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New Ways to Create and to Detect Nonlocal Cooper Pairs in Solid-State Nanodevices

Alexander Schroer

Published Feb 22, 2017• 0 citations
Publisher

Abstract

New strategies to generate and to detect spin-entangled pairs of electrons in mesoscopic solid-state heterostructures are proposed. A bilayer-graphene device is designed in which Cooper pairs from an s-wave superconductor are injected into an electrostatically-defined topological channel. Due to a particular band structure, two electrons of a Cooper pair propagate in opposite directions and are hence spatially separated if atomic-scale defects are sparse. Neither energy filtering nor Coulomb repulsion are required. The device can be interpreted as a normal/superconducting/normal junction, in which emission of nonlocal singlets is equivalent to local Andreev reflection, in contrast to the widespread identification of Cooper pair splitting with crossed Andreev reflection. To detect entanglement, the Josephson current through two parallel single-level quantum dots is investigated at all occupations. Combining exact diagonalization and perturbation theory, signatures of nonlocal Cooper pair transport are identified in the critical current, a macroscopic quantity. The model reproduces recent experimental observations and predicts a nonlocal triplet ground state on the quantum dots due to a tunable superconductor-mediated exchange coupling, which, too, is visible in the critical current exactly if nonlocal Cooper pairs are transported. Entanglement detection is pursued, too, by converting spin-entangled Cooper pairs into polarization-entangled photons, which are subsequently probed by a Bell-type measurement. A closed emission cycle is constructed, such that no correlations between the photons and the electrons remain, which are detrimental for entanglement transfer. Inevitable side channels and imperfections are identified and accounted for by a particular measurement protocol. Furthermore, it is discussed how spin-charge separation can be used to extract signatures of nonlocal spin singlets from the average current through an electronic beam splitter. This complements a known mechanism based on exchange statistics by which only the more difficult-to-access noise is sensitive for entanglement. The device can be realized by two crossed nanowires or by quantum-Hall edge states in Corbino geometry. The thesis also contains a review on entanglement and on recent theoretical and experimental progress in solid-state systems towards entanglement detection and generation, focusing on Cooper pair splitting.

