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Physical Review A

Superfluorescence in photonic crystals with pencil-like excitation

Kazuaki Sakoda, Joseph W. Haus

Published Nov 21, 2003• 5 citations
Publisher

Abstract

Fractional decay of population inversion and spectral shift of superfluorescence in photonic crystals due to anomalous Rabi splitting and localization of macroscopic polarization field are demonstrated by means of the coupled-mode analysis for the pencil-like excitation of embedded atoms. Noninteger exponents of atomic density dependence are predicted for the temporal profile of emitted light pulses.

DOI
10.1103/physreva.68.053809

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For a pencil-shaped extended medium with Fresnel number equal to 1, we have quantum mechanically derived a description of the initiation of superfluorescence in terms of Maxwell-Bloch equations with a fluctuating source due to the zero-point fluctuations of the vacuum field. By the introduction of classical behavior, these equations are extended to include nonlinear behavior due to decreasing atomic inversion. The principal assumption in the derivation is that the main features of superfluorescence are governed by the interaction of atoms with field modes inside two small solid angles around the pencil axis. The delay ${\ensuremath{\tau}}_{D}$, defined as the time at which the mean-squared tipping angle of the collective Bloch vector attains the value 1, turns out to be given by ${\ensuremath{\tau}}_{D}=(\frac{{\ensuremath{\tau}}_{R}}{4}){[\mathrm{ln}{(2\ensuremath{\pi}N)}^{\frac{1}{2}}]}^{2}$, where ${\ensuremath{\tau}}_{R}$ is the radiation time for collective decay and $N$ is the number of atoms. The corresponding effective initial tipping angle roughly equals $\frac{2}{{(N)}^{\frac{1}{2}}}$. A Fokker-Planck equation is derived to describe the statistics of the initial development of the tipping angle. The variance $\ensuremath{\Delta}{\ensuremath{\tau}}_{D}$ of the delay of the superfluorescence pulse satisfies approximately $\ensuremath{\Delta}{\ensuremath{\tau}}_{D}=\frac{2.3}{\mathrm{ln}N}$. A brief comparison with previous treatments of superfluorescence is given.

Physical Review A•Mar 1, 1979•253 citations
Fractional decay of population inversion and spectral shift of superfluorescence in photonic crystals due to anomalous Rabi splitting and localization of macroscopic polarization field are demonstrated by means of the coupled-mode analysis for the pencil-like excitation of embedded atoms. Noninteger exponents of atomic density dependence are predicted for the temporal profile of emitted light pulses.
Abstract In this study, the evolution spectrum and emission dynamics of atoms in a defect-free quasiperiodic photonic crystal are studied. Quasiperiodic photonic crystal have advantages over periodic photonic crystal in terms of abundant and strong localized modes due to the quasiperiodic and self-approximation structures of quasiperiodic photonic crystal. The localized modes exhibit extremely large local density of states and high-quality factors in the quasiperiodic photonic crystal. The frequencies of the large local density of states of the localized modes do not depend on the polarization and the position in a particular area in the quasiperiodic photonic crystals. Due to the extremely large local density of states in the defect-free quasiperiodic photonic crystal, strong coupling between the atom and the localized mode in the quasiperiodic photonic crystal can easily occur. Correspondingly, the population of the excited state displays Rabi oscillation, and the emission spectrum of the atom splits into two peaks. Moreover, the Rabi oscillation and the evolution spectrum of the dressed atom depend on the radiation linewidth.
We discuss from first principles the cooperative decay of a system of two-level atoms, initially prepared in an uncorrelated excited state with population inversion NNN, and we give the conditions under which the superfluorescence effect occurs. Describing the atomic system in terms of collective variables, we derive a master equation for the reduced atomic density operator, which gives rise both to a damping and to a time-dependent frequency shift in the dynamics of collective modes. The coupled equations of motion are solved with a self-consistent approach. It is found that the system goes through a nonexponential decay if the maximum length of the active volume is smaller than a "cooperation range" and larger than a "threshold length," in agreement with the one-mode theory. The radiation burst has a time width proportional to ${N}^{\ensuremath{-}1}$, and its intensity is proportional to N2{N}^{2}N2. Specializing to a pencil-shaped volume, we find that only two atomic modes need to be considered; in this case, the average emitted radiation is all condensed in the two diffraction patterns of the opposite axial modes.
A generalized master equation previously proposed to describe oscillatory superfluorescence is numerically solved in the case of strong ringing. When the atomic system is fully excited, anomalous fluctuations and large atom-field correlations make the time evolution of the mean quantities (e.g., number of photons, total population inversion) quantitatively different from those found in the semiclassical treatment. In particular, because of fluctuations, the minima of the radiation output are notably larger than zero. On the contrary, when the atomic system exhibits a sizable initial macroscopic polarization (superradiance), we find a remarkable non-Markoffian effect consisting of a sizable delay in the radiation emission. However, in such conditions all quantum effects disappear, as in the case of pure superradiance.
Employing a recently developed method that is numerically accurate within a model space simulating the real-time dynamics of few-body systems interacting with macroscopic environmental quantum fields, we analyze the full dynamics of an atomic system coupled to a continuum light field with a gapped spectral density. This is a situation encountered, for example, in the radiation field in a photonic crystal, whose analysis has so far been confined to limiting cases due to the lack of suitable numerical techniques. We show that both atomic population and coherence dynamics can drastically deviate from the results predicted when using the rotating-wave approximation, particularly in the strong-coupling regime. Experimental conditions required to observe these corrections are also discussed.
For a pencil-shaped extended medium with Fresnel number equal to 1, we have quantum mechanically derived a description of the initiation of superfluorescence in terms of Maxwell-Bloch equations with a fluctuating source due to the zero-point fluctuations of the vacuum field. By the introduction of classical behavior, these equations are extended to include nonlinear behavior due to decreasing atomic inversion. The principal assumption in the derivation is that the main features of superfluorescence are governed by the interaction of atoms with field modes inside two small solid angles around the pencil axis. The delay ${\ensuremath{\tau}}_{D}$, defined as the time at which the mean-squared tipping angle of the collective Bloch vector attains the value 1, turns out to be given by ${\ensuremath{\tau}}_{D}=(\frac{{\ensuremath{\tau}}_{R}}{4}){[\mathrm{ln}{(2\ensuremath{\pi}N)}^{\frac{1}{2}}]}^{2}$, where ${\ensuremath{\tau}}_{R}$ is the radiation time for collective decay and NNN is the number of atoms. The corresponding effective initial tipping angle roughly equals 2(N)12\frac{2}{{(N)}^{\frac{1}{2}}}(N)21​2​. A Fokker-Planck equation is derived to describe the statistics of the initial development of the tipping angle. The variance $\ensuremath{\Delta}{\ensuremath{\tau}}_{D}$ of the delay of the superfluorescence pulse satisfies approximately $\ensuremath{\Delta}{\ensuremath{\tau}}_{D}=\frac{2.3}{\mathrm{ln}N}$. A brief comparison with previous treatments of superfluorescence is given.