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Physical Review A

Effect of laser linewidths and collisions on resonance fluorescence in a squeezed vacuum

S. Smart, S. Swain

Published May 1, 1992• 31 citations
Publisher

Abstract

We study the system of a single two-level atom interacting with a braodband squeezed vacuum and a classical applied field. The atom is subject to collisions, and the applied field may possess a finite linewidth. The atomic populations, coherences, resonance fluorescence spectrum, and intensity fluctuation spectrum are calculated. Wherever practicable, analytic expressions are obtained that show the dependence of these quantities on the damping parameters. Numerical plots are presented. Two qualitative results that we obtain are the following: (a) we show that the dependence of the populations on the squeezing phase is increased by increasing the damping parameters, contrary to what might at first have been expected, and (b) we show that, in the absence of external damping, the squeezing induces strong asymmetries in the off-resonant resonance fluorescence spectra.

DOI
10.1103/physreva.45.6863

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We study the system of a single two-level atom interacting with a braodband squeezed vacuum and a classical applied field. The atom is subject to collisions, and the applied field may possess a finite linewidth. The atomic populations, coherences, resonance fluorescence spectrum, and intensity fluctuation spectrum are calculated. Wherever practicable, analytic expressions are obtained that show the dependence of these quantities on the damping parameters. Numerical plots are presented. Two qualitative results that we obtain are the following: (a) we show that the dependence of the populations on the squeezing phase is increased by increasing the damping parameters, contrary to what might at first have been expected, and (b) we show that, in the absence of external damping, the squeezing induces strong asymmetries in the off-resonant resonance fluorescence spectra.
The resonance fluorescence of a two-level atom driven by a coherent laser field and damped by a finite bandwidth squeezed vacuum is analysed. We extend the Yeoman and Barnett technique to a non-zero detuning of the driving field from the atomic resonance and discuss the role of squeezing bandwidth and the detuning in the level shifts, widths and intensities of the spectral lines. The approach is valid for arbitrary values of the Rabi frequency and detuning but for the squeezing bandwidths larger than the natural line-width in order to satisfy the Markoff approximation. The narrowing of the spectral lines is interpreted in terms of the quadrature-noise spectrum. We find that, depending on the Rabi frequency, detuning and the squeezing phase, different factors contribute to the line narrowing. For a strong resonant driving field there is no squeezing in the emitted field and the fluorescence spectrum exactly reveals the noise spectrum. In this case the narrowing of the spectral lines arises from the noise reduction in the input squeezed vacuum. For a weak or detuned driving field the fluorescence exhibits a large squeezing and, as a consequence, the spectral lines have narrowed linewidths. Moreover, the fluorescence spectrum can be asymmetric about the central frequency despite the symmetrical distribution of the noise. The asymmetry arises from the absorption of photons by the squeezed vacuum which reduces the spontaneous emission. For an appropriate choice of the detuning some of the spectral lines can vanish despite that there is no population trapping. Again this process can be interpreted as arising from the absorption of photons by the squeezed vacuum. When the absorption is large it may compensate the spontaneous emission resulting in the vanishing of the fluorescence lines.
Fluorescence from a coherently driven two-level atom that is damped by a squeezed vacuum is studied. We show that the mean atomic polarization depends on the relative phases of the squeezed vacuum and the coherent driving field. The fluorescent spectrum is calculated and shows several modifications over the spectrum for normal resonance fluorescence. In particular, the central peak of the Mollow triplet has a linewidth that depends on the phase of the driving field. For strong squeezing this peak can either be much narrower or much broader than the natural linewidth of the atom.
The authors present analytical and numerical results for resonance fluorescence produced by a two-level atom damped by a broad-band squeezed vacuum. Previous theoretical analyses of this model have assumed that the laser frequency and the carrier frequency of the squeezed vacuum are equal. The authors introduce a non-zero detuning between the laser frequency and the carrier frequency while maintaining resonance between the laser frequency and atomic resonance. In the absence of the driving field there is a squeezing threshold: above threshold the decay rate of the atomic polarization can be reduced, and below threshold a squeezing-induced two peak spectrum and frequency shift, which is analogous to the Bloch-Siegert shift, are predicted. In the presence of the driving field, the spectrum is asymmetric for Rabi frequencies smaller or comparable to the detuning of the squeezed vacuum. A symmetric spectrum is obtained for large Rabi frequencies. An interpretation is predicted by means of a dressed-state analysis. The authors find that for not too large Rabi frequencies a remarkably large population inversion can be induced in the dressed states, even at exact resonance of the driving field, provided that the laser frequency and carrier frequency are detuned. Moreover, for detection times larger than the inverse detuning, the spectrum is insensitive to the phase between the driving field and the squeezed vacuum, in marked contrast to the case of no detuning.
We present an analytical technique for investigating the behaviour of a coherently driven atom damped by a squeezed vacuum with finite squeezing bandwidth. A master equation and analytic expressions for the fluorescent spectrum are derived for the simple case of a two-level atom exactly resonant with the frequencies of both the squeezed field and the driving field. Suitable choices of driving strength, phase and squeezing source lead to either sub-natural lincwidths of the Rabi sidebands or a sub-natural linewidth of the central spectral peak or indeed sub-natural linewidths of all three spectral peaks when squeezing bandwidths are taken into account. We also establish the remarkable result that in the strong driving regime, the width of the central peak of the fluorescent spectrum depends solely on the squeezing found at the Rabi sideband frequencies.
The authors calculate the resonance fluorescence spectrum of a two-level atom interacting with a resonant classical applied field and a squeezed vacuum for general values of the squeezing phase. They find that the spectra are asymmetric under the following conditions: (i) the Rabi frequency must not be too large and (ii) the squeezing phase should be of athe order pi /2. Large asymmetries are obtainable, even if the three peaks of the spectrum are clearly resolved. An interpretation is provided by means of a dressed state analysis. Under conditions (i) and (ii), they also find that very large differences in the dressed state populations can occur.
The fluorescence spectrum of a strongly driven two-level atom located inside an optical cavity damped by a narrow-bandwidth squeezed vacuum is studied. We use a dressed atom model approach, first applied to squeezed vacuum problems by Yeoman and Barnett, to derive the master equation of the system and discuss the role of the cavity and the squeezed vacuum in the narrowing of the spectral lines and the population trapping effect. We find that in the presence of a single-mode cavity the effect of squeezing on the fluorescence spectrum is more evident in the linewidths of the Rabi sidebands rather than in the linewidth of the central component. Even in the absence of squeezing, the cavity can reduce the linewidth of the central component almost to zero, whereas the Rabi sidebands can be narrowed only to some finite value. In the presence of a two-mode cavity and a two-mode squeezed vacuum the signature of squeezing is evident in the linewidths of all spectral lines. We also establish that the narrowing of the spectral lines is very sensitive to the detuning of the driving field from the atomic resonance. Moreover, we find that the population trapping effect, predicted for the broadband squeezed vacuum case, may appear in a narrow-bandwidth case only if the input squeezed modes are perfectly matched to the cavity modes and if there is non-zero squeezing at the Rabi sidebands.