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Raman transitions in cavity QED

A. David. Boozer

Published May 31, 2005• 6 citations
Publisher

Abstract

In order to study quantum effects such as state superposition and entanglement, one would like to construct simple systems for which the damping rates are slow relative to the rate of coherent evolution. One such system is strong-coupling cavity quantum electrodynamics (QED), in which a single atom is coupled to a single mode of a high finesse optical cavity. In recent years, optical trapping techniques have been applied to the cavity QED system, allowing an individual atom to remain coupled to the cavity for long periods of time. For the purpose of future cavity QED experiments, one would like to gain as much control over the trapped atom as possible; in particular, one would like to cool the center of mass motion of the atom, to measure the magnetic field at the location of the atom, and to be able to prepare the atom in a given internal state. In the first part of this thesis, I present a scheme for driving Raman transitions inside the cavity that can be used to achieve these goals. After giving a detailed theoretical treatment of the Raman scheme, I describe how it can be implemented in the lab and discuss some preliminary experimental results. In the second part of this thesis, I present a number of simple field theory models. These models were developed in an attempt to understand some of the central ideas of theoretical physics by looking at how the ideas work in a highly simplified context. The hope is that by reducing the mathematical complexity of an actual theory, the underlying physical concepts can be more easily understood.

DOI
10.7907/f2wh-x491

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In order to study quantum effects such as state superposition and entanglement, one would like to construct simple systems for which the damping rates are slow relative to the rate of coherent evolution. One such system is strong-coupling cavity quantum electrodynamics (QED), in which a single atom is coupled to a single mode of a high finesse optical cavity. In recent years, optical trapping techniques have been applied to the cavity QED system, allowing an individual atom to remain coupled to the cavity for long periods of time. For the purpose of future cavity QED experiments, one would like to gain as much control over the trapped atom as possible; in particular, one would like to cool the center of mass motion of the atom, to measure the magnetic field at the location of the atom, and to be able to prepare the atom in a given internal state. In the first part of this thesis, I present a scheme for driving Raman transitions inside the cavity that can be used to achieve these goals. After giving a detailed theoretical treatment of the Raman scheme, I describe how it can be implemented in the lab and discuss some preliminary experimental results. In the second part of this thesis, I present a number of simple field theory models. These models were developed in an attempt to understand some of the central ideas of theoretical physics by looking at how the ideas work in a highly simplified context. The hope is that by reducing the mathematical complexity of an actual theory, the underlying physical concepts can be more easily understood.
We present two schemes for driving Raman transitions between the ground-state hyperfine manifolds of a single atom trapped within a high-finesse optical cavity. In both schemes, the Raman coupling is generated by standing-wave fields inside the cavity, thus circumventing the optical access limitations that free-space Raman schemes must face in a cavity system. These cavity-based Raman schemes can be used to coherently manipulate both the internal and motional degrees of freedom of the atom, and thus provide powerful tools for studying cavity quantum electrodynamics. We give a detailed theoretical analysis of each scheme, both for a three-level atom and for a multilevel cesium atom. In addition, we show how these Raman schemes can be used to cool the axial motion of the atom to the quantum ground state, and we perform computer simulations of the cooling process.
Cavity quantum electrodynamics (QED) in the strong-coupling regime provides the opportunity to monitor and control the dynamics of a simple quantum system. A single Cesium atom interacts strongly with single-photon fields in the mode of a high-finesse optical cavity. When the resulting coherent coupling rate dominates dissipation in the system, strong coupling is realized and the system displays distinctively quantum behavior. The coupling between atomic internal states and the quantized cavity field allows for diverse protocols in quantum state preparation, quantum communication, and quantum logic. However, the atom's external or motional state must also be taken into account. My research develops cavity QED in the limit where the coherent atom-field coupling dominates the atomic kinetic energy and thus significantly affects the atomic center-of-mass motion. In this regime, the interaction of the atom with the cavity field provides both a means of controlling atomic motion and a signal for detecting that motion in real time with high signal-to-noise. The sensing capability of the ``atom-cavity microscope" is exploited to trap single atoms with single-photon fields and to monitor their orbits in real time as they are bound in the cavity. Such real-time position sensing is the basis for a detailed strategy and ongoing experiment to actively stabilize select aspects of an atom's motion within the cavity. As the cavity-enabled position measurement approaches the standard quantum limit, this work begins to realize a quantum servo for atomic position and to address questions of optimal state estimation and state preparation. In combination with other progress in cavity QED, it furthers the goal of controlled atom-field interactions for quantum information science.
