg state (47p 3/2 or 45f 5/2,7/2) to introduce resonant electric dipole-dipole interactions. The line broadening of the two-photon 46d 5/2 − 47d 5/2 microwave transition due to the interaction of 46d 5/2 with 47p 3/2 or 45f 5/2,7/2 atoms has been used as a probe of the interatomic interactions. This experiment has been repeated with a DC magnetic field applied. The application of a weak magnetic field ( ≤ 0.6 G) has reduced
Resonant electric dipole-dipole interactions between cold Rydberg atoms were observed using microwave spectroscopy. Laser-cooled 85Rb atoms in a magneto-optical trap were optically excited to 45d(5/2) Rydberg states using a pulsed laser. A microwave pulse transferred a fraction of these Rydberg atoms to the 46p(3/2) state. A second microwave pulse then drove atoms in the 45d(5/2) state to the 46d(5/2) state, and was used as a probe of interatomic interactions. The spectral width of this two-photon probe transition was found to depend on the presence of the 46p(3/2) atoms, and is due to the resonant electric dipole-dipole interaction between 45d(5/2) and 46p(3/2) Rydberg atoms.
This dissertation consists of three microwave spectroscopy experiments performed with cold Rb Rydberg atoms in Magneto Optical Trap.The first experiment is a systematic study of a particular type of transition which was first observed in 2012 that involves a pair of Rydberg atoms.In this transition, even though only one microwave photon is absorbed, both atoms in the pair change states.In particular, we describe the transition with the configuration interaction (CI) model and experimentally verify the scaling of fractional population transfer predicted by the CI model.The second experiment builds on the first experiment and reports observations of additional single and multi photon microwave transitions that are allowed due to the same CI as in the first experiment.The observations show clearly that this type of transition involving a pair of Rydberg atoms are a lot more common than initially thought.We show that the transitions can be conveniently described as Forster resonances of Floquet states.The last experiment reports on the technique we used to measure the ng and nh series quantum defects and the ionic dipole and quadrupole polarizabilities of 85 Rb.The technique allows us to obtain zero field intervals of (n + 1)d 5/2 → ng and (n + 1)d 5/2 → nh intervals despite the fact that we can only control the stray electric field in one direction.Using the technique, the quantum defects of ng and nh were determined to be 0.0039741(16) and 0.0014066(57), respectively.The ionic II dipole and quadrupole polarizabilities were determined to be 9.12(2)a 3 0 and 14(3)a 5 0 , respectively.
Atoms in highly excited (Rydberg) states have a number of unique properties which make them attractive for applications in quantum information.These are large dipole moments, lifetimes and polarizabilities, as well as strong long-range interactions between Rydberg atoms.Experimental methods of laser cooling and precision spectroscopy enable the trapping and manipulation of single Rydberg atoms and applying them for practical implementation of quantum gates over qubits of a quantum computer based on single neutral atoms in optical traps.In this paper, we give a review of the experimental and theoretical work performed by the authors at the Rzhanov Institute of Semiconductor Physics SB RAS and Novosibirsk State University on laser and microwave spectroscopy of cold Rb Rydberg atoms in a magneto-optical trap and on their possible applications in quantum information.We also give a brief review of studies done by other groups in this area.