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arXiv:1009.6028 · Physical Review Letters

Interference and Switching of Josephson Current Carried by Nonlocal Spin-Entangled Electrons in a SQUID-Like System with Quantum Dots

Zhi Wang, Xiao Hu

Published Jan 19, 2011• 16 citations
arXivHTMLPDF

Abstract

The Josephson current of spin-entangled electrons through the two branches of a SQUID-like structure with two quantum dots exhibits a magnetic-flux response different from the conventional Josephson current. Because of their interference, the period of maximum Josephson current changes from h/2e to h/e, which can be used for detecting the Cooper-pair splitting efficiency. The nonlocal spin entanglement provides a quantum mechanical functionale for switching on and off this novel Josephson current, and explicitly a switch is formulated by including a pilot junction. It is shown that the device can be used to measure the magnitude of split-tunneling Josephson current.

DOI
10.1103/physrevlett.106.037002

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The Josephson current of spin-entangled electrons through the two branches of a SQUID-like structure with two quantum dots exhibits a magnetic-flux response different from the conventional Josephson current. Because of their interference, the period of maximum Josephson current changes from h/2e to h/e, which can be used for detecting the Cooper-pair splitting efficiency. The nonlocal spin entanglement provides a quantum mechanical functionale for switching on and off this novel Josephson current, and explicitly a switch is formulated by including a pilot junction. It is shown that the device can be used to measure the magnitude of split-tunneling Josephson current.
Devices to generate on-demand non-local spin entangled electron pairs have potential application as solid-state analogues of the entangled photon sources used in quantum optics. Recently, Andreev entanglers that use two quantum dots as filters to adiabatically split and separate the quasi-particles of Cooper pairs have shown efficient splitting through measurements of the transport charge but the spin entanglement has not been directly confirmed. Here we report measurements on parallel quantum dot Josephson junction devices allowing a Josephson current to flow due to the adiabatic splitting and recombination of the Cooper pair between the dots. The evidence for this non-local transport is confirmed through study of the non-dissipative supercurrent while tuning independently the dots with local electrical gates. As the Josephson current arises only from processes that maintain the coherence, we can confirm that a current flows from the spatially separated entangled pair.
We investigate the switching current of a Cooper pair transistor with tunable Josephson energy. The junctions are fabricated in a superconducting quantum interference device (SQUID) geometry which allows for an in situ tunable effective Josephson energy by application of a magnetic field. We find a 2e2e2e-periodic switching current versus gate charge. As the magnetic field is increased the switching current stays 2e2e2e-periodic but the magnitude is suppressed. At a magnetic field of half a flux quantum through the SQUID's the switching current is minimum. We can theoretically model the experimental data by assuming a switching current which is proportional to the ideal critical current squarred. We show that such a dependence is expected in the limit where the effect of thermal fluctuations on the system is strong.
Superconducting quantum interference devices (SQUIDs) that incorporate two superconductor/insulator/superconductor (SIS) Josephson junctions in a closed loop form the core of some of the most sensitive detectors of magnetic and electric fields currently available. SQUIDs in these applications are typically operated with a finite voltage which generates microwave radiation through the ac Josephson effect. This radiation may impact the system being measured. We describe here a SQUID in which the Josephson junctions are formed from strips of normal metal (N) in good electrical contact with the superconductor (S). Such SNS SQUIDs can be operated under a finite voltage bias with performance comparable or potentially better than conventional SIS SQUIDs. However, they also permit a mode of operation that is based on the unusual interplay of quasiparticle currents and supercurrents in the normal metal of the Josephson junction. The method allows measurements of the flux dependence of the critical current of the SNS SQUID without applying a finite voltage bias across the SNS junction, enabling sensitive flux detection without generating microwave radiation.
We study a double quantum dot, each dot of which is tunnel coupled to superconducting leads. In the Coulomb blockade regime, a spin-dependent Josephson coupling between two superconductors is induced, as well as an antiferromagnetic Heisenberg exchange coupling between the spins on the double dot that can be tuned by the superconducting phase difference. We show that the correlated spin states---singlet or triplets---on the double dot can be probed via the Josephson current in a dc-superconducting quantum interference device setup.
We propose a many-body mechanism for a strong Josephson diode effect (JDE) in an interacting nanoscale SQUID formed by two parallel quantum dots coupled to superconducting leads. Unlike conventional diode behavior, where nonreciprocity originates from a skewed current-phase relation within a single, continuously evolving ground state, the JDE reported here is \emph{branch selected}: the positive and negative critical currents are optimized on different many-body branches across the 000-πππ phase boundary, yielding a substantial enhancement of the diode efficiency. We further show that a \emph{nonlocal} Cooper-pair tunneling channel, which binds the two electrons on different arms, is essential: it reshapes the 000-πππ boundary and produces a pronounced ``diode band'' in parameter space, in sharp contrast to the fragile hotspot obtained when only local Cooper-pair transfer is available. While the key physics is captured by an effective model in the superconducting atomic limit, our conclusions remain robust for realistic finite-gap devices, as demonstrated within a generalized atomic-limit framework.
New strategies to generate and to detect spin-entangled pairs of electrons in mesoscopic solid-state heterostructures are proposed. A bilayer-graphene device is designed in which Cooper pairs from an s-wave superconductor are injected into an electrostatically-defined topological channel. Due to a particular band structure, two electrons of a Cooper pair propagate in opposite directions and are hence spatially separated if atomic-scale defects are sparse. Neither energy filtering nor Coulomb repulsion are required. The device can be interpreted as a normal/superconducting/normal junction, in which emission of nonlocal singlets is equivalent to local Andreev reflection, in contrast to the widespread identification of Cooper pair splitting with crossed Andreev reflection. To detect entanglement, the Josephson current through two parallel single-level quantum dots is investigated at all occupations. Combining exact diagonalization and perturbation theory, signatures of nonlocal Cooper pair transport are identified in the critical current, a macroscopic quantity. The model reproduces recent experimental observations and predicts a nonlocal triplet ground state on the quantum dots due to a tunable superconductor-mediated exchange coupling, which, too, is visible in the critical current exactly if nonlocal Cooper pairs are transported. Entanglement detection is pursued, too, by converting spin-entangled Cooper pairs into polarization-entangled photons, which are subsequently probed by a Bell-type measurement. A closed emission cycle is constructed, such that no correlations between the photons and the electrons remain, which are detrimental for entanglement transfer. Inevitable side channels and imperfections are identified and accounted for by a particular measurement protocol. Furthermore, it is discussed how spin-charge separation can be used to extract signatures of nonlocal spin singlets from the average current through an electronic beam splitter. This complements a known mechanism based on exchange statistics by which only the more difficult-to-access noise is sensitive for entanglement. The device can be realized by two crossed nanowires or by quantum-Hall edge states in Corbino geometry. The thesis also contains a review on entanglement and on recent theoretical and experimental progress in solid-state systems towards entanglement detection and generation, focusing on Cooper pair splitting.