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arXiv:1504.06808 · Cambridge University Press eBooks

Light propagation and emission in complex photonic media

Willem L. Vos, Ad Lagendijk, Allard P. Mosk

Published Nov 30, 2014• 9 citations
arXivHTMLPDF

Abstract

General overview In many areas in the physical sciences, the propagation of waves in complex mediaplays a central role. Acoustics, applied mathematics, elastics, environmental sciences, mechanics, marine sciences, medical sciences, microwaves, and seismology are just a few examples, and of course nanophotonics [6, 429, 448, 449]. Here, complex media are understood to exhibit a strongly inhomogeneous spatial structure, which determines to a large extent their linear and nonlinear properties. Examples of complex media are random, heterogeneous, porous, and fractal media. The challenges that researchers in these areas must surmount to describe, understand, and ultimately predict wave propagation are formidable. Right from the start of this field – in the early 1900s – it was clear that new concepts and major approximations had to be introduced. Famous examples of such concepts are the effective medium theory [55, 60, 321] and the radiative transport theory [81, 491]. These concepts are very much alive, even today. The fundamental challenge with these approximate concepts is that often the length scales of the inhomogeneities in the complex medium are comparable with the wavelength, whereas the range of validity of these approximations is restricted to situations where these length scales are much larger than the wavelength. Consequently, many relevant situations arise where either the effective medium theory, or radiative transport theory, or both, fail dramatically. Examples of such situations are given in this introduction and throughout this book. The complexity of the medium that supports wave propagation can be classified in a number of ways. Many different types of spatial inhomogeneities in a host matrix can be envisioned, varying from completely random, via aperiodic and waveguide structures, to quasi-crystalline and even structures with long-range periodic order. The in homogeneities could be of a self-organized form, or the fruit of precise engineering. An additional classification is whether or not the complexity is confined to the surface (in two dimensions (2D)) or is present throughout the volume of the medium (in three dimensions (3D)), as in porous media.

DOI
10.1017/cbo9781139839501.002

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Nonlinear optics is the study of the response of dielectric media to strong optical fields. The fields are sufficiently strong that the response of the medium is, as its name implies, nonlinear. That is, the polarization, which is the dipole moment per unit volume in the medium, is not a linear function of the applied electric field. In the equation for the polarization, there is a linear term, but, in addition, there are terms containing higher powers of the electric field. This leads to significant new types of behavior, one of the most notable being that frequencies different from that of the incident electromagnetic wave, such as harmonics or subharmonics, can be generated. Linear media do not change the frequency of light incident upon them. The first observation of a nonlinear optical effect was, in fact, second-harmonic generation – a laser beam entering a nonlinear medium produced a second beam at twice the frequency of the original. Another type of behavior that becomes possible in nonlinear media is that the index of refraction, rather than being a constant, is a function of the intensity of the light. For a light beam with a nonuniform intensity profile, this can lead to self-focusing of the beam. Most nonlinear optical effects can be described using classical electromagnetic fields, and, in fact, the initial theory of nonlinear optics was formulated assuming the fields were classical. When the fields are quantized, however, a number of new effects emerge. Quantized fields are necessary if we want to describe fields that originate from spontaneous emission. For example, in a process known as spontaneous parametric down-conversion, a beam of light at one frequency, the pump, produces a beam at half the original frequency, the signal. This second beam is a result of spontaneous emission.
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Light Propagation: From Atomic to Nuclear Quantim Optics (J Evers et al.) Relativistic High-Order Harmonic Generation (M C Kohler & K Z Hatsagortsyan) Entangled Light and Matter Waves via Non-linear Interactions (M Macovei et al.) Irreversible Photon Transfer in an Ensemble of Λ-Type Atoms and Photon Diode (G Nikoghosyan & M Fleischhauer) Dissipative Chaos in Quantum Distributions (T V Gevorgyan et al.) Frequency Chirped Laser Pulses in Atomic Physics: Coherent Control of Inner and Translational Quantum States (G P Djotyan et al.) Strongly Correlated Quantum Dynamics of Multimode Light Coupled to a Two-Level Atom in a Cavity (T Kumar et al.) Feedback-Driven Adiabatic Quantum Dynamics (A E Allahverdyan & G Mahler) Landau-Zener Transition in Nonlinear Quantum System (A M Ishkhanyan) Photonic and Electronic Phenomena in Structured Media: Multiple Interactions in Multilayered Structures of Nonlinear Materials (D A Antonosyan & G Yu Kryuchkyan) Integrated Photonic Device Structures with Nano-Scale Features: For Sensitive Applications (R M De La Rue) One-, Two-Electronic and Excitonic States in a Quantum Dots with Nontrivial Geometries: Adiabatic Description (K G Dvoyan et al.) Plannar Plasmonic Structures and Non-linear Metal-Dielectric Subwavelength Waveguides (A R Davoyan et al.) Computer Algebra Study of Structural and Symmetry Properties of Discrete Dynamical Systems (V V Kornyak) Exotic Few-Body Bound States in a Lattice (D Petrosyan & M Valiente) Slow Light and Phase Transition in the Array of Atomic Polaritons (I O Barinov et al.) Nonlinear Optical Effects and Spectroscopy: Formation of Narrow Optical Resonances Using Submicron-Thin Atomic Vapor Layers (D Sarkisyan & A Papoyan) Modelling Magneto-Optical Resonances in Atomic Rubidium at D1 Excitation in Extremely Thin Cells While Maintaining a Self-Consistent Set of Theoretical Parameters (L Kalvans et al.) Laser Isotope Separation in Atomic Vapour. Photo-Chemical Method vs Photo-Ionization One (P A Bokhan et al.) Two-Dimensional Confined Terahertz Wave Propagation in Gap Plasmon Waveguide Formed by Two Cyclindrical Surfaces (Yu H Avetisyan et al.) Broadband Similariton: Features and Applications (A Zeytunyan et al.).
Kinetic equations have played a significant role in optics since the introduction of the radiative transport equation (RTE) by Schuster in the early 20th century. Now they are applied in many scientific fields such as atmospheric physics and biomedical imaging to understand how light interacts with a complex medium. In this thesis we investigate how these equations arise in: 1. models of classical optics in an inhomogeneous disordered scattering medium 2. in fully quantum real space models with a random distribution of atoms In certain spatial and temporal regimes it has been empirically observed that light interacting with a highly disordered scattering medium may be described by a radiative transport equation with a constant scattering coefficient. One way to derive such equations from microscopic principles is to model the medium as a random field which is statistically homogeneous. We show that in a quasi-homogeneous media, where statistical correlations vary rapidly on small length scales and slowly on large length scales, light obeys a radiative transport equation with variable scattering coefficient. In the second part of this thesis we introduce a new model in quantum optics which allows us to treat a quantized electromagnetic field coupled to a medium of two level atoms, both in real space. The rest of the chapter focuses on the interaction of atoms with a field consisting of at most one photon. First we recover a classical result due to Wigner and Weisskopf on the rate of single atom spontaneous emission. Next we show that in a statistically homogeneous distribution of two level atoms the field and atomic amplitude satisfy linear kinetic equations. Finally we show that at sufficiently long times and large distances these amplitudes are asymptotically governed by diffusion equations which may be solved analytically. In the final chapter we use the previous model to analyze a system in which there can be at most two photons. This allows us to study the time evolution of states that initially contain two entangled photons, a phenomenon which has no classical analogue. We show that the various probability amplitudes satisfy linear two particle kinetic equations which again may be asymptotically evaluated at large distances and long times.