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physica status solidi (b)

Carbon nanotube based magnetic flux detector for molecular spintronics

Jean-Pierre Cleuziou, Wolfgang Wernsdorfer, Vincent Bouchiat, Thierry Ondarçuhu, Marc Monthioux

Published Oct 1, 2007• 4 citations
Publisher

Abstract

Abstract This work describes the study of a superconducting quantum interference device (SQUID) with single‐walled carbon nanotube (CNT) Josephson junctions. Quantum confinement in each junction induces a discrete quantum dot (QD) energy level structure, which can be controlled with two lateral electrostatic gates. The gates are also used to directly tune the quantum phase interference of the Cooper pairs circulating in the SQUID ring. Optimal modulation of the switching current with magnetic flux is achieved when both QD junctions are in the ‘on’ or ‘off’ state. In particular, the SQUID design establishes that these CNT Josephson junctions can be used as gate‐controlled π junctions. Besides, the CNT‐SQUIDs are sensitive local magnetometers, which are very promising for the study of magnetization reversal of an individual magnetic particle or molecule placed on one of the two CNT Josephson junctions. (© 2007 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)

DOI
10.1002/pssb.200776188

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Abstract This work describes the study of a superconducting quantum interference device (SQUID) with single‐walled carbon nanotube (CNT) Josephson junctions. Quantum confinement in each junction induces a discrete quantum dot (QD) energy level structure, which can be controlled with two lateral electrostatic gates. The gates are also used to directly tune the quantum phase interference of the Cooper pairs circulating in the SQUID ring. Optimal modulation of the switching current with magnetic flux is achieved when both QD junctions are in the ‘on’ or ‘off’ state. In particular, the SQUID design establishes that these CNT Josephson junctions can be used as gate‐controlled π junctions. Besides, the CNT‐SQUIDs are sensitive local magnetometers, which are very promising for the study of magnetization reversal of an individual magnetic particle or molecule placed on one of the two CNT Josephson junctions. (© 2007 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
We have fabricated and studied a promising kind of direct current superconducting quantum interference device (dc-SQUID) in which the magnitude and sign of the critical current of the individual Josephson junctions can be controlled by additional voltage probes connected to the junctions. We show that the amplitude of the voltage oscillations of the SQUID as a function of the applied magnetic field can be tuned and that the phase of the oscillations can be switched between 0 and π in the temperature range of 0.1–4.2 K using a suitable control voltage. This is equivalent to the external application of (n+1/2) flux quantum.
The Josephson current of spin-entangled electrons through the two branches of a SQUID-like structure with two quantum dots exhibits a magnetic-flux response different from the conventional Josephson current. Because of their interference, the period of maximum Josephson current changes from h/2e to h/e, which can be used for detecting the Cooper-pair splitting efficiency. The nonlocal spin entanglement provides a quantum mechanical functionale for switching on and off this novel Josephson current, and explicitly a switch is formulated by including a pilot junction. It is shown that the device can be used to measure the magnitude of split-tunneling Josephson current.
The quantum behaviour of mechanical resonators is a new and emerging field driven by recent experiments reaching the quantum ground state. The high frequency, small mass, and large quality-factor of carbon nanotube resonators make them attractive for quantum nanomechanical applications. A common element in experiments achieving the resonator ground state is a second quantum system, such as coherent photons or a superconducting device, coupled to the resonators motion. For nanotubes, however, this is a challenge due to their small size. Here, we couple a carbon nanoelectromechanical (NEMS) device to a superconducting circuit. Suspended carbon nanotubes act as both superconducting junctions and moving elements in a Superconducting Quantum Interference Device (SQUID). We observe a strong modulation of the flux through the SQUID from displacements of the nanotube. Incorporating this SQUID into superconducting resonators and qubits should enable the detection and manipulation of nanotube mechanical quantum states at the single-phonon level.
Gate-tunable transmon qubits are based on quantum conductors used as weak links within hybrid Josephson junctions. These gatemons have been implemented in just a handful of systems, all relying on extended conductors, namely epitaxial semiconductors or exfoliated graphene. Here we present the coherent control of a gatemon based on a single molecule, a one-dimensional carbon nanotube, which is integrated into a circuit quantum electrodynamics architecture. The measured qubit spectrum can be tuned with a gate voltage and reflects the quantum dot behavior of the nanotube. Our ultraclean integration, using a hexagonal boron nitride substrate, results in record coherence times of 200 ns for carbon nanotube-based qubits. Furthermore, we investigate its decoherence mechanisms, thus revealing a strong gate dependence and identifying charge noise as a limiting factor. On top of positioning carbon nanotubes as contenders for future quantum technologies, our work paves the way for studying microscopic fermionic processes in low-dimensional quantum conductors. Gatemons, or gate-tunable transmons, are superconducting qubits based on hybrid Josephson junctions, which typically use extended quantum conductors as weak links. Here the authors report a gatemon made with a carbon-nanotube-based junction, showing improved coherence time compared to graphene-based devices.
We investigated, at temperature 4.2 K, electric transport, flux noise, and resulting spin sensitivity of miniaturized Nb direct current superconducting quantum interference devices (SQUIDs) based on submicron Josephson junctions with HfTi barriers. The SQUIDs are either of the magnetometer-type or gradiometric in layout. In the white noise regime, for the best magnetometer we obtain a flux noise SΦ1/2=250nΦ0/Hz1/2, corresponding to a spin sensitivity Sμ1/2≥29μB/Hz1/2. For the gradiometer we find SΦ1/2=300nΦ0/Hz1/2 and Sμ1/2≥44μB/Hz1/2. The devices can still be optimized with respect to flux noise and coupling between a magnetic particle and the SQUID, leaving room for further improvement towards single spin resolution.
This article presents a study on the characteristics of single Cooper-pair transistors when integrated into a Superconducting Quantum Interface Device (SQUID) circuit. SQUID is a highly sensitive magnetometer that uses phase balance checks through single Cooper-pair transistors when Josephson currents flow. The study explores the tuning of the supercurrent of the single Cooper-pair transistors in a circuit with a loop coupled to gate voltage. Understanding the behavior of single Cooper-pair transistors in this loop structure is crucial for integrating them with other superconducting electronic circuits. The research includes simulations of the single Cooper-pair transistor in one branch of a SQUID loop circuit. The simulation results indicate that single Cooper-pair transistors can be used as superconducting current switches.