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The European Physical Journal Applied Physics

High-Q photonic crystal nanocavities on diamond for quantum electrodynamics

Igal Bayn, J. Salzman

Published Nov 14, 2006• 19 citations
Publisher

Abstract

A slab two-dimensional photonic crystal in diamond is being considered for quantum information processing. In view of the low refractive index of diamond, the question whether a high Q cavity is achievable has to be addressed. Here, various geometrical designs of single point defects and double heterostructures for the formation of high Q nanocavities in diamond are modeled. The highest value of vertical quality factor was achieved in double heterostructures. This result seems to be significant for further consideration of photonic crystals in diamond for quantum electrodynamics applications.

DOI
10.1051/epjap:2006131

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A slab two-dimensional photonic crystal in diamond is being considered for quantum information processing. In view of the low refractive index of diamond, the question whether a high Q cavity is achievable has to be addressed. Here, various geometrical designs of single point defects and double heterostructures for the formation of high Q nanocavities in diamond are modeled. The highest value of vertical quality factor was achieved in double heterostructures. This result seems to be significant for further consideration of photonic crystals in diamond for quantum electrodynamics applications.
Diamond photonics provides an attractive architecture to explore room temperature cavity quantum electrodynamics and to realize scalable multi-qubit computing. Here, we review the present state of diamond photonic technology. The design, fabrication and characterization of a novel nanobeam cavity produced in a single crystal diamond are demonstrated. The present cavity design, based on a triangular cross-section, allows vertical confinement and better signal collection efficiency than that of slab-based nanocavities and eliminates the need for a pre-existing membrane. The nanobeam is fabricated by focused-ion-beam (FIB) patterning. The cavity is characterized by confocal photoluminescence. The modes display quality factors of Q ∼220 and deviate in wavelength by only ∼1.7 nm from the nitrogen-vacancy (NV − ) color center zero phonon line (ZPL). The measured results are found to be in good agreement with three-dimensional finite-difference-time-domain (FDTD) calculations. A more advanced cavity design with Q =22 000 is modeled, showing the potential for high- Q implementations using the triangular geometry. The prospects of this concept and its application in spin non-demolition measurement and quantum computing are discussed.
We demonstrate the controlled coupling of a single diamond nanocrystal to a planar photonic crystal double-heterostructure cavity. A dip-pen deposition method and subsequent manipulation with an atomic force microscope was used to precisely position the nanocrystal on top of the cavity. The optical properties of this combined system are investigated with regard to changes in the quality factor and resonance wavelength of the cavity mode as a function of the size and relative position of the diamond nanocrystal. These studies represent an important step toward well-controlled cavity-QED experiments with single-defect centers in diamond.
Abstract : This report summarizes our recent progress on the development of photonic nanostructures for sensing and information processing. We have developed a nitrogen vacancy (NV) spin qubit-cavity system in the strong Purcell regime in which the spin qubit predominantly interacts with the cavity mode. This system is realized in a single-crystal diamond photonic crystal nanocavity with quality factors (Q) up to 104. Furthermore, we measure electron spin coherence times of cavity-coupled NVs of 200 us. We have also developed techniques for NV-based super-resolution imaging and precision sensing, using high-speed parallel readout on a microscope camera; and we have developed techniques for precision clocks based on collective oscillation of ensembles of NVs. We also report on graphene electro-optic devices and sensors.
Recently, developments in novel and high-purity materials allow for the presence of a single, solitary crystalline defect to define the electronic, magnetic, and optical functionality of a device. The discrete nature of the active dopant, whose properties are defined by a quantum mechanical description of its structure, enables radically new quantum investigations and applications in these arenas. Finally,there has been significant development in large-scale device engineering due to mature semiconductor manufacturing techniques. The diverse set of photonic device architectures offering light confinement, guiding, and extraction is a prime example. These three paradigms – solitary dopant photonics and optoelectronics (solotronics), quantum science\tand technology, and device engineering – merge in the development of novel quantum photonic devices for the next generation of information processing systems. We present in this thesis a series of investigations of optical nanostructures for single optically active spins in single crystal diamond. Chapter 1 introduces the Nitrogen-Vacancy (NV) color center, summarizes its applications, and motivates the need for their integration into photonic structures. Chapter 2 describes two prototype nanobeam photonic crystal cavities for generating strong light-matter interactions with NV centers. The first device consists of a silicon nitride photonic crystal nanobeam cavity with high quality factor \\(Q \\sim 10^5\\) and small mode volume \\(V \\sim 0.5*(\\lambda/n)^3\\). The second device consists of a monolithic diamond nanobeam cavity fabricated with the focused ion beam (FIB) directly in a single crystal diamond sample. Chapter 3 presents a high-efficiency source of single photons consisting of a single NV center in a photonic diamond nanowire. Early FIB prototypes are described, as is the first successful realization of the device achieved via reactive ion etching nanowires in a single crystal diamond containing NV centers, and finally a variation of this approach based on incorporation of NV centers in pure diamond via ion implantation. In chapter 4 we consider the optimal design of photonic devices offering both collection efficiency and cavity-enhancements and extend the model of the NV center to include photonic effects. In chapter 5 we briefly introduce a novel optically active spin discovered in a diamond nanowire. Finally, in chapter 6 we conclude with several proposals to extend this research program.