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Physical Review A

Lifetime distribution of spontaneous emission from an assembly of atoms in a dielectric slab

Fu-He Wang, Xue Hua Wang, Ben–Yuan Gu, Yun-Song Zhou

Published Mar 28, 2003• 10 citations
Publisher

Abstract

Spontaneous decay behavior from an assembly of atoms (or molecules) in a dielectric slab sandwiched by two dielectric semi-infinite spaces with arbitrary refractive indices is investigated. We introduce a lifetime distribution function to describe decay kinetics. The zero-point fluctuations of the electromagnetic field are calculated as a function of the position of atom in the slab. They display a symmetric profile with respect to the central plane of the slab in symmetric structure sample and the contributions of the guided modes and the radiation modes components both exhibit cosinelike variation with a base but with a phase difference of \ensuremath{\pi}. With the increase of the thickness of the slab, the oscillations become dense. In contrast, for the asymmetric structure case, the related curves are asymmetric with respect to the middle plane of slab and exhibit considerably distorted cosinelike oscillations. The dependence of the spontaneous emission rate of atoms on the thickness of the slab and the refractive indices of substrate also is surveyed. Our calculations show that quite wide or narrow lifetime distribution can occur for different thicknesses of the slab. The coexistence of both accelerated and inhibited decay processes appears. The calculated results are in good agreement with experimental results.

DOI
10.1103/physreva.67.035802

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Spontaneous decay behavior from an assembly of atoms (or molecules) in a dielectric slab sandwiched by two dielectric semi-infinite spaces with arbitrary refractive indices is investigated. We introduce a lifetime distribution function to describe decay kinetics. The zero-point fluctuations of the electromagnetic field are calculated as a function of the position of atom in the slab. They display a symmetric profile with respect to the central plane of the slab in symmetric structure sample and the contributions of the guided modes and the radiation modes components both exhibit cosinelike variation with a base but with a phase difference of \ensuremath{\pi}. With the increase of the thickness of the slab, the oscillations become dense. In contrast, for the asymmetric structure case, the related curves are asymmetric with respect to the middle plane of slab and exhibit considerably distorted cosinelike oscillations. The dependence of the spontaneous emission rate of atoms on the thickness of the slab and the refractive indices of substrate also is surveyed. Our calculations show that quite wide or narrow lifetime distribution can occur for different thicknesses of the slab. The coexistence of both accelerated and inhibited decay processes appears. The calculated results are in good agreement with experimental results.
We study the spontaneous emission rate of excited atoms in a dielectric microcavity sandwiched by two dielectric semi-infinite spaces and introduce a lifetime distribution function to reveal decay kinetics in this paper.The spontaneous emission rate of atoms is calculated as a function of the position of atom in the microcavity in both symmetric and asymmetric structure cases.Our calculations show that the spontaneous emission rate of atoms depends on the thickness of the microcavity and the refractive indices of substrate.Both accelerated and inhibited decay processes appear.The lifetime distribution with a single-exponential decay can be observed in the much thicker microcavity.The calculated results are in good agreement with experimental results.
Abstract The electromagnetic field is quantized on the basis of the complete set of spatial modes of a plane dielectric slab of arbitrary thickness and refractive index but infinite transverse dimensions, located in otherwise empty three-dimensional space. The vacuum field fluctuations and spontaneous emission rates are evaluated as functions of position both inside and outside the slab. The source-field operator is derived for emission by atoms inside the slab, in the direction perpendicular to its surfaces. Particular attention is given to the possibility of suppressing spontaneous emission by placing atoms in, or close to, a dielectric slab.
Spontaneous decay behaviors from an assembly of atoms (or molecules) in 3D photonic crystals (PC's) with pseudogaps are investigated. Theoretically, a lifetime distribution function for these atoms or molecules is defined to reveal decay kinetics. Our calculations show that quite wide or narrow lifetime distributions can occur for different spread configurations of the atoms (or molecules). The pure PC effect may lead to coexistence of both accelerated and inhibited decay processes. These results provide theoretical clarification for substantial discrepancies in the recent reported experiments.
The spontaneous emission of photons by an atom placed near the dielectric slab is analyzed using global free electromagnetic modes, satisfying necessary continuity conditions at the slab boundaries. These modes include the modes extended over the whole space (traveling) and the modes trapped to a waveguide formed by the slab (trapped). To describe angular properties of spontaneous emission a parametrization of the traveling modes by the outgoing waves has been proposed. Angular characteristics of the traveling photon emission, distributions of the trapped photon emission, as well as global decay rates have been calculated using the quantum approach and standard perturbation theory. Enhancement and suppression of radiative decay rates in various configurations have been shown. A certain calculational error in an earlier paper by Khosravi and Loudon [Proc. R. Soc. London Ser. A 436, 373 (1992)] affecting thin slabs and results near waveguide-mode thresholds has been improved.