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Journal of the Optical Society of America B

Saturated-absorption spectroscopy of weak-field Zeeman splittings in rubidium

Jason L. Bowie, Jack Boyce, R. Y. Chiao

Published Oct 1, 1995• 11 citations
Publisher

Abstract

Using an external cavity-tuned diode laser in Doppler-free saturation spectroscopy, we are able to resolve the weak-field Zeeman splittings in the hyperfine levels of the rubidium D1 line. The number of lines observed in the Zeeman structure of rubidium and their measured energy-level splittings are as expected from theory. The measured amplitudes of the saturated-absorption signals, crossover resonances, and velocity-selective optical pumping signals are used in the analysis of various theories concerning saturated-absorption spectroscopy.

DOI
10.1364/josab.12.001839

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Using an external cavity-tuned diode laser in Doppler-free saturation spectroscopy, we are able to resolve the weak-field Zeeman splittings in the hyperfine levels of the rubidium D1 line. The number of lines observed in the Zeeman structure of rubidium and their measured energy-level splittings are as expected from theory. The measured amplitudes of the saturated-absorption signals, crossover resonances, and velocity-selective optical pumping signals are used in the analysis of various theories concerning saturated-absorption spectroscopy.
High-resolution saturated absorption spectroscopy of the 85RbD1 line has been used for observation of the Zeeman effect by use of a diode laser with a narrow linewidth. Experimental results were compared with both Breit–Rabi theory related to shifted resonant frequencies and Nakayama's single-cycle optical pumping theory related to signal magnitudes of signal [J. Opt. Soc. Am. B2, 1431 (1985)]. A comparison of our results with those of Bowie [J. Opt. Soc. Am. B12, 1839 (1995)], who used perturbation theory to obtain the energy-level shifts, yielded experimental results that differ significantly in some respects.
In this paper, we describe two complementary nonlinear spectroscopy methods which both allow one to achieve Doppler-free spectra of atomic gases. First, saturated absorption spectroscopy is used to investigate the structure of the 5S 1/2 → 5P 3/2 transition in rubidium. Using a slightly modified experimental setup, Doppler-free two-photon absorption spectroscopy is then performed on the 5S 1/2 → 5D 5/2 transition in rubidium, leading to accurate measurements of the hyperfine structure of the 5D 5/2 energy level. In addition, electric dipole selection rules of the two-photon transition are investigated, first by modifying the polarization of the excitation laser, and then by measuring two-photon absorption spectra when a magnetic field is applied close to the rubidium vapour. All experiments are performed with the same grating-feedback laser diode, providing an opportunity to compare different high-resolution spectroscopy methods using a single experimental setup. Such experiments may acquaint students with quantum mechanics selection rules, atomic spectra and Zeeman effect.
Zeeman splitting in the D 2 line of rubidium atoms ( 87 Rb and 85 Rb) has been studied using 'Doppler broadened' as well as 'saturation absorption spectroscopy'. While a linearly polarized beam was used for the former experiment, in the latter case a (π, σ ± ) polarization configuration was employed for both pump and probe beams. Zeeman lines have been observed by applying a field up to 5 mT. The field variation of relative line intensities in Doppler-broadened spectrum was determined following Tremblay et al and Nakayama's four-level model. For the saturation spectrum, a four-level model was used. Because the enhancement of absorption at the field is as low as 1 mT, the F g = 2 to F e = 3 transition for 87 Rb can be used as the reference for laser locking. Level crossing is observed in 85 Rb at fields less than 5 mT.
We perform saturated absorption spectroscopy on the D2_22​ line for room temperature rubidium atoms immersed in magnetic fields within the 0.05-0.13 T range. At those medium-high field values the hyperfine structure in the excited state is broken by the Zeeman effect, while in the ground state hyperfine structure and Zeeman shifts are comparable. The observed spectra are composed by a large number of absorption lines. We identify them as saturated absorptions on two-level systems, on three-level systems in a V configuration and on four-level systems in a N or double-N configuration where two optical transitions not sharing a common level are coupled by spontaneous emission decays. We analyze the intensity of all those transitions within a unified simple theoretical model. We concentrate our attention on the double-N crossovers signals whose intensity is very large because of the symmetry in the branching ratios of the four levels. We point out that these structures, present in all alkali atoms at medium-high magnetic fields, have interesting properties for electromagnetically induced transparency and slow light applications.
We perform saturated absorption spectroscopy on the D2{D}_{2}D2​ line for room temperature rubidium atoms immersed in magnetic fields within the 0.05--0.13 T range. At those medium-high field values the hyperfine structure in the excited state is broken by the Zeeman effect, while in the ground-state hyperfine structure and Zeeman shifts are comparable. The observed spectra are composed by a large number of absorption lines. We identify them as saturated absorptions on two-level systems, on three-level systems in a V\mathsf{V}V configuration, and on four-level systems in an N\mathsf{N}N or double-N\mathsf{N}N configuration where two optical transitions not sharing a common level are coupled by spontaneous emission decays. We analyze the intensity of all those transitions within a unified simple theoretical model. We concentrate our attention on the double-N\mathsf{N}N crossovers signals whose intensity is very large because of the symmetry in the branching ratios of the four levels. We point out that these structures, present in all alkali-metal atoms at medium-high magnetic fields, have interesting properties for electromagnetically induced transparency and slow light applications.