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arXiv:1205.2897 · Physical Review A

Quantum dynamics in photonic crystals

Javier Prior, Inés de Vega, Alex W. Chin, Susana F. Huelga, Martin Bodo Plenio

Published Jan 24, 2013• 42 citations
arXivHTMLPDF

Abstract

Employing a recently developed method that is numerically accurate within a model space simulating the real-time dynamics of few-body systems interacting with macroscopic environmental quantum fields, we analyze the full dynamics of an atomic system coupled to a continuum light field with a gapped spectral density. This is a situation encountered, for example, in the radiation field in a photonic crystal, whose analysis has so far been confined to limiting cases due to the lack of suitable numerical techniques. We show that both atomic population and coherence dynamics can drastically deviate from the results predicted when using the rotating-wave approximation, particularly in the strong-coupling regime. Experimental conditions required to observe these corrections are also discussed.

DOI
10.1103/physreva.87.013428

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Employing a recently developed method that is numerically accurate within a model space simulating the real-time dynamics of few-body systems interacting with macroscopic environmental quantum fields, we analyze the full dynamics of an atomic system coupled to a continuum light field with a gapped spectral density. This is a situation encountered, for example, in the radiation field in a photonic crystal, whose analysis has so far been confined to limiting cases due to the lack of suitable numerical techniques. We show that both atomic population and coherence dynamics can drastically deviate from the results predicted when using the rotating-wave approximation, particularly in the strong-coupling regime. Experimental conditions required to observe these corrections are also discussed.
The rotating-wave approximation (discarded of counter-rotating interactions) to light-matter interactions is widely used in the quantum electrodynamics Hamiltonian; however, its validity has long been a matter of debate. In this article, we explore the importance of counter-rotating interactions in the quantum dynamics of multiple molecules in complex dielectric environments within the framework of macroscopic quantum electrodynamics. Through our analytical analysis, we find that, in the weak coupling regime, the lack of counter-rotating interactions results in the absence of the Casimir-Polder potentials (medium-assisted energy shifts) in the ground-state molecules and a significant deviation of the intermolecule dipole-dipole interactions. Notably, the deviation of intermolecule dipole-dipole interaction can reach up to 50 percent in the near-field zone (short intermolecule distance). We also conduct a case study on the population dynamics of a pair of identical molecules above a plasmonic surface. Through analytical and numerical analysis, it is revealed that the lack of counter-rotating interactions can profoundly affect the dynamics, especially the oscillatory pattern due to intermolecule dipole-dipole interactions, of the molecules in both strong and weak coupling regimes, emphasizing the need for careful consideration when making the rotating-wave approximation in a multiple-molecule system coupled with quantum light.
We present a formula to evaluate the spontaneous emission spectra of an atom in contact with a radiation field with non-Markovian effects. This formula is written in terms of a two-time correlation of system observables and the environmental correlation function, and depends on the distance between the emitting atom and the detector. As an example, we use it to analyze the fluorescence spectra of a two level atom placed as an impurity in a photonic crystal. The radiation field within those materials has a gap or discontinuity where electromagnetic modes cannot propagate in the stationary limit. In that situation, the atomic emission occurs in the form of evanescent waves which are detected with less efficiency the farther we place the detector. The methodology presented in this paper may be useful to study the non-Markovian dynamics of any quantum open system in linear interaction with a harmonic oscillator reservoir and within the weak-coupling approximation.
This article explores the dynamics of many-body atomic systems symmetrically coupled to Lorentzian photonic cavity systems. Our study reveals interesting dynamical characteristics, including non-zero steady states, super-radiant decay, enhanced energy transfer, and the ability to modulate oscillations in the atomic system by tuning environmental degrees of freedom. We also analyze a configuration consisting of a three-atom chain embedded in a photonic cavity. Similarly, we find a strong enhancement of the energy transfer rate between the two ends of the chain and identified specific initial conditions that lead to significantly reduced dissipation between the two atoms at the end of the chain. Another configuration of interest consists of two symmetrical detuned reservoirs with respect to the atomic system. In the single atom case, we show that it is possible to enhance the decay rate of the system by modulating its reservoir detuning. In contrast, in the many-atom case, this results in dynamics akin to the on-resonant cavity. Finally, we examine the validity of the rotating wave approximation through a direct comparison against the numerically exact hierarchical equations of motion. We find good agreement in the weak coupling regime, while in the intermediate coupling regime, we identify qualitative similarities, but the rotating wave approximation becomes less reliable. In the moderate coupling regime, we find deviations of the steady states due to the formation of mixed photon-atom states.
We study the dynamics of a quantum emitter coupled to a two-dimensional photonic crystal featuring a finite bandwidth with sharp edges and a Van-Hove singularity. We study the effect of strong system-bath coupling and non-Markovianity of the photonic environment using a nonperturbative approach based on the recently introduced NCA dynamical map for open quantum systems. We show that several characteristic features of the dynamics near a photonic band-edge such as the freezing of spontaneous emission and the maximum light-matter entanglement, get strongly modified in presence of counter-rotating terms in the system-bath coupling, beyond the rotating-wave approximation. Furthermore, by computing the spectral function of the quantum emitter we comment on the role played by atom-photon bound-state and show that this acquires a much larger lifetime once the rotating-wave approximation is relaxed.
This thesis considers novel phenomena arising in the few and many-body physics of ultracold atomic gases. The specific models considered are motivated by recent experimental developments. A main focus will be the theoretical description of systems used in the simulation of artificial gauge fields via time-modulated tuning of system parameters and via the coupling of internal atomic states by Raman lasers. A second aspect will be the study of systems with synthetic dimensions and the effects of the unconventional infinite range interactions that arise in this description. It explores time-dependent effects in the single and few particle setting and the collective many-body phases arising in these models. Using the framework of Floquet theory it studies the interplay of time-dependence and particle-interactions both in continuum and lattice systems. In particular, it provides a general explanation for how heating effects can arise in interacting periodically time-dependent quantum systems, identifying an underlying mechanism for heating via two-particle collisions and the relevant scaling of the associated rates with system parameters. Furthermore, the general framework is applied to specific experimental set-ups. This yields heating rates and population dynamics in agreement with the experimental data. Finally, it also proposes improvements to the experiment that allow to limit the heating rates which is required to access the strongly interacting regime. In the case of synthetic dimensions the focus lies on the intriguing interplay of artificial gauge fields and strong particle interactions of atoms confined in optical lattices. In these systems a suitable coupling of internal spin-states of the atoms allows to simulate an additional finite dimension. In contrast to the typically encountered situation of short-range interactions the particle interactions are infinite-range in this synthetic dimension. In the strong coupling limit an effective description for this system is derived and its ground state phase diagram is studied using numerical tools.