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International Conference on Transparent Optical Networks

Forerunners and shapes of the signal in the propagation of radiation in structured nonlinear dispersive dielectrics

Maciej Janowicz, Arkadiusz Orłowski

Published Sep 12, 2005• 0 citations
Publisher

Abstract

Propagation of radiation in nonlinear dispersive media has been analyzed numerically without standard assumptions (like the envelope approximation or the rotating wave approximation) in the near-resonant regime in one spatial dimension. The medium has been modeled as an assemblage of two-, three-, or four-level systems. An attempt to include inhomogeneous broadening has been made with the help of random spatial modulation of the frequencies of transitions in those systems. Particular attention has been directed to the propagation in spatially structured media. Non-trivial dynamics of forerunners have been obtained in the cases of "stopped" light and "superluminal" propagation. The shapes of the signal, and, in particular, the propagation of the wings of the signal have been investigated. The time- and parameter-dependence of the group velocity have been studied in detail, and the vagueness of the concept of the group velocity has been stressed.

DOI
10.1109/icton.2005.1506155

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Propagation of radiation in nonlinear dispersive media has been analyzed numerically without standard assumptions (like the envelope approximation or the rotating wave approximation) in the near-resonant regime in one spatial dimension. The medium has been modeled as an assemblage of two-, three-, or four-level systems. An attempt to include inhomogeneous broadening has been made with the help of random spatial modulation of the frequencies of transitions in those systems. Particular attention has been directed to the propagation in spatially structured media. Non-trivial dynamics of forerunners have been obtained in the cases of "stopped" light and "superluminal" propagation. The shapes of the signal, and, in particular, the propagation of the wings of the signal have been investigated. The time- and parameter-dependence of the group velocity have been studied in detail, and the vagueness of the concept of the group velocity has been stressed.
Electromagnetic pulse propagation in the slow light regime and near a zero group velocity point is relevant to a plethora of potential applications, and has analogies in numerous other wave systems. Unfortunately, the standard frequency-based formulation for pulse propagation is unsuitable for describing the dynamics in such regimes, due to the divergence of the dispersion coefficients. Moreover, in the presence of absorption, it is not clear how to interpret the propagation dynamics due to the drastic change induced by absorption upon the dispersion curves. As a remedy, we present an alternative momentum-based formulation, which is rapidly converging in these regimes, and naturally suitable for lossy and nonlinear media. It is specialized to a waveguide geometry which provides a significant simplification with respect to existing momentum-based schemes. Doing so, we provide a somewhat alternative, yet intuitive picture of the seeming enhanced absorption and nonlinear response in these regimes, and show that light-matter interactions are not enhanced in the slow/stopped light regimes.
A technique of canonical quantization in a general dispersive nonlinear dielectric medium is presented. The medium can be inhomogeneous and anisotropic. The fields are expanded in a slowly varying envelope approximation to allow quantization. An arbitrary number of envelopes is included, assuming lossless propagation in each relevant frequency band. The resulting Lagrangian and Hamiltonian agree with known propagation equations and expressions for the dispersive energy. The central result of the theory is an expansion of the quantum Hamiltonian in terms of annihilation and creation operators corresponding to group-velocity photon-polariton excitations in the dielectric.
General overview In many areas in the physical sciences, the propagation of waves in complex mediaplays a central role. Acoustics, applied mathematics, elastics, environmental sciences, mechanics, marine sciences, medical sciences, microwaves, and seismology are just a few examples, and of course nanophotonics [6, 429, 448, 449]. Here, complex media are understood to exhibit a strongly inhomogeneous spatial structure, which determines to a large extent their linear and nonlinear properties. Examples of complex media are random, heterogeneous, porous, and fractal media. The challenges that researchers in these areas must surmount to describe, understand, and ultimately predict wave propagation are formidable. Right from the start of this field – in the early 1900s – it was clear that new concepts and major approximations had to be introduced. Famous examples of such concepts are the effective medium theory [55, 60, 321] and the radiative transport theory [81, 491]. These concepts are very much alive, even today. The fundamental challenge with these approximate concepts is that often the length scales of the inhomogeneities in the complex medium are comparable with the wavelength, whereas the range of validity of these approximations is restricted to situations where these length scales are much larger than the wavelength. Consequently, many relevant situations arise where either the effective medium theory, or radiative transport theory, or both, fail dramatically. Examples of such situations are given in this introduction and throughout this book. The complexity of the medium that supports wave propagation can be classified in a number of ways. Many different types of spatial inhomogeneities in a host matrix can be envisioned, varying from completely random, via aperiodic and waveguide structures, to quasi-crystalline and even structures with long-range periodic order. The in homogeneities could be of a self-organized form, or the fruit of precise engineering. An additional classification is whether or not the complexity is confined to the surface (in two dimensions (2D)) or is present throughout the volume of the medium (in three dimensions (3D)), as in porous media.
Propagation of an ultrashort, small-area (circularly polarized) pulse through a gas medium of three-level atoms near one-photon resonance is studied. The expression for the propagating pulse shape is obtained within the rotating wave and dipole approximations. Results are compared, both analytically and numerically, with those for two-level model. Sinusoidal and Gaussian shapes of input pulses are compared, and a high sensitivity of modulation of the light pulse for envelope to its input shape is revealed.
It is shown that, when a narrow-band signal with a non-Gaussian envelope propagates in a medium with a strong dispersion, the signal envelope being distorted due to the dispersion of the gain (or) absorption in the medium. Nevertheless, the amplitude-modulated signal having a symmetric (even) intensity envelope remains the same. The propagation velocity of the `middle point' (i.e., the symmetry centre) of the signal coincides with the real group velocity of the wave with a given carrier frequency in the medium and can be subluminal, superluminal or negative. Therefore, the concept of a real group velocity (including the superluminal or negative velocity) is also applicable in media with a strong dispersion of the gain (or absorption).
Spectral reshaping and nonuniform phase delay associated with an electromagnetic pulse propagating in a temporally dispersive medium may lead to interesting observations in which the group velocity becomes superluminal or even negative. In such cases, the finite bandwidth of the superluminal region implies the inevitable existence of a cutoff distance beyond which a superluminal pulse becomes subluminal. In this paper, we derive a closed-form analytic expression to estimate this cutoff distance in abnormal dispersive media with gain. Moreover, the method of steepest descent is used to track the time-frequency dynamics associated with the evolution of the center of mass of a superluminal pulse to the subluminal regime. This evolution takes place at longer propagation depths as a result of the subluminal components affecting the behavior of the pulse. Finally, the analysis presents the fundamental limitations of superluminal propagation in light of factors such as the medium depth, pulse width, and the medium dispersion strength.