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Le Journal de Physique Colloques

SWITCHING DYNAMICS OF BISTABLE CdS ABSORPTIVE PLATELETS

J.‐Y. Bigot, A. Daunois, Noureddine Cherkaoui Eddeqaqi, Jean Oberlé, M. Wegener, Claus F. Klingshirn

Published Jun 1, 1988• 1 citation
Publisher

Abstract

The switching dynamics of thermally induced optical bistability due to increasing absorption is investigated in thin CdS platelets, at room temperature. Fast and slow components can be observed during the switching process, they depend on the holding point intensity and on the switching pulse energy. It is shown that the transverse relaxation of the temperature in the sample influences this dynamics. The spectral shift of the band to band absorption edge, at the origin of the bistable behavior, is observed in a three beam experiment.

DOI
10.1051/jphyscol:1988236

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The switching dynamics of thermally induced optical bistability due to increasing absorption is investigated in thin CdS platelets, at room temperature. Fast and slow components can be observed during the switching process, they depend on the holding point intensity and on the switching pulse energy. It is shown that the transverse relaxation of the temperature in the sample influences this dynamics. The spectral shift of the band to band absorption edge, at the origin of the bistable behavior, is observed in a three beam experiment.
The switching dynamics of photothermal-induced absorption optical bistability is studied in CdS. The bistable element being held near its switching threshold is switched by a pulse of an excimer laser, which can be regarded as δ shaped in time with respect to the thermal relaxation time of the sample. The dynamics of the switching process is influenced by the transverse relaxation of the temperature in the sample. Under appropriate conditions either a slowing down or a fast switching is observed.
Abstract The transmission spectra of CdS platelets are studied at room temperature with a time‐resolved pump‐probe technique. These measurements are also performed during the switching between the two transmission levels of the bistable crystal induced by the pump pulse. In this case, the third beam from a cw argon laser holds the sample around the switching threshold. These spectral and temporally resolved experiments allow the analysis of the switching dynamics of such absorptive bistable devices.
Fast switching times in thermooptic bistable elements held by a cw laser beam and driven by an external pulse have been observed [1,2,3]. An overheating of the nonlinear material may occur during the switching. In this case, a complicated switching behavior is observed [4]. This dynamics can be understood if the temporal variation of the medium temperature is calculated [5]. Moreover, in the experiments with CdS platelets, the transport of heat is very important and the complete spatio-temporal dynamics must be taken into account.
We have observed high-speed optical switching based on the optical bistability of CdSe at low temperatures due both to induced absorption and to dispersion changes. Using a streak camera to record the response of a thin CdSe platelet to high-intensity dye-laser pulses at near-band-gap energies, we have studied these phenomena on a picosecond time scale and measured switching times of several hundred picoseconds. We attribute our observations to nonlinearities caused by exciton interactions in the semiconductor material. Finally, we discuss the part played in these phenomena by thermal and other dynamic effects.