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Physical Review A

Spontaneous emission from a dielectric slab

Hendrik Paul Urbach, Geert L. J. A. Rikken

Published May 1, 1998• 100 citations
Publisher

Abstract

The electromagnetic field in a dielectric slab bounded by two dielectric half spaces with arbitrary refractive indices is quantized by computing the complete set of orthonormal electromagnetic modes. The zero-point fluctuations of the electromagnetic field are determined as a function of position. The dependence of the rate of spontaneous emission of thin dielectric films on the thicknesses of the films and the refractive index of the substrate is studied and compared with experimental results.

DOI
10.1103/physreva.57.3913

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The electromagnetic field in a dielectric slab bounded by two dielectric half spaces with arbitrary refractive indices is quantized by computing the complete set of orthonormal electromagnetic modes. The zero-point fluctuations of the electromagnetic field are determined as a function of position. The dependence of the rate of spontaneous emission of thin dielectric films on the thicknesses of the films and the refractive index of the substrate is studied and compared with experimental results.
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Abstract The electromagnetic field is quantized on the basis of the classical spatial modes of a system geometry in which half of space is filled by a dielectric of constant refractive index and the other half of space is empty. The vacuum field fluctuations and spontaneous emission rates are evaluated as functions of position and polarization both inside and outside the dielectric. Particular attention is given to the variations of these quantities in the vicinity of the interface. The source-field operator is derived for emission by atoms inside and outside the dielectric, in the direction perpendicular to the interface.
Spontaneous decay behavior from an assembly of atoms (or molecules) in a dielectric slab sandwiched by two dielectric semi-infinite spaces with arbitrary refractive indices is investigated. We introduce a lifetime distribution function to describe decay kinetics. The zero-point fluctuations of the electromagnetic field are calculated as a function of the position of atom in the slab. They display a symmetric profile with respect to the central plane of the slab in symmetric structure sample and the contributions of the guided modes and the radiation modes components both exhibit cosinelike variation with a base but with a phase difference of \ensuremath{\pi}. With the increase of the thickness of the slab, the oscillations become dense. In contrast, for the asymmetric structure case, the related curves are asymmetric with respect to the middle plane of slab and exhibit considerably distorted cosinelike oscillations. The dependence of the spontaneous emission rate of atoms on the thickness of the slab and the refractive indices of substrate also is surveyed. Our calculations show that quite wide or narrow lifetime distribution can occur for different thicknesses of the slab. The coexistence of both accelerated and inhibited decay processes appears. The calculated results are in good agreement with experimental results.
The rate of spontaneous emission of an atom in the presence of an interface between two dielectrics was calculated using the quantum theory of electromagnetic radiation. Spatial distribution of the field for quasi-continuous spectrum inside an infinite cavity with ideally conducting walls was determined for multiple values of real refractive indices. Spontaneous emission in the continuous spectrum of the field was calculated using the known spatial Green’s function for a one-dimensional dielectric interface. The rate of spontaneous emission of an atom may either be higher or much lower than that in the free space, depending on the refractive indices and the distance between the atom and the interface between dielectrics.
The spontaneous emission of photons by an atom placed near the dielectric slab is analyzed using global free electromagnetic modes, satisfying necessary continuity conditions at the slab boundaries. These modes include the modes extended over the whole space (traveling) and the modes trapped to a waveguide formed by the slab (trapped). To describe angular properties of spontaneous emission a parametrization of the traveling modes by the outgoing waves has been proposed. Angular characteristics of the traveling photon emission, distributions of the trapped photon emission, as well as global decay rates have been calculated using the quantum approach and standard perturbation theory. Enhancement and suppression of radiative decay rates in various configurations have been shown. A certain calculational error in an earlier paper by Khosravi and Loudon [Proc. R. Soc. London Ser. A 436, 373 (1992)] affecting thin slabs and results near waveguide-mode thresholds has been improved.
The spontaneous-emission rates of emitters embedded in a thin layer 0 of a loss-free dielectric depend on their optical environment, i.e., on the optical properties of the two media 1 and 2 adjoining layer 0. For electric- and magnetic-dipole transitions the spontaneous-emission rates, normalized with respect to those in an infinite medium 0, are expressed in terms of the Fresnel reflection coefficients for plane and evanescent waves incident from medium 0 on the interfaces to the planar-stratified or homogeneous media 1 and 2, respectively. From this result which is valid for arbitrary layer thicknesses d0{d}_{0}d0​ we derive an approximation for extremely thin layers of optical thickness ${n}_{0}{d}_{0}\ensuremath{\ll}\frac{\ensuremath{\lambda}}{8}$ (where $\ensuremath{\lambda}$ is the emission wavelength) between two homogeneous loss-free dielectric media 1 and 2. For the normalized spontaneous-emission rates as functions of the refractive indices nj{n}_{j}nj​ of media j=0,1,and2j=0, 1, \mathrm{and} 2j=0,1,and2 analytical expressions are obtained. We have used these expressions previously without proof [Phys. Rev. B 21, 4814 (1980)] to analyze experimentally observed changes in the fluorescence lifetime of Eu3+{\mathrm{Eu}}^{3+}Eu3+ ions in varying optical environments, which yielded the quantum efficiency of the emitting state.