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Physical Review A

Strong-signal laser operation. II. Specific cases

J. B. Hambenne, M. Sargent

Published Feb 1, 1976• 18 citations
Publisher

Abstract

The multimode strong-signal theory of the preceding paper is applied to a number of two- and three-mode cases. A two-mode stability analysis yields strong-signal counterparts to the third-order coupling parameter. Two-mode homogeneous-broadened operation leads to the discussion of population inversion gratings and associated Bragg scattering. Symmetry properties of the equations for the bidirectional ring are examined. Results for Doppler-broadened two-mode special cases and the three-mode locked unidirectional-ring operation are presented. The strong-signal results are compared to those of the third-order and rate-equation-approximation theories. For the bidirectional ring the historical third-order domain of relative excitation from 1.0 to 1.2 is divided into a valid third-order region and a less accurate region. The condition of bistable operation vs monostable operation is seen to be dependent on the relative excitation and the amount of homogeneous broadening. Two types of bistable operation are seen to exist, one where one mode is completely suppressed and another where both modes may have nonzero intensities.

DOI
10.1103/physreva.13.797

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The multimode strong-signal theory of the preceding paper is applied to a number of two- and three-mode cases. A two-mode stability analysis yields strong-signal counterparts to the third-order coupling parameter. Two-mode homogeneous-broadened operation leads to the discussion of population inversion gratings and associated Bragg scattering. Symmetry properties of the equations for the bidirectional ring are examined. Results for Doppler-broadened two-mode special cases and the three-mode locked unidirectional-ring operation are presented. The strong-signal results are compared to those of the third-order and rate-equation-approximation theories. For the bidirectional ring the historical third-order domain of relative excitation from 1.0 to 1.2 is divided into a valid third-order region and a less accurate region. The condition of bistable operation vs monostable operation is seen to be dependent on the relative excitation and the amount of homogeneous broadening. Two types of bistable operation are seen to exist, one where one mode is completely suppressed and another where both modes may have nonzero intensities.
A Lamb semiclassical theory is developed for multimode, mode-locked laser operation. The equality of frequency spacings between adjacent modes causes population pulsations generated in the nonlinear atomic response to be integer multiples of the adjacent-mode spacing. This allows the atomic response to be written in terms of Fourier series, thereby reducing coupled differential equations of motion to algebraic equations ultimately expressible in terms of a continued fraction. A unidirectional ring configuration is assumed so that the more complicated spatial dependence of standing waves is avoided. Reductions are made to the rateequation limit and to the special two-mode cases of bidirectional ring operation and single-mode, standing-wave, gas-laser operation. Numerical analysis of the equations is motivated. Specific results are given in the following (companion) paper.
We provide a comprehensive analysis of the standard model of the bidirectional ring laser in which only one mode can be supported in each direction and in the limit that the polarization can be eliminated adiabatically. The interaction between the two counterpropagating modes can be derived and it is most naturally viewed as a coupling between them via scattering from a spatial grating formed in the population inversion. If the grating is a sufficiently small modulation of the spatial average of the population inversion, it can be approximated by a sinusoidal function. A systematic derivation of the model with only a sinusoidal grating for the homogeneously broadened case is presented that reveals and corrects errors in several previously published analyses. The stability of the steady-state solution is analyzed. The bidirectional steady-state solution is unstable and the unidirectional steady-state solutions may be stable or unstable depending on the parameters. The well-established result of bistability between the two modes when the cavity is tuned to resonance is recovered, a result that persists, in part, even when the losses between the two modes are different.With detuning, the unidirectional steady-state solutions can be destabilized, creating regions in the parameter space where only time-dependent solutions are found. For parameters characteristic of solid-state or molecular gas lasers, the instability can occur for very small detunings and even very close to the lasing threshold. Asymptotic limits of the instability boundaries for these parameters are presented. Additional results are derived formally for inhomogeneous broadening with a Lorentzian line shape and for arbitrary inhomogeneous linewidths. Explicit analytic results are presented in the limits of very small and very large inhomogeneous linewidths compared with the homogeneous linewidth. Time-dependent solutions in the homogeneously broadened case for relaxation rates appropriate to CO2{\mathrm{CO}}_{2}CO2​ lasers show that there are broad regions in the parameter space of gain and detuning for which the behavior is dynamically chaotic in the form of nearly ``square-wave'' alternation between the counterpropagating modes of the laser with irregular switching times. In other regions of that parameter space we find more irregular pulsations and pulse alternations. Regions of periodic pulsations also have been found.
The instabilities in homogeneously broadened lasers, which we described in the previous chapter, have a paradigmatic importance because they arise in models which allow one to perform the linear-stability analysis in a simple analytic form. The treatment of the corresponding instabilities in the case of in homogeneously broadened lasers is substantially more complex in general. However, it is very interesting because, as we shall see, the instabilities arise in parametric domains that are much more accessible from the experimental viewpoint. A related issue is that of the possibility of multimodal emission in a laser. It is common knowledge that in order to attain multimode emission it is necessary to have a sort of in homogeneity in the gain medium, because in a completely homogeneous configuration all modes interact with all atoms, and the arising competition among modes implies that only one of them survives. There are basically two main kinds of in homogeneity, the first is of spatial nature and the other is of spectral nature. The first kind is realized in Fabry–Perot lasers, because different cavity modes interact with atoms at different spatial positions in the cavity thanks to the standing-wave configuration of the field and to the consequent phenomenon of spatial hole- burning (see Section 14.2 and Fig. 14.1). This circumstance is capable of weakening the mode–mode competition and allowing multimode operation. In unidirectional ring lasers, on the other hand, there is an “inhomogeneous” configuration in the case of inhomogeneous broadening, because different groups of atoms have different transition frequencies and therefore interact with different modes thanks to the spectral hole-burning (see Section 15.2 and Fig. 15.3). Again, this weakens the mode–mode competition and allows multimode operation. However, these are qualitative considerations, and the only reliable and quantitative method to determine the possibility of multimodal operation is the linear-stability analysis of the single-mode stationary solutions.
We use the semiclassical strong-signal theory of the laser to predict and explain the onset of side-mode buildup in lasers with one oscillating mode. Two general categories are considered: one for which the side modes and the oscillating mode all have the same wavelength and the other for which they have different wavelengths. The treatments include an arbitrary amount of inhomogeneous broadening. Our approach unifies the treatments of the side-mode instabilities presented earlier and extends them to handle standing waves in addition to the previously treated running waves. We write the field and the population matrix elements as Fourier series in the adjacent-mode beat frequency. This approach has been used extensively in both multimode laser theory and saturation spectroscopy. This technique coincides with linear stability analyses used by others, provided that our beat frequency includes a contribution that is proportional to the complex side-mode gain. We give a solution that allows for detuned operation along with its simpler, centrally tuned special case. The connection with saturation spectroscopy clearly reveals that the side-mode instabilities require side-mode gain. For the single-wavelength case, nonlinear anomalous dispersion is also required. The side-mode gain and dispersion result from both inhomogeneous broadening and population pulsations. The lowest instability thresholds occur when both of these mechanisms play a role. The approach can also be used to treat instabilities in optical bistability by substituting the appropriate equation of state for the strong-mode intensity and by changing the sign of the absorption coefficient. In homogeneously broadened, standing-wave lasers, we show that multiwavelength instabilities depend strongly on the position of the medium in the cavity. We illustrate the theory by giving numerical results for the output pulsation frequency and for the instability threshold by using parameters that are appropriate for the He–Xe laser. These results correlate well with experimental observations.