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Physical Review A

Quantum theory for superradiance

Elisabeth Ressayre, Andree A. Tallet

Published Jun 1, 1977• 51 citations
Publisher

Abstract

In order to study the cooperative emission of radiation from an extended system of $N$ two-level atoms, we use the master-equation approach within the Born and Markov approximations. All the properties of the emission of radiation can be deduced from the diagonalization of the coupling matrix $\ensuremath{\Gamma}$, where an element ${\ensuremath{\Gamma}}_{\mathrm{jk}}$ gives the coupling between the atoms labeled $j$ and $k$ via the electromagnetic field. We choose a pencil-shaped volume and study analytically the coupling matrix in the limit for small and large Fresnel numbers. For Fresnel numbers of order unity numerical methods are used. Thus we prove that, for the pencil-shaped geometry, any elaborated model must take into account the interaction of the atoms with the infinity of electromagnetic field modes lying inside two small solid angles about the axis of the largest linear dimension, which we label the $z$ axis. In other words, the intensity of radiation emitted by any atom of the system depends on its position with respect to the others and this "propagation effect" cannot be neglected when interpreting superradiance experiments. For small Fresnel numbers the $z$ dependence predominates, in the opposite case the ($x, y$) dependence does, while for Fresnel numbers of order unity the dependence of all three components must be taken into account. Preliminary calculations are given for which only the $z$ dependence is considered; for Fresnel numbers of magnitude of order unity or smaller, the effect of propagation along the $z$ axis displays large delays for the appearance of superradiance with respect to the time at which the superradiant pulse is maximum when the "propagation effects" are neglected (one-mode model).

