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Physical Review A

Strong-signal laser operation. I. General theory

J. B. Hambenne, M. Sargent

Published Feb 1, 1976• 26 citations
Publisher

Abstract

A Lamb semiclassical theory is developed for multimode, mode-locked laser operation. The equality of frequency spacings between adjacent modes causes population pulsations generated in the nonlinear atomic response to be integer multiples of the adjacent-mode spacing. This allows the atomic response to be written in terms of Fourier series, thereby reducing coupled differential equations of motion to algebraic equations ultimately expressible in terms of a continued fraction. A unidirectional ring configuration is assumed so that the more complicated spatial dependence of standing waves is avoided. Reductions are made to the rateequation limit and to the special two-mode cases of bidirectional ring operation and single-mode, standing-wave, gas-laser operation. Numerical analysis of the equations is motivated. Specific results are given in the following (companion) paper.

DOI
10.1103/physreva.13.784

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Physical Review•May 10, 1969•191 citations
A Lamb semiclassical theory is developed for multimode, mode-locked laser operation. The equality of frequency spacings between adjacent modes causes population pulsations generated in the nonlinear atomic response to be integer multiples of the adjacent-mode spacing. This allows the atomic response to be written in terms of Fourier series, thereby reducing coupled differential equations of motion to algebraic equations ultimately expressible in terms of a continued fraction. A unidirectional ring configuration is assumed so that the more complicated spatial dependence of standing waves is avoided. Reductions are made to the rateequation limit and to the special two-mode cases of bidirectional ring operation and single-mode, standing-wave, gas-laser operation. Numerical analysis of the equations is motivated. Specific results are given in the following (companion) paper.
The semiclassical interaction of a two-level system with a multimode electromagnetic field is discussed in detail. The equations of motion for the macroscopic density matrix are transformed into a single integral equation for the population density, with a complex kernel which can take into account both running- and standing-wave configurations. The iterative solution to this integral equation, which corresponds to an expansion in terms of powers of the electromagnetic field amplitudes, turns out to be divergent when the field amplitudes are greater than some critical value. In the case in which the kernel is a periodic or quasiperiodic function of time, a general solution to the integral equation is found, and this solution turns out to be unique and convergent for every value of the electromagnetic (e.m.) field amplitude. This solution is expressed through a continued-fraction expansion, whose terms are matrices, which can be readily obtained from the kernel. This solution is a generalization of the continued-fraction expansion usually met in the strong-signal semiclassical theory of lasers. Some particular cases are then treated in detail; among them, the solution to the multimode operation in laser devices is given in which the excited level lifetime is long compared with the period of the beating term between two adjacent modes. Although the theory presented is directed towards the steady-state regime in multimode lasers, it may also treat the transient regime of laser operations, or it may be extended to include phenomena where a strong e.m. field, made up of several modes equally spaced in frequency, interacts with a two-level system.
We use the semiclassical strong-signal theory of the laser to predict and explain the onset of side-mode buildup in lasers with one oscillating mode. Two general categories are considered: one for which the side modes and the oscillating mode all have the same wavelength and the other for which they have different wavelengths. The treatments include an arbitrary amount of inhomogeneous broadening. Our approach unifies the treatments of the side-mode instabilities presented earlier and extends them to handle standing waves in addition to the previously treated running waves. We write the field and the population matrix elements as Fourier series in the adjacent-mode beat frequency. This approach has been used extensively in both multimode laser theory and saturation spectroscopy. This technique coincides with linear stability analyses used by others, provided that our beat frequency includes a contribution that is proportional to the complex side-mode gain. We give a solution that allows for detuned operation along with its simpler, centrally tuned special case. The connection with saturation spectroscopy clearly reveals that the side-mode instabilities require side-mode gain. For the single-wavelength case, nonlinear anomalous dispersion is also required. The side-mode gain and dispersion result from both inhomogeneous broadening and population pulsations. The lowest instability thresholds occur when both of these mechanisms play a role. The approach can also be used to treat instabilities in optical bistability by substituting the appropriate equation of state for the strong-mode intensity and by changing the sign of the absorption coefficient. In homogeneously broadened, standing-wave lasers, we show that multiwavelength instabilities depend strongly on the position of the medium in the cavity. We illustrate the theory by giving numerical results for the output pulsation frequency and for the instability threshold by using parameters that are appropriate for the He–Xe laser. These results correlate well with experimental observations.
