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Physical Review A

High-brightness, high-purity spin-polarized cesium beam

Bernard P. Masterson, Carol E. Tanner, H. Patrick, Carl Wieman

Published Mar 1, 1993• 28 citations
Publisher

Abstract

We describe a cesium atomic beam (${10}^{14}$ atoms ${\mathrm{s}}^{\mathrm{\ensuremath{-}}1}$, 6\ifmmode\times\else\texttimes\fi{}${10}^{16}$ atoms ${\mathrm{sr}}^{\mathrm{\ensuremath{-}}1}$ ${\mathrm{s}}^{\mathrm{\ensuremath{-}}1}$) spin polarized using light from two diode lasers. Of the atoms, 95% may be placed into either the 6${\mathit{S}}_{1/2}$(F,${\mathit{m}}_{\mathit{F}}$)=(3,3) or (4,4) state, with less than 2\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}4}$ of the atoms left in the depleted hyperfine level. The latter fraction rises linearly with atomic beam intensity because of reabsorption of light scattered during the optical pumping process. This and other effects limiting complete hyperfine pumping are discussed.

DOI
10.1103/physreva.47.2139

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Optical pumping of potassium atoms followed by spin-exchange scattering with deuterium atoms in a high magnetic field was found to produce an intense, highly spin-polarized beam of atomic deuterium. In particular, the atomic polarization of deuterium was determined to be (73\ifmmode\pm\else\textpm\fi{}3)% at an intensity of 2.1\ifmmode\times\else\texttimes\fi{}${10}^{17}$ atoms/s.

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We describe a cesium atomic beam (1014{10}^{14}1014 atoms s\ensuremath−1{\mathrm{s}}^{\mathrm{\ensuremath{-}}1}s\ensuremath−1, 6\ifmmode\times\else\texttimes\fi{}1016{10}^{16}1016 atoms sr\ensuremath−1{\mathrm{sr}}^{\mathrm{\ensuremath{-}}1}sr\ensuremath−1 s\ensuremath−1{\mathrm{s}}^{\mathrm{\ensuremath{-}}1}s\ensuremath−1) spin polarized using light from two diode lasers. Of the atoms, 95% may be placed into either the 6S1/2{\mathit{S}}_{1/2}S1/2​(F,mF{\mathit{m}}_{\mathit{F}}mF​)=(3,3) or (4,4) state, with less than 2\ifmmode\times\else\texttimes\fi{}10\ensuremath−4{10}^{\mathrm{\ensuremath{-}}4}10\ensuremath−4 of the atoms left in the depleted hyperfine level. The latter fraction rises linearly with atomic beam intensity because of reabsorption of light scattered during the optical pumping process. This and other effects limiting complete hyperfine pumping are discussed.
A cesium atomic beam having a high degree of polarization is prepared by optical pumping with two circularly polarized diode lasers, and a technique for state-sensitive atomic detection involving laser-induced fluorescence in a magnetic field (LIFB) is introduced. An atomic-beam polarization of 93% is measured using the LIFB technique, and the combined use of optical-state preparation and LIFB detection in an atomic-recoil experiment to study spin-changing electron-atom collisions is demonstrated.
A cesium atomic beam having a high degree of polarization is prepared by optical pumping with two circularly polarized diode lasers, and a technique for state-sensitive atomic detection involving laser-induced fluorescence in a magnetic field (LIFB) is introduced. An atomic-beam polarization of 93% is measured using the LIFB technique, and the combined use of optical-state preparation and LIFB detection in an atomic-recoil experiment to study spin-changing electron-atom collisions is demonstrated.
The ground state magnetic sublevel populations of a cesium atomic beam have been measured by laser-induced fluorescence in a 430 G magnetic field. The detected induced fluorescence spectrum is in excellent agreement with calculation. After preparing the beam in the F=4, M=-4 state by optical pumping with diode lasers, this novel detection technique was used to measure a 93% spin polarization of the atomic beam. We have also demonstrated the use of this technique to detect changes in atomic spin after collisions with electrons.
We describe optically pumping a beam of sodium atoms to >96% mS and >92% mS, mI state selection. (We have accurately measured the population of every mS, mI state in the optically pumped beam.) For the optical pumping both ground hyperfine states are pumped, using single-mode cw dye-laser radiation tuned to the 3S1/2–3P1/2 transition that is phase modulated in a LiTaO3 crystal to produce first-order sidebands at approximately the 1772-MHz hyperfine splitting of the ground state. The z-directed optical pumping is performed in a z-directed magnetic field of ~5 G. The state-selected atoms then move, in ~1 cm, into an ~200 G, z-directed field. The downstream probe laser beam is scanned through the 3S1/2 (mS, mI) → 3P3/2 (mS′, mI) transitions, which are spectroscopically resolved at 200 G, and the fluorescence intensities portray the residual populations in each of the eight 3S1/2 states.
The results of two experiments involving the rapid frequency modulation of diode lasers are presented. In the first experiment, a cesium beam of 10('14) atoms/sec is produced with more than 98% of the atoms in a single spin state. The beam is polarized by optically pumping it with a single diode laser whose frequency is switched between the 6s(F = 4)-6p(,3/2)(F = 5) and 6s(F = 3)-6p(,3/2)(F = 4) transitions at 100 kHz. To do this, the frequency response of a diode laser to changes in injection current was first determined and the injection current modified to force a jump of 9.2 GHz in 1.5 (mu)sec. The same laser is used to probe the atomic population distribution simultaneously. In the second experiment, two diode lasers, tuned to the 6s(F = 4)-6p(,3/2)(F = 5) and 6s(F = 3)-6p(,3/2)(F = 4) transitions, are used to cool and stop a beam of cesium atoms. The laser frequencies are swept to keep them in resonance with the slowing atoms. The same lasers are used to probe the resulting velocity distribution. More than 10('10) atoms/sec are slowed to a velocity of 0 (+OR-) 15 m/sec, corresponding to a temperature of 1(DEGREES)K. Both of these experiments demonstrate extremely simple and inexpensive ways to manipulate atomic cesium.
Optical pumping of potassium atoms followed by spin-exchange scattering with deuterium atoms in a high magnetic field was found to produce an intense, highly spin-polarized beam of atomic deuterium. In particular, the atomic polarization of deuterium was determined to be (73\ifmmode\pm\else\textpm\fi{}3)% at an intensity of 2.1\ifmmode\times\else\texttimes\fi{}1017{10}^{17}1017 atoms/s.