The experiments discussed in this thesis focus on the interaction of a single trapped atom with the single mode of a high-finesse optical cavity, in the regime of strong coupling. Chapter 1 gives a brief introduction, after which Chapter 2 describes our recent measurements of the transmission spectrum of the atom-cavity system. The spectrum exhibits a clearly resolved vacuum-Rabi splitting, in good quantitative agreement with theoretical predictions. A new Raman scheme for cooling atomic motion along the cavity axis enables a complete spectrum to be recorded for an individual atom trapped within the cavity mode, in contrast to all previous measurements of this type that have required averaging over 10^3-10^5 atoms. Chapter 3 discusses our observations of photon blockade for the transmitted light in the presence of one trapped atom. Excitation of the atom-cavity system by a first photon blocks the transmission of a second one, thereby converting an incident Poissonian stream of photons into a sub-Poissonian, anti-bunched stream, as confirmed by measurements of the photon statistics of the transmitted field. The intensity correlations of the cavity transmission also reveal the energy distribution for oscillatory motion of the trapped atom. Chapter 4 details a set of simple but necessary measurements of relevant experimental parameters such as cavity geometry, linewidth, mirror properties, birefringence, and detection efficiency. The thesis concludes with Appendix A, describing the efficient laser setup we use for our magneto-optical traps.
In recent years, remarkable advances in the science of laser cooling and trapping of atomic samples have lead to breakthroughs in quantum optics and, in particular, in cavity quantum electrodynamics (QED). The ability to optically trap an atom within the mode of a ultra-high finesse cavity of small mode volume for experimentally significant periods of time now allows for the continuous observation of fundamental quantum optical effects. This dissertation will focus on experiments conducted to fully characterize and exert quantum control over a strongly-coupled atom-cavity system consisting of single cesium atoms isolated by a dipole trapping in the mode of a Fabry-Perot optical resonator. In particular, we describe techniques developed and implemented for exerting coherent control over the internal and quantum motional state of these atoms using stimulated Raman processes. We also focus on the applications of this system to quantum networking and quantum information science, particularly within the context of coherently transferring quantum states from atom to quantum optical fields and back. Finally, we describe a series of measurements carried out to explore the characteristic dynamics of the Jaynes-Cummings Hamiltonian which governs the system. This includes spectroscopic measurement of the signature vacuum Rabi splitting for strongly-coupled cavity QED as well as evidence in the time domain for coherent Rabi nutation of excitation between atom and field on resonance.
We report on recent progress in our lab involving cavity quantum electrodynamics with optically trapped atoms. \n \nIn particular, we will focus on a recent measurement of the Vacuum-Rabi splitting for one atom strongly coupled to the field of a high finesse optical resonator. This splitting is characteristic of the normal modes in the eigenvalue spectrum of the atom-cavity system. A new Raman scheme for cooling atomic motion along the cavity axis enables a complete spectrum to be recorded for an individual atom trapped within the cavity mode, in contrast to all previous measurements in cavity QED that have required averaging over many atoms.
Cavity quantum electrodynamics (QED), the system of a single atom interacting with a single mode of a high finesse optical resonator, has tremendous potential for use in quantum logic, quantum information processing, and in enabling observation of quantum mechanical effects in the laboratory. The work of this thesis demonstrates a number of steps toward realizing these goals, by employing an experimental system with the strongest atom-field coupling achieved to date in optical cavity QED. The effects of strong coupling in cavity QED are studied for single cold atoms measured one at a time, in real time. The passage of single atoms through the cavity is employed to map out the frequency response of the system, and to demonstrate that quantum rather than semiclassical theory provides the correct theoretical model. The mechanical effects of strong coupling on single atoms are explored, these experiments demonstrating the first trapping of single atoms with single photons. Additionally, strong coupling enables high signal-to-noise ratio for monitoring atomic position at single photon field strengths; this capability is employed to investigate the motion of atoms trapped within the cavity. The transmitted cavity field is used to reconstruct the trajectories of single atoms, thereby realizing a new form of microscopy - the Atom-Cavity Microscope. Technical developments necessary to create the cavities used in this experiment are detailed. Ideas for future extensions to the experiment are proposed; a zero light-shift dipole force trap, and measurement of photon statistics of a single strongly coupled atom (which realizes a photon blockade device) are discussed.