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Physical Review A

Semiclassical theory of multimode operation in lasers: The high-intensity field solution

Arturo Bambini

Published Oct 1, 1976• 15 citations
Publisher

Abstract

The semiclassical interaction of a two-level system with a multimode electromagnetic field is discussed in detail. The equations of motion for the macroscopic density matrix are transformed into a single integral equation for the population density, with a complex kernel which can take into account both running- and standing-wave configurations. The iterative solution to this integral equation, which corresponds to an expansion in terms of powers of the electromagnetic field amplitudes, turns out to be divergent when the field amplitudes are greater than some critical value. In the case in which the kernel is a periodic or quasiperiodic function of time, a general solution to the integral equation is found, and this solution turns out to be unique and convergent for every value of the electromagnetic (e.m.) field amplitude. This solution is expressed through a continued-fraction expansion, whose terms are matrices, which can be readily obtained from the kernel. This solution is a generalization of the continued-fraction expansion usually met in the strong-signal semiclassical theory of lasers. Some particular cases are then treated in detail; among them, the solution to the multimode operation in laser devices is given in which the excited level lifetime is long compared with the period of the beating term between two adjacent modes. Although the theory presented is directed towards the steady-state regime in multimode lasers, it may also treat the transient regime of laser operations, or it may be extended to include phenomena where a strong e.m. field, made up of several modes equally spaced in frequency, interacts with a two-level system.