The multimode strong-signal theory of the preceding paper is applied to a number of two- and three-mode cases. A two-mode stability analysis yields strong-signal counterparts to the third-order coupling parameter. Two-mode homogeneous-broadened operation leads to the discussion of population inversion gratings and associated Bragg scattering. Symmetry properties of the equations for the bidirectional ring are examined. Results for Doppler-broadened two-mode special cases and the three-mode locked unidirectional-ring operation are presented. The strong-signal results are compared to those of the third-order and rate-equation-approximation theories. For the bidirectional ring the historical third-order domain of relative excitation from 1.0 to 1.2 is divided into a valid third-order region and a less accurate region. The condition of bistable operation vs monostable operation is seen to be dependent on the relative excitation and the amount of homogeneous broadening. Two types of bistable operation are seen to exist, one where one mode is completely suppressed and another where both modes may have nonzero intensities.
This paper presents a semiclassical theory of a single-mode gas laser valid for essentially arbitrary values of field intensity. The theory is formulated in terms of an ensemble-averaged form of the density-matrix equations of motion involving a single set of coordinates. The polarization and the population-inversion density are expanded in spatial Fourier components. One obtains a set of coupled difference equations in the Fourier coefficients yn{y}_{n}yn​, which may be solved subject to appropriate boundary conditions on yn{y}_{n}yn​ for large nnn. The solutions may be expressed in terms of continued fractions in the general case, and in closed form in important special cases. Quantities of interest are evaluated by computer. The steady-state laser intensity and frequency are obtained from the coupled electromagnetic field equations as functions of the cavity parameters and the linear gain of the amplifying medium. At moderate values of field intensity, the velocity distribution of the space-averaged population inversion density exhibits a fine structure for low-velocity atoms superimposed on the usual broader depletion. This structure is a manifestation of the coherent ringing of the amplifying medium. The results are compared with those obtained in the rate-equation approximation, and with the recent work of Stenholm and Lamb. Discrepancies with the latter paper are explained.
In this thesis we develop a Lamb-type theory for a two-mode, standing wave, homogeneously broadened laser. The theory differs from Lamb's in that the coupled equations of motion for the atomic system are solved with a matrix perturbation theory that converges best for large, nearly equal mode amplitudes rather than with a perturbation theory that is a power series in the field which converges poorly for large mode amplitudes. The theory has an exact matrix solution when certain symmetries in mode amplitude and mode detuning occur. Asymmetries in these parameters may then be treated by a perturbation theory that converges best when the mode amplitudes are large and nearly equal. The theory makes it possible to solve for the macroscopic polarization at certain cavity positions, and it is found that the polarization consists of an infinite number of harmonic sidebands spaced at multiples of the mode difference frequency from atomic resonance. The projection of the first order polarization onto the two spatial modes gives the first order driving functions for the mode amplitude equations. Two investigations are made: 1) we expand the driving functions in powers of the mode amplitudes to compare with Lamb theory, and 2) we program the mode amplitude equations on a digital computer without expanding in a power series in mode amplitudes to plot out the evolution of the amplitudes for strong fields. The computer shows that even for strong fields, the stronger mode quenches the weaker mode in a time dependent on the laser parameters. Although the theory has been developed for use with longitudinal modes, it may also be used for transverse modes. While the losses of the various longitudinal modes are approximately equal, higher order transverse modes arc known to have higher losses than lower order transverse modes. When the losses of the various modes are taken to be unequal, the matrix theory is expected to give different results than in the case for longitudinal modes.
This paper extends the calculations of the semiclassical Lamb theory of a Doppler-broadened gas laser (optical maser) to arbitrary intensities for the case of single-mode operation. The coupled equations of the classical electromagnetic field and an ensemble of two-level atoms are set up, and a solution is obtained in the form of a continued fraction. This is used to compute intensity-detuning curves and atomic population inversion densities as functions of both the velocity and the position in the laser. When the laser is tuned to resonance, the velocity dependence of the inversion density shows a previously unknown fine structure consisting of a "bump" in the bottom of the hole. The calculations are compared to results obtained from a perturbation expansion in powers of the field and exact results known for atoms with zero velocity. The response of the laser output to a slow modulation and the buildup of oscillations are also discussed.