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Physical Review A

Electromagnetic quantization in dispersive inhomogeneous nonlinear dielectrics

P. D. Drummond

Published Dec 1, 1990• 162 citations
Publisher

Abstract

A technique of canonical quantization in a general dispersive nonlinear dielectric medium is presented. The medium can be inhomogeneous and anisotropic. The fields are expanded in a slowly varying envelope approximation to allow quantization. An arbitrary number of envelopes is included, assuming lossless propagation in each relevant frequency band. The resulting Lagrangian and Hamiltonian agree with known propagation equations and expressions for the dispersive energy. The central result of the theory is an expansion of the quantum Hamiltonian in terms of annihilation and creation operators corresponding to group-velocity photon-polariton excitations in the dielectric.

DOI
10.1103/physreva.42.6845

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A technique of canonical quantization in a general dispersive nonlinear dielectric medium is presented. The medium can be inhomogeneous and anisotropic. The fields are expanded in a slowly varying envelope approximation to allow quantization. An arbitrary number of envelopes is included, assuming lossless propagation in each relevant frequency band. The resulting Lagrangian and Hamiltonian agree with known propagation equations and expressions for the dispersive energy. The central result of the theory is an expansion of the quantum Hamiltonian in terms of annihilation and creation operators corresponding to group-velocity photon-polariton excitations in the dielectric.
We consider the quantization of slowly varying optical fields in a dispersive nonlinear medium and the application of phase-space methods to the resulting quantum field equations. A pragmatic approach to the quantization of the electromagnetic field is adopted whereby we apply canonical quantization to the Hamiltonian expressed in terms of the slowly varying electric field envelope, all approximations (quasimonochromatic and paraxial) having been made at the classical level. This approach allows us to include material dispersion, diffraction, and nonlinearity. Using phase-space methods we then develop a c-number functional Fokker-Planck equation from which the quantum statistical properties of propagating optical fields can be deduced.
We present a fully canonical quantization scheme for the electromagnetic field in dispersive and lossy linear dielectrics. This scheme is based on a microscopic model, in which the medium is represented by a collection of interacting matter fields. We calculate the exact eigenoperators for the coupled system and express the electromagnetic field operators in terms of them. The dielectric constant of the medium is explicitly derived and is shown to satisfy the Kramers-Kronig relations. We apply these results to treat the propagation of light in dielectrics and obtain simple expressions for the electromagnetic field in the medium in terms of space-dependent creation and annihilation operators. These operators satisfy a set of equal-space commutation relations and obey spatial Langevin equations of evolution. This justifies the use of such operators in phenomenological models in quantum optics. We also obtain two interesting relationships between the group and the phase velocity in dielectrics.
The electromagnetic field is quantized in nonlinear media whose dielectric functions and nonlinear susceptibilities may vary with space. Given the dielectric function and nonlinear susceptibilities, the Hamiltonian of the electromagnetic field is determined completely by this quantization method. From Heisenberg equations we prove that Maxwell's equations are satisfied for the field operators. When the nonlinearity goes to zero, this quantization method returns to the generalized canonical quantization procedure developed in Ref.[1] for linear inhomogeneous media. The general formalism is illustrated by applications to quantization of the second-order and third-order nonlinear quasi-steady-state processes.
The electromagnetic field is quantized in a material whose dielectric function varies with frequency and one spatial dimension. The dielectric function is assumed to have a known form and to be real over the range of frequencies important for a particular application, for example the propagation of an optical signal. General properties of the mode functions are derived and employed in the quantization procedure. Expressions are obtained for the energy and momentum density and current operators, and these are shown to satisfy the appropriate conservation and continuity relations. The general formalism is illustrated by application to the examples of a homogeneous dielectric and two different dielectrics with a sharp interface.
Theories which have been used to describe the quantized electromagnetic field interacting with a nonlinear dielectric medium are either phenomenological or derived by quantizing the macroscopic Maxwell equations. Here we take a different approach and derive a Hamiltonian describing interacting fields from one which contains both field and matter degrees of freedom. The medium is modeled as a collection of two-level atoms, and these interact with the electromagnetic field. The atoms are grouped into effective spins and the the Holstein-Primakoff representation of the spin operators is used to expand them in inverse powers of the total spin. When the lowest order term of the interaction is combined with the free atomic and field Hamiltonians, a Hamiltonian describing a theory of noninteracting polaritons results. When higher order terms are expressed in terms of polariton operators standard nonlinear optical interactions emerge. These are then compared to the results of phenomenological and macroscopic theories. The theory is also used to derive an effective Hamiltonian describing counterpropagating modes in a nonlinear medium.
The problem of quantizing the radiation field inside a nonlinear dielectric is studied. Based on the quantization of radiation in a linear dielectric which includes absorption and dispersion, we extend the theory in order to treat also nonlinear optical processes. We derive propagation equations in space and time for the quantized radiation field including the effects of linear absorption and dispersion as well as nonlinear optical effects. As a special case we derive the propagation equation of a narrow-frequency band light pulse in a Kerr medium.