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Journal of Physics B Atomic Molecular and Optical Physics

Electromagnetically induced transparency in nanocells

A N Litvinov, Georgy A. Kazakov, Boris G. Matisov

Published Jul 22, 2009• 13 citations
Publisher

Abstract

The formation of the electromagnetically induced transparency (EIT) resonance in nanocells is considered. It is shown that the Dicke narrowing of the optical transition takes place in nanocells with the wall coating providing the specular reflection of atoms. The width of the EIT resonance can reach some hundreds of hertz in such cells. It is shown that the effect of the coherent Dicke narrowing of the EIT resonance can appear in both nanometre and centimetre cells.

DOI
10.1088/0953-4075/42/16/165402

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The phenomenon of electromagnetically induced transparency (EIT) is investigated in a Λ-system of the 87Rb D 1 line in an external transverse magnetic field. Two spectroscopic cells having strongly different values of the relaxation rates γrel are used: an Rb cell with antirelaxation coating (L ~ 1 cm) and an Rb nanometric- thin cell (nanocell) with a thickness of the atomic vapor column L = 795 nm. For the EIT in the nanocell, we have the usual EIT resonances characterized by a reduction in the absorption (dark resonance (DR)), whereas for the EIT in the Rb cell with an antirelaxation coating, the resonances demonstrate an increase in the absorption (bright resonances (BR)). We suppose that such an unusual behavior of the EIT resonances (i.e., the reversal of the sign from DR to BR) is caused by the influence of an alignment process. The influence of alignment strongly depends on the configuration of the coupling and probe frequencies as well as on the configuration of the magnetic field.

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Resonance of Electromagnetically Induced Transparency in the Selective Reflection Signal of Atomic Cs Vapor

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Abstract The process of electromagnetically induced transparency (EIT) was investigated using two different probe radiations in Cs atomic vapor: in the first case probe radiation– transmission through a nanocell (NC) with the formation of EITT; in the second–selective reflection (SR) of laser radiation from the boundary of the atom-dielectric vapor (dielectric is nanocell window) with the formation of EITSR. To form EIT resonances, we used two continuous narrow-band lasers with λ = 852 nm and a nanocell with an atomic vapor column thickness in the range of 150–1500 nm. A comparison of the formation of EIT resonance in the first and second cases was carried out. Probe radiation containing EITT and EITSR-resonances propagates in opposite directions. It is noted that in a few cases, the formation of EIT resonance is more effective using SR radiation. The splitting of the EITSR-resonance in the longitudinal magnetic field into seven equidistant components was recorded, which allows remote monitoring of the magnetic field.

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Electromagnetically Induced Transparency in Gas Cells with Antirelaxation Coating

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Abstract The features of electromagnetically induced transparency (EIT) in gas cells with antirelaxation coating of the walls are considered. It is shown that the simultaneous effect of the motion of atoms, the finite size of a cell, and the nondegeneracy of the ground state of atoms leads to a number of qualitative phenomena. In particular, even for the simplest three-level lambda scheme with a nondegenerate ground state, a significant difference in the spectra of EIT is revealed and investigated in detail depending on the relation between the frequencies of the probe and control fields, i.e., depending on whether the probe radiation is scattered in the Stokes or anti-Stokes channel. A significant spatial inhomogeneity of the excited low-frequency coherence is observed, which persists for large cells even far from their boundaries. In this case, the EIT resonances formed by atoms in different regions of a cell turn out to be differently shifted in frequency, which causes an additional inhomogeneous broadening of the observed profile. The observed effects are studied as a function of the nature of the accommodation of atoms on the surface of the antirelaxation coating.

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Influence of collisions on the effect of electromagnetic-induced transparency in cells of finite sizes with anti-relaxation coating of walls

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Based on the semiclassical theory of the interaction of two-frequency laser radiation with a resonant atomic medium, an analytical expression is obtained that describes the form of resonances of electromagnetically induced transparency detected in a cell with a finite direction in the longitudinal laser beam direction with an anti-relaxation coating of walls, taking into account the motion of atoms and collisions with walls. The following types of reflection from walls are considered: diffuse, specular, and specular-incoherent. It is found that in a number of cases the diffuse type of reflection exhibits the properties of a mirror-incoherent one. It is also shown that the nondegeneracy of the excited state in a number of cases significantly changes the shape of the transparency resonance. Keywords: Electromagnetically induced transparency, Gas cell, anti-relaxation coating, diffuse reflection, specular reflection, specular-incoherent reflection.

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The effect of electromagnetically induced transparency (EIT) in a Λ-system formed by rubidium atoms contained in thin (10–60 μm) and extremely thin (0.3–5 μm) cells was studied experimentally. It was found that parameters of the EIT resonance degrade slowly in the case where the frequency of the coupling laser is in resonance with the D 2 transition of rubidium, which enabled the registration of the EIT resonance in a record thin cell with a thickness of L = 390 nm. The specific features of EIT in extremely thin cells reveal themselves when the coupling laser has a frequency detuning Δ from the atomic transition. In this case, the width of the EIT resonance rapidly increases upon an increase in Δ at fixed L (an opposite effect takes place in centimeter-scale cells). It is shown that the width of the EIT resonance is inversely proportional to L in the case of fixed large detuning Δ. The nearly tenfold broadening of the EIT resonance for large values of detuning Δ is caused by the influence of atomic collisions with cell windows on dephasing rate of coherence. The expressions that allow the estimation of the EIT-resonance width for various values of detuning Δ and small values of thickness L are found.

