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Physical Chemistry Chemical Physics

Rydberg dressing evolution via Rabi frequency control in thermal atomic vapors

Junling Che, Huaibin Zheng, Zhaoyang Zhang, Xin Yao, Cheng Li, Zhenkun Wu, Yanpeng Zhang

Published Jan 1, 2014• 4 citations
Publisher

Abstract

We report for the first time the theoretical and experimental research on Rydberg electromagnetically induced transparency and second-order fluorescence dressing evolution by Rabi frequency control in thermal atomic vapors, in which the controlled results are well explained by the dressing effect and the Rydberg excitation blockade. Based on the certification of the Rydberg excitation blockade fraction through the dependence on principle quantum number n, we obtain dressing evolution curves, consisting of single-dressing and double-dressing in local and nonlocal blockade samples by scanning the probe and dressing fields. In addition, the competition between the Rydberg dressing second-order fluorescence and fourth-order fluorescence is first investigated. A corresponding theory is presented, which is consistent with the experimental results. Such blockade evolution regularity has potential applications in quantum control, and the Rydberg dressing may be useful for investigating multiple-body interactions, as well as for inducing short range interactions in Bose-Einstein condensates.

DOI
10.1039/c4cp02560a

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We report for the first time the theoretical and experimental research on Rydberg electromagnetically induced transparency and second-order fluorescence dressing evolution by Rabi frequency control in thermal atomic vapors, in which the controlled results are well explained by the dressing effect and the Rydberg excitation blockade. Based on the certification of the Rydberg excitation blockade fraction through the dependence on principle quantum number n, we obtain dressing evolution curves, consisting of single-dressing and double-dressing in local and nonlocal blockade samples by scanning the probe and dressing fields. In addition, the competition between the Rydberg dressing second-order fluorescence and fourth-order fluorescence is first investigated. A corresponding theory is presented, which is consistent with the experimental results. Such blockade evolution regularity has potential applications in quantum control, and the Rydberg dressing may be useful for investigating multiple-body interactions, as well as for inducing short range interactions in Bose-Einstein condensates.
We investigate the interaction between dark states and Rydberg excitation blockade by using electromagnetically induced transparency (EIT), fluorescence, and four-wave mixing (FWM) signals both theoretically and experimentally. By scanning the frequency detunings of the probe and dressing fields, respectively, we first observe these signals (three coexisting EIT windows, two fluorescence signals, and two FWM signals) under Rydberg excitation blockade. Next, frequency detuning dependences of these signals are obtained, in which the modulated results are well explained by introducing the dressing effects (leading to the dark states) with the corrected factor of the Rydberg excitation blockade. In addition, the variations by changing the principal quantum number n of Rydberg state shown some interesting phenomena resulting from Rydberg blockade are observed. The unique nature of such blockaded signals can have potential application in the demonstration of quantum computing.
Rb vapor both theoretically and experimentally. By use of a disturbance-free optical detection method, the Rydberg EWM characterized by multiple sets of spin coherence is presented via the interplay and competition between the dressing-state effects and excitation blockade caused by strong Rydberg-Rydberg interaction. Such interplay and competition can be demonstrated by the intensity evolutions of multi-wave mixing (MWM) signals via controlling the atomic density, the frequency detuning and Rabi frequencies of corresponding laser fields. The observed Rydberg EWM tailored by EIT windows can possess of much narrower linewidth <30MHz and provide a new way for the study of Rydberg effect in the atomic ensemble above room temperature.
We present the experimental demonstration of interaction induced enhancement in Rydberg excitation or Rydberg anti-blockade in thermal atomic vapor. We have used optical heterodyne detection technique to measure Rydberg population due to two-photon excitation to the Rydberg state. The anti-blockade peak which doesn't satisfy the two-photon resonant condition is observed along with the usual two-photon resonant peak which can't be explained using the model with non-interacting three-level atomic system. A model involving two interacting atoms is formulated for thermal atomic vapor using the dressed states of three-level atomic system to explain the experimental observations. A non-linear dependence of vapor density is observed for the anti-blockade peak which also increases with increase in principal quantum number of the Rydberg state. A good agreement is found between the experimental observations and the proposed interacting model. Our result implies possible applications towards quantum logic gates using Rydberg anti-blockade in thermal atomic vapor.
Rydberg-dressed four-wave mixing (FWM) is theoretically and experimentally demonstrated with two electromagnetically induced transparency (EIT) windows generated in a Y-type Rb85 atomic configuration. Such dressing effect related to Rydberg states can lead to enhancement and suppression in the FWM process, which can be manipulated by the frequency detuning, Rabi frequency, and polarization of laser fields. Particularly, with the enhancement condition satisfied, coexisting FWM and Rydberg six-wave mixing (SWM) peaks with ultranarrow linewidth (much less than 30 MHz) are simultaneously observed. The controllable enhancement and suppression in a Rydberg-EIT medium can provide a novel nondestructive nonlinear method to investigate the spectrum involving Rydberg excitation in the atomic ensemble above room temperature.
In this paper, we study the realization of a multi-contact switch using the double-dressing regularity of probe, fluorescence, and six-wave mixing signals in a five-level 85Rb atomic system. For the first time, we compare the dressing regularity of Rydberg states by observing electromagnetically induced transparency and signals. With the scanning probe and dressing fields, both large and small line shifts in signals are observed. The small line shifts are induced by double-dressed line shifts. Also, the big line shifts result from the Rydberg dressing. In addition, with an increase in the principal quantum number n of the Rydberg state, all the signals become weaker, while the line shifts of the signals become enhanced. Using the regularity in line shifts of the signals and an acoustic optical modulator to modulate the frequency detuning, we can realize a multi-contact switch action and fast conversion between different contacts.
The strong interaction between Rydberg atoms can be used to control the strength and character of the interatomic interaction in ultracold gases by weakly dressing the atoms with a Rydberg state. Elaborate theoretical proposals for the realization of various complex phases and applications in quantum simulation exist. Also a simple model has been already developed that describes the basic idea of Rydberg dressing in a two-atom basis. However, an experimental realization has been elusive so far. We present a model describing the ground state of a Bose–Einstein condensate dressed with a Rydberg level based on the Rydberg blockade. This approach provides an intuitive understanding of the transition from pure two-body interaction to a regime of collective interactions. Furthermore it enables us to calculate the deformation of a three-dimensional sample under realistic experimental conditions in mean-field approximation. We compare full three-dimensional numerical calculations of the ground state to an analytic expression obtained within Thomas–Fermi approximation. Finally we discuss limitations and problems arising in an experimental realization of Rydberg dressing based on our experimental results and point out possible solutions for future approaches. Our work enables the reader to straight forwardly estimate the experimental feasibility of Rydberg dressing in realistic three-dimensional atomic samples.