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Optics Express

Modification of local field effects in two level systems due to quantum corrections

Susanne F. Yelin, Michael Fleischhauer

Published Sep 15, 1997• 5 citations
Publisher

Abstract

Quantum corrections to the Lorentz{Lorenz formula are given for a dense ensemble of atoms interacting with the quantized radiation field. The in uence of these corrections on local-field effects in two-level systems is discussed in the non-cooperative limit. For initially inverted atoms we find superluminescence and radiation trapping. Furthermore it is shown that the quantum corrections set strong limitations to intrinsic optical bistability.

DOI
10.1364/oe.1.000160

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Quantum corrections to the Lorentz{Lorenz formula are given for a dense ensemble of atoms interacting with the quantized radiation field. The in uence of these corrections on local-field effects in two-level systems is discussed in the non-cooperative limit. For initially inverted atoms we find superluminescence and radiation trapping. Furthermore it is shown that the quantum corrections set strong limitations to intrinsic optical bistability.
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Summary form only given. The dynamics of a medium consisting of a dense collection of two-level atoms interacting via the electromagnetic field has been derived from first principles. In dense media and condensed matter, the microscopic local field that couples with a single atom is related to the macroscopic field and volume propagation by the Lorentz-Lorenz relation written for an isotropic homogeneous medium. The dynamical equations for the medium, coupled self-consistently with the Maxwell inhomogeneous wave equation, are given in the rotating wave and dipole coupling approximations. The microscopic development is used within the framework of full quantization, and the explicit effects of spontaneous relaxation for the host as well as the atoms are treated, together with corresponding fluctuations. Particular effects upon intrinsic adiabatic inversion, self-induced transparency, and lasing without inversion, are presented and discussed. In particular, the equilibrium, stationary, and dynamical effects of the host medium, and medium and field fluctuations upon local field effects are discussed.
We investigate the effect of a linear host medium on the dynamics of a dense collection of resonant atoms. We find that near dipole-dipole interaction is enhanced by the presence of the host dielectric, resulting in a lower threshold density and a greater hysteresis area for intrinsic optical bistability. Cooperative decay terms appear that represent the interaction of near dipoles mediated by the absorptive component of the dielectric function of the host medium. These terms are part of the local response and correspond to local cooperative decay effects. \textcopyright{} 1996 The American Physical Society.
We have developed the quantum theory of the interaction of ultracold atomic ensemble with the electromagnetic field of vacuum and laser photons. The main attention is paid to the consistent consideration of dynamical dipole-dipole interactions in the case of the second quantized matter. We show that the retardation effects significantly influence the behavior of atomic ensemble in the radiation field. We have derived the general system of equations, which can be used for the investigation of various linear and nonlinear phenomena in atom optics. As an example, we have considered the diffraction of ultracold atomic beam by the standard laser wave. We show that with the increase of the initial density of the intensities of diffractions modes decrease. We also show that the angles of diffraction for different modes depend on the density.
Cooperative scattering has been the subject of intense research in the last years. In this article, we discuss the concept of cooperative scattering from a broad perspective. We briefly review the various collective effects that occur when light interacts with an ensemble of atoms. We show that some effects that have been recently discussed in the context of ‘single-photon superradiance’, or cooperative scattering in the linear-optics regime, can also be explained by ‘standard optics’, i.e. using macroscopic quantities such as the susceptibility or the diffusion coefficient. We explain why some collective effects depend on the atomic density, and others on the optical depth. In particular, we show that, for a large and dilute atomic sample driven by a far-detuned laser, the decay of the fluorescence, which exhibits superradiant and subradiant dynamics, depends only on the on-resonance optical depth. We also discuss the link between concepts that are independently studied in the quantum-optics community and in the mesoscopic-physics community. We show that the coupled-dipole model predicts a departure from Ohm’s law for the diffuse light, that incoherent multiple scattering can induce a saturation of fluorescence and we also show the similarity between the weak-localization correction to the diffusion coefficient and the inaccuracy of Lorentz local field correction to the susceptibility.