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Physical Review A

Superfluorescence: Quantum-mechanical derivation of Maxwell-Bloch description with fluctuating field source

D. Polder, Martin F. H. Schuurmans, Quirin H. F. Vrehen

Published Mar 1, 1979• 253 citations
Publisher

Abstract

For a pencil-shaped extended medium with Fresnel number equal to 1, we have quantum mechanically derived a description of the initiation of superfluorescence in terms of Maxwell-Bloch equations with a fluctuating source due to the zero-point fluctuations of the vacuum field. By the introduction of classical behavior, these equations are extended to include nonlinear behavior due to decreasing atomic inversion. The principal assumption in the derivation is that the main features of superfluorescence are governed by the interaction of atoms with field modes inside two small solid angles around the pencil axis. The delay ${\ensuremath{\tau}}_{D}$, defined as the time at which the mean-squared tipping angle of the collective Bloch vector attains the value 1, turns out to be given by ${\ensuremath{\tau}}_{D}=(\frac{{\ensuremath{\tau}}_{R}}{4}){[\mathrm{ln}{(2\ensuremath{\pi}N)}^{\frac{1}{2}}]}^{2}$, where ${\ensuremath{\tau}}_{R}$ is the radiation time for collective decay and $N$ is the number of atoms. The corresponding effective initial tipping angle roughly equals $\frac{2}{{(N)}^{\frac{1}{2}}}$. A Fokker-Planck equation is derived to describe the statistics of the initial development of the tipping angle. The variance $\ensuremath{\Delta}{\ensuremath{\tau}}_{D}$ of the delay of the superfluorescence pulse satisfies approximately $\ensuremath{\Delta}{\ensuremath{\tau}}_{D}=\frac{2.3}{\mathrm{ln}N}$. A brief comparison with previous treatments of superfluorescence is given.

DOI
10.1103/physreva.19.1192

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For a pencil-shaped extended medium with Fresnel number equal to 1, we have quantum mechanically derived a description of the initiation of superfluorescence in terms of Maxwell-Bloch equations with a fluctuating source due to the zero-point fluctuations of the vacuum field. By the introduction of classical behavior, these equations are extended to include nonlinear behavior due to decreasing atomic inversion. The principal assumption in the derivation is that the main features of superfluorescence are governed by the interaction of atoms with field modes inside two small solid angles around the pencil axis. The delay \ensuremathτD{\ensuremath{\tau}}_{D}\ensuremathτD​, defined as the time at which the mean-squared tipping angle of the collective Bloch vector attains the value 1, turns out to be given by \ensuremathτD=(\ensuremathτR4)[ln(2\ensuremathπN)12]2{\ensuremath{\tau}}_{D}=(\frac{{\ensuremath{\tau}}_{R}}{4}){[\mathrm{ln}{(2\ensuremath{\pi}N)}^{\frac{1}{2}}]}^{2}\ensuremathτD​=(4\ensuremathτR​​)[ln(2\ensuremathπN)21​]2, where \ensuremathτR{\ensuremath{\tau}}_{R}\ensuremathτR​ is the radiation time for collective decay and NNN is the number of atoms. The corresponding effective initial tipping angle roughly equals 2(N)12\frac{2}{{(N)}^{\frac{1}{2}}}(N)21​2​. A Fokker-Planck equation is derived to describe the statistics of the initial development of the tipping angle. The variance \ensuremathΔ\ensuremathτD\ensuremath{\Delta}{\ensuremath{\tau}}_{D}\ensuremathΔ\ensuremathτD​ of the delay of the superfluorescence pulse satisfies approximately \ensuremathΔ\ensuremathτD=2.3lnN\ensuremath{\Delta}{\ensuremath{\tau}}_{D}=\frac{2.3}{\mathrm{ln}N}\ensuremathΔ\ensuremathτD​=lnN2.3​. A brief comparison with previous treatments of superfluorescence is given.
Superfluorescence emission profiles are computed using one-way coupled Maxwell-Bloch equations. Transverse effects are included in the full three-spatial-dimension case as well as in the cylindrical-symmetry case. Initiating quantum fluctuations are approximated by a random polarization source with a completely random phase and root-mean-square tipping angle of 2N\frac{2}{\sqrt{N}}N​2​, where NNN is the number of atoms in each volume element. These fluctuations reduce the tail of the output obtained with transverse effects alone. In fact, the fluctuations in output pulse shapes encompass the Cs data of Gibbs, Vrehen, and Hikspoors. The standard deviation for the delay time is found to be (12.5\ifmmode\pm\else\textpm\fi{}4)% for Fresnel number of 0.8 compared with the value (10\ifmmode\pm\else\textpm\fi{}2)% recently measured by Vrehen and der Weduwe, also for Cs. Inhomogeneous-broadening effects are also included in some simulations.
We have formulated the quantum theory of formation of the superfluorescence pulse from a pencil-like amplifier. The coupled system of the linearized Bloch equations for two-level atoms and the three-dimensional wave equation for the electric field has been solved in the geometrical-optics approximation for Fresnel numbers $F \ensuremath{\ge} 1$. Several properties of the superfluorescence pulse are discussed. The spatial coherence function of the pulse has been found as a function of the Fresnel number. This function provides a precise formulation of the concept of "diffraction modes." The delay-time distribution function for various Fresnel numbers has been found. The results are consistent with experimental data and numerical simulations.
To demonstrate its attractiveness, the distribution function for the atomic coherent states called the QQQ representation is used to describe the evolution of superfluorescence. An exact Fokker-Planck equation in the phase space is obtained. It indicates that the dynamics is almost completely classical, even in the very beginning. This implies that all the fluctuations in superfluorescence must originate from the initial distribution corresponding to a complete inversion. Therefore, in a sense, the initial tipping angle possesses physical reality and is not fictitious.
We show that certain properties of superfluorescent pulses radiated spontaneously by a system of many initially excited two-level atoms can be described by means of the classical Maxwell-Bloch equations. The quantum fluctuations which initiate the pulse are random initial polarizations. The radiated fields which arise from different initial polarization distributions vary significantly from pulse to pulse. Such variations represent quantum uncertainties amplified to the macroscopic level. Probability distributions are calculated for various parameters characterizing the shape of the output pulse as well as the mean and the variance of the radiated intensity.
The fluctuating properties of superradiant and superfluorescent systems are investigated by supplementing the equations of motion for the expectation values of quantum observables with random force terms. In the case of a small atomic system the time evolution of the radiated intensity as well as the intensity fluctuations are computed. We also find the time dependence of the average dipole moment in the presence of chirping. For a pencil-shaped geometry, a generalized system of Maxwell–Bloch equations is analysed. The inhomogeneous broadening is then included. We compare the semiclassical equation for the probability distribution of the atomic variables with the quantum equations based both on normal and antinormal ordering. With the exception of the region in the vicinity of the poles of the Bloch sphere, a close correspondence between the semiclassical and quantum theories is established. The oscillatory superfluorescence is treated similarly to quantum analysis by employing a new method of Lugiato for open systems.
Conservation laws for Maxwell-Bloch equations applied to describe superfluorescence are studied. Modifications due to the initial boundary conditions are discussed. For initial polarization in the form of a constant tipping angle, conservation laws are integrated to give exact dependence of all field moments on the propagation length. Three regions of propagation are distinguished: the linear region, where the field energy is negligibly small, the region of rapid exponential growth, and the saturation region. The characteristic distance, where maximum radiation occurs, is explicitly evaluated; it defines the threshold length for superfluoresence. A small chirping, proportional to the square of the tipping angle, is found. The change of the pulse width with propagation length is estimated.