DOI
10.1103/physreva.14.1479

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The semiclassical interaction of a two-level system with a multimode electromagnetic field is discussed in detail. The equations of motion for the macroscopic density matrix are transformed into a single integral equation for the population density, with a complex kernel which can take into account both running- and standing-wave configurations. The iterative solution to this integral equation, which corresponds to an expansion in terms of powers of the electromagnetic field amplitudes, turns out to be divergent when the field amplitudes are greater than some critical value. In the case in which the kernel is a periodic or quasiperiodic function of time, a general solution to the integral equation is found, and this solution turns out to be unique and convergent for every value of the electromagnetic (e.m.) field amplitude. This solution is expressed through a continued-fraction expansion, whose terms are matrices, which can be readily obtained from the kernel. This solution is a generalization of the continued-fraction expansion usually met in the strong-signal semiclassical theory of lasers. Some particular cases are then treated in detail; among them, the solution to the multimode operation in laser devices is given in which the excited level lifetime is long compared with the period of the beating term between two adjacent modes. Although the theory presented is directed towards the steady-state regime in multimode lasers, it may also treat the transient regime of laser operations, or it may be extended to include phenomena where a strong e.m. field, made up of several modes equally spaced in frequency, interacts with a two-level system.
This paper presents a semiclassical theory of a single-mode gas laser valid for essentially arbitrary values of field intensity. The theory is formulated in terms of an ensemble-averaged form of the density-matrix equations of motion involving a single set of coordinates. The polarization and the population-inversion density are expanded in spatial Fourier components. One obtains a set of coupled difference equations in the Fourier coefficients yn{y}_{n}yn​, which may be solved subject to appropriate boundary conditions on yn{y}_{n}yn​ for large nnn. The solutions may be expressed in terms of continued fractions in the general case, and in closed form in important special cases. Quantities of interest are evaluated by computer. The steady-state laser intensity and frequency are obtained from the coupled electromagnetic field equations as functions of the cavity parameters and the linear gain of the amplifying medium. At moderate values of field intensity, the velocity distribution of the space-averaged population inversion density exhibits a fine structure for low-velocity atoms superimposed on the usual broader depletion. This structure is a manifestation of the coherent ringing of the amplifying medium. The results are compared with those obtained in the rate-equation approximation, and with the recent work of Stenholm and Lamb. Discrepancies with the latter paper are explained.
A Lamb semiclassical theory is developed for multimode, mode-locked laser operation. The equality of frequency spacings between adjacent modes causes population pulsations generated in the nonlinear atomic response to be integer multiples of the adjacent-mode spacing. This allows the atomic response to be written in terms of Fourier series, thereby reducing coupled differential equations of motion to algebraic equations ultimately expressible in terms of a continued fraction. A unidirectional ring configuration is assumed so that the more complicated spatial dependence of standing waves is avoided. Reductions are made to the rateequation limit and to the special two-mode cases of bidirectional ring operation and single-mode, standing-wave, gas-laser operation. Numerical analysis of the equations is motivated. Specific results are given in the following (companion) paper.
Abstract This present paper is an attempt to describe the operation of a laser by a method patterned closely after the classical theory of dispersion. There, the electromagnetic field is treated as a classical system interacting with a collection of classical harmonic oscillators which are at rest. In the present case the radiation field is still treated classically, but, in accordance with the correspondence principle, the oscillators are now virtual oscillators associated with the up-and-down transitions in effective two-state atoms which are described quantum mechanically. The atoms carrying these virtual oscillators are not at rest but move with different velocities. We show how the Lorentz averaging can be performed for such systems, and derive a closed set of equations linking the average electric field E, with the average polarization density P„ and the average population inversion density Mp associated with atoms moving with the velocity v. Next, we investigate the conditions for the existence of a steady state if pumping is present, and if the electric field is represented by a standing wave, or a travelling wave of a single frequency (single-mode case). It turns out that, notwithstanding the nonlinear nature of the equations, the steady-state conditions give a simple complex dispersion relation; moreover, the real and imaginary part of this dispersion relation are equivalent to the usual heuristic expressions which specify the operating frequency in terms of the index of refraction and cavity length, and which balance the gain against the losses. The single-mode case is analysed in detail without any smallness assumptions for the resultant intensity. The small-intensity case gives the usual results exhibiting the tuning dip. For high intensities the relative depth of the dip tends to zero. At the end of the paper we discuss proposed extensions and additional applications.
We extend the investigation of the long-time behavior of a model consisting of N two-level atoms interacting with a single electromagnetic cavity mode to include interaction with many cavity modes. We show that, as a consequence of the coupling between radiation modes produced by spatial density variations of the population inversion, there is no strictly stationary state possible for multimode behavior. However we obtain a stationary state by neglecting the rapidly oscillating terms. The steady-state population inversion is then a solution of an eigenvalue problem. The eigenvalue determinate is a function of the number of modes and the coupling between modes in addition to the usual dependence on frequencies and relaxation times. We explicitly solve for the unique eigenvalue in special cases. The corresponding eigenvector gives the steady-state mode intensity ratios. The absolute values of the steady-state intensities are determined by the energy conservation equation generalized to include pumping and dissipation. We also calculate the steady-state frequency shifts for each mode. The mode frequency shifts are practically independent of each other and have the same functional form as the single-mode frequency shifts.
This paper extends the calculations of the semiclassical Lamb theory of a Doppler-broadened gas laser (optical maser) to arbitrary intensities for the case of single-mode operation. The coupled equations of the classical electromagnetic field and an ensemble of two-level atoms are set up, and a solution is obtained in the form of a continued fraction. This is used to compute intensity-detuning curves and atomic population inversion densities as functions of both the velocity and the position in the laser. When the laser is tuned to resonance, the velocity dependence of the inversion density shows a previously unknown fine structure consisting of a "bump" in the bottom of the hole. The calculations are compared to results obtained from a perturbation expansion in powers of the field and exact results known for atoms with zero velocity. The response of the laser output to a slow modulation and the buildup of oscillations are also discussed.
We use the semiclassical strong-signal theory of the laser to predict and explain the onset of side-mode buildup in lasers with one oscillating mode. Two general categories are considered: one for which the side modes and the oscillating mode all have the same wavelength and the other for which they have different wavelengths. The treatments include an arbitrary amount of inhomogeneous broadening. Our approach unifies the treatments of the side-mode instabilities presented earlier and extends them to handle standing waves in addition to the previously treated running waves. We write the field and the population matrix elements as Fourier series in the adjacent-mode beat frequency. This approach has been used extensively in both multimode laser theory and saturation spectroscopy. This technique coincides with linear stability analyses used by others, provided that our beat frequency includes a contribution that is proportional to the complex side-mode gain. We give a solution that allows for detuned operation along with its simpler, centrally tuned special case. The connection with saturation spectroscopy clearly reveals that the side-mode instabilities require side-mode gain. For the single-wavelength case, nonlinear anomalous dispersion is also required. The side-mode gain and dispersion result from both inhomogeneous broadening and population pulsations. The lowest instability thresholds occur when both of these mechanisms play a role. The approach can also be used to treat instabilities in optical bistability by substituting the appropriate equation of state for the strong-mode intensity and by changing the sign of the absorption coefficient. In homogeneously broadened, standing-wave lasers, we show that multiwavelength instabilities depend strongly on the position of the medium in the cavity. We illustrate the theory by giving numerical results for the output pulsation frequency and for the instability threshold by using parameters that are appropriate for the He–Xe laser. These results correlate well with experimental observations.