We discuss the solution of the "superradiance master equation" derived in a preceding paper. During the first few photon transient times the cooperative atomic decay goes through a non-adiabatic oscillatory regime. For later times the decay takes place monotonically in time with the electromagnetic field following it adiabatically. The emitted light pulse has different statistical properties for an incoherently and a coherently prepared "superradiant" atomic initial state. The former case is characterized by large quantum fluctuations and strong atom-atom and atom-field correlations. In the latter case quantum fluctuations are small and the system behaves essentially classically. By also solving for a class of coherently prepared intermediate initial states we show that large quantum fluctuations occur only if the initial total occupancy of the excited state differs from the total number of atoms at most by a number of order unity.
In order to study the cooperative emission of radiation from an extended system of
N two-level atoms, we use the master-equation approach within the Born and Markov approximations. All the properties of the emission of radiation can be deduced from the diagonalization of the coupling matrix $\ensuremath{\Gamma}$, where an element ${\ensuremath{\Gamma}}_{\mathrm{jk}}$ gives the coupling between the atoms labeled
j and
k via the electromagnetic field. We choose a pencil-shaped volume and study analytically the coupling matrix in the limit for small and large Fresnel numbers. For Fresnel numbers of order unity numerical methods are used. Thus we prove that, for the pencil-shaped geometry, any elaborated model must take into account the interaction of the atoms with the infinity of electromagnetic field modes lying inside two small solid angles about the axis of the largest linear dimension, which we label the
z axis. In other words, the intensity of radiation emitted by any atom of the system depends on its position with respect to the others and this "propagation effect" cannot be neglected when interpreting superradiance experiments. For small Fresnel numbers the
z dependence predominates, in the opposite case the (
x,y) dependence does, while for Fresnel numbers of order unity the dependence of all three components must be taken into account. Preliminary calculations are given for which only the
z dependence is considered; for Fresnel numbers of magnitude of order unity or smaller, the effect of propagation along the
z axis displays large delays for the appearance of superradiance with respect to the time at which the superradiant pulse is maximum when the "propagation effects" are neglected (one-mode model).
A system of many #we-level atoms or molecules in a collective Dieke state (1) interacting with a single resonant mode of the quantized radiation field has often been adopted as a quantum-mechanical model for a point laser (2). In a previous paper (3) we reported exact dosed-form solutions and photon statistics of coherent spontaneous emission for the model atom-field state in the l imit of infinitely large co-operation number. The purpose of this paper is to report more general results based on this modeI. We give the exact closed-form solutions and photon statistics of coherent emission in the presence of an applied field for the model atom-field state in the same limit. For an initial atomic Dicke state interacting with an applied field in a coherent (Glauber) state (a), the emitted pulse can be desoribed in terms of Glauber states only when the levels of excitation of the initial Dicke states are (~ superradiant ~ (~). For an initially highly inverted system or low excited system, the photon distributions undergo large fluctuations. The model interaction Hamil tonian is given by
We give a general nonperturbative treatment of cooperative emission in systems of
N two-level atoms, starting from first principles and including inhomogeneous broadening. In particular, we study superfluorescence, which is defined as the cooperative spontaneous emission, i.e., radiation rate proportional to
N2, from an atomic system initially excited with zero macroscopic dipole moment and a uniform population difference between the excited and the fundamental states. The atomic system is described by means of collective dipole operators. A fundamental justification is given for the existence of damped "quasimodes" of the mirrorless active volume. The damping of such modes is simply due to the propagation of the Maxwell field, which escapes from the active volume. A general atom-field master equation is derived for the system atoms plus field inside the active volume, described, respectively, in terms of collective dipole operators and quasimode operators. An important feature of this equation is that inhomogeneous broadening simply appears via a time-dependent atom-field coupling constant. In this paper we give a semiclassical treatment of such a master equation. For a pencil-shaped geometry of the active volume, generalized Maxwell-Bloch equations are derived for the envelopes of the radiation inside the active volume and polarization. Such equations take into account the two directions of propagation of the radiation and the inhomogeneous broadening. Suitably phrasing our initial condition in semiclassical terms, we find that propagation effects can be neglected at all times and the generalized Maxwell-Bloch equations reduce to a simple pendulum equation. On the basis of the discussion of the pendulum equation, we conclude that superfluorescence occurs when (i) the length
L of the active volume is much larger than a suitable threshold length
LT (this condition ensures that the dephasing atomic processes occur on a time scale much larger than the times characteristic of the cooperative emission); (ii) the length
L is smaller or of the same order of a suitable cooperation length
Lc (this condition ensures that cooperative spontaneous emission dominates stimulated processes, which give radiation proportional to
N). For $L\ensuremath{\ll}{L}_{c}$, one has a hyperbolic-secant superfluorescent pulse; for $L\ensuremath{\approx}{L}_{c}$, as one has in the recent experiments of Skribanowitz et al., one finds oscillations in the cooperative decay and in the radiation emission. Such oscillations are due to the contribution of stimulated processes. For $L\ensuremath{\gg}{L}_{c}$, this contribution increases. As a consequence one gets more oscillations in the radiated intensity, which becomes proportional to
N, so that superfluorescence effects disappear.
We discuss from first principles the cooperative decay of a system of two-level atoms, initially prepared in an uncorrelated excited state with population inversion
N, and we give the conditions under which the superfluorescence effect occurs. Describing the atomic system in terms of collective variables, we derive a master equation for the reduced atomic density operator, which gives rise both to a damping and to a time-dependent frequency shift in the dynamics of collective modes. The coupled equations of motion are solved with a self-consistent approach. It is found that the system goes through a nonexponential decay if the maximum length of the active volume is smaller than a "cooperation range" and larger than a "threshold length," in agreement with the one-mode theory. The radiation burst has a time width proportional to ${N}^{\ensuremath{-}1}$, and its intensity is proportional to
N2. Specializing to a pencil-shaped volume, we find that only two atomic modes need to be considered; in this case, the average emitted radiation is all condensed in the two diffraction patterns of the opposite axial modes.