Optics and Spectroscopy•Sep 1, 2011•10 citations
The formation of the electromagnetically induced transparency (EIT) resonance in nanocells is considered. It is shown that the Dicke narrowing of the optical transition takes place in nanocells with the wall coating providing the specular reflection of atoms. The width of the EIT resonance can reach some hundreds of hertz in such cells. It is shown that the effect of the coherent Dicke narrowing of the EIT resonance can appear in both nanometre and centimetre cells.
The phenomenon of electromagnetically induced transparency (EIT) is investigated in a Λ-system of the 87Rb D 1 line in an external transverse magnetic field. Two spectroscopic cells having strongly different values of the relaxation rates γrel are used: an Rb cell with antirelaxation coating (L ~ 1 cm) and an Rb nanometric- thin cell (nanocell) with a thickness of the atomic vapor column L = 795 nm. For the EIT in the nanocell, we have the usual EIT resonances characterized by a reduction in the absorption (dark resonance (DR)), whereas for the EIT in the Rb cell with an antirelaxation coating, the resonances demonstrate an increase in the absorption (bright resonances (BR)). We suppose that such an unusual behavior of the EIT resonances (i.e., the reversal of the sign from DR to BR) is caused by the influence of an alignment process. The influence of alignment strongly depends on the configuration of the coupling and probe frequencies as well as on the configuration of the magnetic field.
Abstract The process of electromagnetically induced transparency (EIT) was investigated using two different probe radiations in Cs atomic vapor: in the first case probe radiation– transmission through a nanocell (NC) with the formation of EITT; in the second–selective reflection (SR) of laser radiation from the boundary of the atom-dielectric vapor (dielectric is nanocell window) with the formation of EITSR. To form EIT resonances, we used two continuous narrow-band lasers with λ = 852 nm and a nanocell with an atomic vapor column thickness in the range of 150–1500 nm. A comparison of the formation of EIT resonance in the first and second cases was carried out. Probe radiation containing EITT and EITSR-resonances propagates in opposite directions. It is noted that in a few cases, the formation of EIT resonance is more effective using SR radiation. The splitting of the EITSR-resonance in the longitudinal magnetic field into seven equidistant components was recorded, which allows remote monitoring of the magnetic field.
Abstract The features of electromagnetically induced transparency (EIT) in gas cells with antirelaxation coating of the walls are considered. It is shown that the simultaneous effect of the motion of atoms, the finite size of a cell, and the nondegeneracy of the ground state of atoms leads to a number of qualitative phenomena. In particular, even for the simplest three-level lambda scheme with a nondegenerate ground state, a significant difference in the spectra of EIT is revealed and investigated in detail depending on the relation between the frequencies of the probe and control fields, i.e., depending on whether the probe radiation is scattered in the Stokes or anti-Stokes channel. A significant spatial inhomogeneity of the excited low-frequency coherence is observed, which persists for large cells even far from their boundaries. In this case, the EIT resonances formed by atoms in different regions of a cell turn out to be differently shifted in frequency, which causes an additional inhomogeneous broadening of the observed profile. The observed effects are studied as a function of the nature of the accommodation of atoms on the surface of the antirelaxation coating.
Based on the semiclassical theory of the interaction of two-frequency laser radiation with a resonant atomic medium, an analytical expression is obtained that describes the form of resonances of electromagnetically induced transparency detected in a cell with a finite direction in the longitudinal laser beam direction with an anti-relaxation coating of walls, taking into account the motion of atoms and collisions with walls. The following types of reflection from walls are considered: diffuse, specular, and specular-incoherent. It is found that in a number of cases the diffuse type of reflection exhibits the properties of a mirror-incoherent one. It is also shown that the nondegeneracy of the excited state in a number of cases significantly changes the shape of the transparency resonance. Keywords: Electromagnetically induced transparency, Gas cell, anti-relaxation coating, diffuse reflection, specular reflection, specular-incoherent reflection.
The effect of electromagnetically induced transparency (EIT) in a Λ-system formed by rubidium atoms contained in thin (10–60 μm) and extremely thin (0.3–5 μm) cells was studied experimentally. It was found that parameters of the EIT resonance degrade slowly in the case where the frequency of the coupling laser is in resonance with the D 2 transition of rubidium, which enabled the registration of the EIT resonance in a record thin cell with a thickness of L = 390 nm. The specific features of EIT in extremely thin cells reveal themselves when the coupling laser has a frequency detuning Δ from the atomic transition. In this case, the width of the EIT resonance rapidly increases upon an increase in Δ at fixed L (an opposite effect takes place in centimeter-scale cells). It is shown that the width of the EIT resonance is inversely proportional to L in the case of fixed large detuning Δ. The nearly tenfold broadening of the EIT resonance for large values of detuning Δ is caused by the influence of atomic collisions with cell windows on dephasing rate of coherence. The expressions that allow the estimation of the EIT-resonance width for various values of detuning Δ and small values of thickness L are found.