DOI
10.1103/physreva.15.2410

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Physical Review A•Sep 1, 1973•20 citations
In order to study the cooperative emission of radiation from an extended system of NNN two-level atoms, we use the master-equation approach within the Born and Markov approximations. All the properties of the emission of radiation can be deduced from the diagonalization of the coupling matrix \ensuremathΓ\ensuremath{\Gamma}\ensuremathΓ, where an element \ensuremathΓjk{\ensuremath{\Gamma}}_{\mathrm{jk}}\ensuremathΓjk​ gives the coupling between the atoms labeled jjj and kkk via the electromagnetic field. We choose a pencil-shaped volume and study analytically the coupling matrix in the limit for small and large Fresnel numbers. For Fresnel numbers of order unity numerical methods are used. Thus we prove that, for the pencil-shaped geometry, any elaborated model must take into account the interaction of the atoms with the infinity of electromagnetic field modes lying inside two small solid angles about the axis of the largest linear dimension, which we label the zzz axis. In other words, the intensity of radiation emitted by any atom of the system depends on its position with respect to the others and this "propagation effect" cannot be neglected when interpreting superradiance experiments. For small Fresnel numbers the zzz dependence predominates, in the opposite case the (x,yx, yx,y) dependence does, while for Fresnel numbers of order unity the dependence of all three components must be taken into account. Preliminary calculations are given for which only the zzz dependence is considered; for Fresnel numbers of magnitude of order unity or smaller, the effect of propagation along the zzz axis displays large delays for the appearance of superradiance with respect to the time at which the superradiant pulse is maximum when the "propagation effects" are neglected (one-mode model).
Basic properties for the emission of radiation are derived from the diagonalization of the matrix (${\ensuremath{\Gamma}}_{\mathrm{ij}}$), where an element ${\ensuremath{\Gamma}}_{\mathrm{ij}}$ gives the coupling between two atoms iii and jjj via the electromagnetic field. This method gives naturally an estimate of the solid angles in which the radiation can take place. By using these estimates, we discuss whether the emission process can be described by a one- (two-) mode model. As expected, this model fails in the two limiting cases of large and small Fresnel numbers. Also for Fresnel numbers of the order of a of few units, it is not obvious whether such a model is valid.
When atoms are coupled to a common electromagnetic environment, the exchange of photons through dipole-dipole interactions leads to the emergence of cooperative effects. As a particular example, superradiance arises from spontaneous emission when this exchange leads to constructive interference of the emitted photons. Here, we introduce an integrated method for studying cooperative radiation in many-body systems. This method, which allows to study extended systems with arbitrarily large number of particles, can be formulated by an effective, nonlinear, two-atom master equation that describes the dynamics using a closed form which treats single- and many-body terms on an equal footing. We apply this method to a homogeneous gas of initially inverted two-level atoms, and demonstrate the appearance of both superradiance and subradiance, identifying a many-body coherence term as the source of these cooperative effects. We describe the many-body induced broadening -- which is analytically found to scale with the optical depth of the system -- and light shifts, and distinguish spontaneous effects from induced ones. In addition, we theoretically predict the time-dependence of subradiance, and the phase change of the radiated field during the cooperative decay.
We discuss the cooperative decay of initial atomic excitation for a pencil-shaped active volume filled with two-level atoms. As long as the length of the sample is much smaller than a certain maximal cooperation length, the atom-field interaction producing the superradiant pulse can be treated in terms of the simplest possible laser model (single mode). The basic laser master equation turns out to be exactly solvable if specified for the superradiance limit which is characterized by two conditions: (i) The photons escape from the low-QQQ cavity so fast that they cannot feed themselves back into atomic excitation to any appreciable amount (this no-feedback condition is equivalent to the above-mentioned requirement for the length of the sample). (ii) The incoherent atomic decay due to natural relaxation is so slow that the individual atomic dipoles do not dephase before engaging themselves cooperatively in the interaction with the electromagnetic field. The present paper presents the derivation and general discussion of the equations describing the statistical properties of atoms and field in a superradiant pulse. Analytical and numerical solutions will be presented in a subsequent paper.
We give a general nonperturbative treatment of cooperative emission in systems of NNN two-level atoms, starting from first principles and including inhomogeneous broadening. In particular, we study superfluorescence, which is defined as the cooperative spontaneous emission, i.e., radiation rate proportional to N2{N}^{2}N2, from an atomic system initially excited with zero macroscopic dipole moment and a uniform population difference between the excited and the fundamental states. The atomic system is described by means of collective dipole operators. A fundamental justification is given for the existence of damped "quasimodes" of the mirrorless active volume. The damping of such modes is simply due to the propagation of the Maxwell field, which escapes from the active volume. A general atom-field master equation is derived for the system atoms plus field inside the active volume, described, respectively, in terms of collective dipole operators and quasimode operators. An important feature of this equation is that inhomogeneous broadening simply appears via a time-dependent atom-field coupling constant. In this paper we give a semiclassical treatment of such a master equation. For a pencil-shaped geometry of the active volume, generalized Maxwell-Bloch equations are derived for the envelopes of the radiation inside the active volume and polarization. Such equations take into account the two directions of propagation of the radiation and the inhomogeneous broadening. Suitably phrasing our initial condition in semiclassical terms, we find that propagation effects can be neglected at all times and the generalized Maxwell-Bloch equations reduce to a simple pendulum equation. On the basis of the discussion of the pendulum equation, we conclude that superfluorescence occurs when (i) the length LLL of the active volume is much larger than a suitable threshold length LT{L}_{T}LT​ (this condition ensures that the dephasing atomic processes occur on a time scale much larger than the times characteristic of the cooperative emission); (ii) the length LLL is smaller or of the same order of a suitable cooperation length Lc{L}_{c}Lc​ (this condition ensures that cooperative spontaneous emission dominates stimulated processes, which give radiation proportional to NNN). For $L\ensuremath{\ll}{L}_{c}$, one has a hyperbolic-secant superfluorescent pulse; for $L\ensuremath{\approx}{L}_{c}$, as one has in the recent experiments of Skribanowitz et al., one finds oscillations in the cooperative decay and in the radiation emission. Such oscillations are due to the contribution of stimulated processes. For $L\ensuremath{\gg}{L}_{c}$, this contribution increases. As a consequence one gets more oscillations in the radiated intensity, which becomes proportional to NNN, so that superfluorescence effects disappear.
We introduce a straightforward quantum-electrodynamic approach to the problem of superradiant spontaneous emission from a system of two-level atoms, and also discuss two classical superradiant systems. The same physical concepts underlie our treatment of both the quantum and classical cases. Explicit expressions are found which describe the time evolution and directional character of the radiated power. Our approach applies to an arbitrary number of atoms which are confined to a region with linear dimensions which may be large compared with the mean wavelength of the emitted radiation. The radiative decay half-life of a large many-atom system is found to be much shorter than the natural lifetime of a single atom, but not as short as the half-life of a small atomic system with the same number of atoms. The far-field radiation pattern appropriate to the case of a circular cylinder of emitters which have been excited by a plane-wave pulse is considered in detail. Polar plots are presented of the radiation patterns produced when the atoms are excited by a plane-wave pulse. Exciting pulses traveling in directions both parallel and at an angle of 10\ifmmode^\circ\else\textdegree\fi{} to the axis of the cylinder are considered. A discussion and generalization of Dicke's "coherence-brightening" criterion is given.
In this paper we attempt to unify the theoretical treatment of a variety of cooperative interaction phenomena occurring in resonantly interacting radiation-matter systems. The system consists of a multimode optical field interacting with NNN resonant atoms in a region of large spatial extent. The field and atoms may or may not be coupled to reservoirs. We derive a set of coupled master equations for the reduced matter and radiation density operators of the composite system in the first Born approximation, using a method due to Bogoliubov. These equations describe within a single framework phenomena involving superradiant emission and coherent propagation. In the first place, our theory generalizes existing formulations of the superradiance problem by treating the radiation field as part of the dynamical system rather than as a reservoir. Hence, our equations describe stimulated interaction effects, which are entirely absent in the usual superradiance master equations. Moreover, our equations contain terms describing the self-consistent interaction of an average field with a set of polarizable atoms, as in the coupled Bloch and Maxwell equations of the theory of coherent pulse propagation, and enable us to describe fluctuations, arising from incoherent emission, about the average behavior described by the Bloch-Maxwell theory. We solve formally the dynamical equation for the radiation density operator and obtain a displaced multivariate Gaussian distribution centered on the solution of the Maxwell wave equation, which has as parameters the first and second moments of the matter density operator. Then we derive and discuss the field and atomic-moment equations, both in the wave-number and position representations. The moment equations enable us to show the relationship between descriptions of superradiant damping based on the Bloch equations and those based on the existence of correlated atomic states, including both as special cases. We introduce reduced matter moments, which allow us to separate incoherent- and coherent-emission effects and enable us to discuss the question of the closure of the moment equations. Then we consider cases where the behavior of the atomic system is dominated by a strong coherent pump wave or where the atoms are in a symmetric correlated state and show how the slowly-varying-envelope approximation simplifies the radiation-moment equations in these two cases. In the former case, we obtain an approximate theory which consists, in lowest order, of the Bloch-Maxwell equations with radiative-damping terms, plus an equation describing the time development of the correlation function for field fluctuations. Returning to our general formalism, we relate the usual parameters of the theory of radiative decay and of resonant interactions to the more general quantities appearing in our spatial analysis. Finally, we discuss the importance of the stimulated-emission terms appearing in our theory and describe several extensions, including the introduction of inhomogeneous broadening.