DOI
10.24355/dbbs.084-201702221213-0

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New strategies to generate and to detect spin-entangled pairs of electrons in mesoscopic solid-state heterostructures are proposed. A bilayer-graphene device is designed in which Cooper pairs from an s-wave superconductor are injected into an electrostatically-defined topological channel. Due to a particular band structure, two electrons of a Cooper pair propagate in opposite directions and are hence spatially separated if atomic-scale defects are sparse. Neither energy filtering nor Coulomb repulsion are required. The device can be interpreted as a normal/superconducting/normal junction, in which emission of nonlocal singlets is equivalent to local Andreev reflection, in contrast to the widespread identification of Cooper pair splitting with crossed Andreev reflection. To detect entanglement, the Josephson current through two parallel single-level quantum dots is investigated at all occupations. Combining exact diagonalization and perturbation theory, signatures of nonlocal Cooper pair transport are identified in the critical current, a macroscopic quantity. The model reproduces recent experimental observations and predicts a nonlocal triplet ground state on the quantum dots due to a tunable superconductor-mediated exchange coupling, which, too, is visible in the critical current exactly if nonlocal Cooper pairs are transported. Entanglement detection is pursued, too, by converting spin-entangled Cooper pairs into polarization-entangled photons, which are subsequently probed by a Bell-type measurement. A closed emission cycle is constructed, such that no correlations between the photons and the electrons remain, which are detrimental for entanglement transfer. Inevitable side channels and imperfections are identified and accounted for by a particular measurement protocol. Furthermore, it is discussed how spin-charge separation can be used to extract signatures of nonlocal spin singlets from the average current through an electronic beam splitter. This complements a known mechanism based on exchange statistics by which only the more difficult-to-access noise is sensitive for entanglement. The device can be realized by two crossed nanowires or by quantum-Hall edge states in Corbino geometry. The thesis also contains a review on entanglement and on recent theoretical and experimental progress in solid-state systems towards entanglement detection and generation, focusing on Cooper pair splitting.
Abstract Correlations are fundamental in describing many body systems - not only in natural sciences. However, in experiments, correlations are notoriously difficult to assess on the microscopic scale, especially for electron spins. Here, we demonstrate a direct measurement of the spin cross-correlations between the currents of a Cooper pair splitter, an electronic device that emits electrons originating from Cooper pairs in a superconductor. While it is firmly established theoretically that these electron pairs form maximally spin-entangled singlet states with opposite spin projections, no spin correlation experiments have been demonstrated so far. We use ferromagnetic sidegates, compatible with superconducting electronic structures, to individually spin polarize the transmissions of two quantum dots fabricated in the two electronic paths, which act as tunable spin filters. The signals are detected in standard transport and in highly sensitive transconductance experiments. We find that the spin-cross correlation is negative, compatible with spin singlet emission, and deviates from the ideal value mostly due to a finite overlap of the Zeeman split quantum dot states. Our results demonstrate a new route to perform spin auto- and cross correlation experiments in nanometer scaled electronic devices, especially suitable for those relying on magnetic field sensitive superconducting elements, like unconventional, triplet or topologically non-trivial superconductors, or to perform Bell tests with massive particles, like electrons.
Devices to generate on-demand non-local spin entangled electron pairs have potential application as solid-state analogues of the entangled photon sources used in quantum optics. Recently, Andreev entanglers that use two quantum dots as filters to adiabatically split and separate the quasi-particles of Cooper pairs have shown efficient splitting through measurements of the transport charge but the spin entanglement has not been directly confirmed. Here we report measurements on parallel quantum dot Josephson junction devices allowing a Josephson current to flow due to the adiabatic splitting and recombination of the Cooper pair between the dots. The evidence for this non-local transport is confirmed through study of the non-dissipative supercurrent while tuning independently the dots with local electrical gates. As the Josephson current arises only from processes that maintain the coherence, we can confirm that a current flows from the spatially separated entangled pair.
A Cooper-pair or electron-hole splitter is a device capable of spatially separating entangled fermionic quasiparticles into mesoscopic solid-state systems such as quantum dots or quantum wires. We theoretically study such a splitter based on a pair of helical Luttinger liquids, which arise naturally at the edges of a quantum spin Hall insulator. Equipping each helical liquid with a beam splitter, current-current cross correlations can be used to construct a Bell inequality whose violation would indicate nonlocal orbital entanglement of the injected electrons and/or holes. Due to the Luttinger-liquid correlations, however, the entanglement is suppressed depending on ambient temperature and voltage bias.
We study the critical Josephson current flowing through a double quantum dot weakly coupled to two superconducting leads. We use analytical as well as numerical methods to investigate this setup in the limit of small and large bandwidth leads in all possible charging states, where we account for on-site interactions exactly. Our results provide clear signatures of nonlocal spin-entangled pairs, which support interpretations of recent experiments [R. S. Deacon, A. Oiwa, J. Sailer, S. Baba, Y. Kanai, K. Shibata, K. Hirakawa, and S. Tarucha, Nat. Commun. 6, 7446 (2015)]. In addition, we find that the ground state with one electron on each quantum dot can undergo a tunable singlet-triplet phase transition in the regime where the superconducting gap in the leads is not too large, which gives rise to an additional new signature of nonlocal Cooper-pair transport.
The generation of spin-entangled electrons is an important prerequisite for future solid-state quantum technologies. Cooper pairs in a superconductor can be split into separate electrons in a spin-singlet state, however, detecting their entanglement remains an open experimental challenge. Proposals to detect the entanglement by violating a Bell inequality typically require a large number of current cross-correlation measurements, and not all entangled states can be detected in this way. Here, we instead formulate an entanglement witness that can detect the spin-entanglement using only three cross-correlation measurements of the currents in the outputs of a Cooper pair splitter. We identify the optimal measurement settings for witnessing the entanglement, and we illustrate the use of our entanglement witness with a realistic model of a Cooper pair splitter for which we evaluate the cross-correlations of the output currents. Specifically, we find that the entanglement of the spins can be detected even with a moderate level of decoherence. Our work thereby paves the way for an experimental detection of the entanglement produced by Cooper pair splitters.
A Cooper pair splitter consists of two quantum dots side-coupled to a conventional superconductor. Usually, the quantum dots are assumed to have a large charging energy compared to the superconducting gap, in order to suppress processes other than the coherent splitting of Cooper pairs. In this work, in contrast, we investigate the limit in which the charging energy is smaller than the superconducting gap. This allows us, in particular, to study the effect of a Zeeman field comparable to the charging energy. We find analytically that in this parameter regime the superconductor mediates an interdot tunneling term with a spin symmetry determined by the Zeeman field. Together with electrostatically tunable quantum dots, we show that this makes it possible to engineer a spin triplet state shared between the quantum dots. Compared to previous works, we thus extend the capabilities of the Cooper pair splitter to create entangled nonlocal electron pairs.