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Physical review. B, Condensed matter

Anharmonic oscillator model for driven and vacuum-field Rabi oscillations

S. Rudin, T. L. Reinecke

Published Jan 25, 2001• 6 citations
Publisher

Abstract

The dynamics of electronic excitations coupled to photons in semiconductor microcavities is discussed using an anharmonic oscillator model to represent the electronic excitations. It is shown that this description, unlike the harmonic oscillator model, exhibits driven Rabi oscillations in addition to vacuum-field Rabi splitting, and the magnitude of the anharmonicity needed is discussed. In the limit of large anharmonicity, a two-level description of the electronic excitations is recovered. A picture of the anharmonicity arising from exciton-exciton interactions is discussed.

DOI
10.1103/physrevb.63.075308

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The dynamics of electronic excitations coupled to photons in semiconductor microcavities is discussed using an anharmonic oscillator model to represent the electronic excitations. It is shown that this description, unlike the harmonic oscillator model, exhibits driven Rabi oscillations in addition to vacuum-field Rabi splitting, and the magnitude of the anharmonicity needed is discussed. In the limit of large anharmonicity, a two-level description of the electronic excitations is recovered. A picture of the anharmonicity arising from exciton-exciton interactions is discussed.
The vacuum-field Rabi splitting of an optical mode in a cavity interacting with a system of N excitations (atomic or electronic) represented by harmonic oscillators is obtained quantum mechanically both without and with coupling to dissipation. The optical lineshapes and the scaling of the Rabi splitting with the number of oscillators and its dependence on the damping parameters are given. Corresponding results are given for a classical treatment of the oscillators, and it is shown that to the leading order in the dissipation, the quantum mechanical results for absorption are the same as the classical ones.
Recently, several research groups have reported investigations of vacuum-field Rabi splittings (VRS) in the linear response of strongly coupled semiconductor microcavities [1-4]. We have previously reported on the dynamics of time-domain vacuum Rabi oscillations, which are most easily understood in the framework of cavity exciton-polaritons, in which the in-plane momentum k|| is conserved [2], so that at each k|| a single cavity mode interacts with only a single mode of the electromagnetic field (Jaynes-Cummings model). In high Q semiconductor microcavities, the strong coupling between two-dimensional excitons and planar distributed- Bragg-reflector cavity modes results in several-meV splittings observable in the reflectivity or absorption spectrum. In the low excitation regime, the VRS is independent of light intensity incident on the cavity, since the vacuum-Rabi frequency exceeds the externally-driven Rabi frequency (in which case the Jaynes-Cummings model is equivalent to the linear dispersion of the coupled exciton-cavity system). As the incident light intensity is increased, two different effects may be expected to contribute to the nonlinear response. First, as long as the excitonic absorption is equivalent to a two-level system, higher-lying states of the Jaynes-Cummings ladder might be observable. Second, at high intensity phase-space filling and Coulomb screening of the exciton states results in a reduced oscillator strength which leads to a reduced VRS; this effect has no analogue in the case of atom-cavity systems. In this paper, we apply several ultrafast nonlinear techniques to investigate the nonlinear response of semiconductor microcavities.
Recently, cavity quantum electrodynamic (QED) effects in semiconductor microcavities have been of considerable interest since, in the weak-coupling regime they play an important role in selectively increasing spontaneous emission into the lasing mode of vertical-cavity surface-emitting lasers (VCSEL’s) [1,2], enabling low-threshold, high speed, and high efficiency. In a strong-coupling regime, the normal modes of the coupled system are superpositions of the exciton and cavity modes. Hence the impulsively excited system will evolve in time with the energy oscillating between the exciton and cavity modes. This is known as a vacuum-Rabi oscillation (VRO), with a frequency of Ω=d¯⋅E¯/@@h, where d¯ is the transition dipole moment of atoms and E¯ the vacuum-field strength. Of course, VRO are observable only when the cavity lifetime and exciton dephasing time are long enough compared to VRO period. Recently, Weisbuch et al. [3] have reported an observation of the normal-mode vacuum Rabi splitting in 2-D-exciton/planar-DBR microcavities. The observed splittings were as large as 6 meV in reflection and transmission spectra, implying 690-fs vacuum Rabi oscillations.
Recent progress in vertical surface-emitting-laser-diode technology has raised considerable interest in cavity-QED effects in high-quality vertical semiconductor microcavities. When an excitonic transition and a single cavity mode are strongly coupled, the normal modes of the system are coupled modes split by the vacuum-Rabi frequency, corresponding in the time domain to an oscillation of the excitation between modes of exciton and photon character. Recently, the vacuum-Rabi splitting and preliminary observations of time-domain oscillation in semiconductor quantum microcavities have been reported.1,2 In this paper we investigate rigorously the time-domain vacuum-Rabi oscillation by femtosecond upconversion and pump-probe techniques.
The excitonic dynamics in a single quantum dot within a microcavity is investigated theoretically in terms of the perturbation treatment based on a unitary transformation. The excitonic Rabi oscillations with a damping rate are obtained explicitly. It is shown that the damping rate depends on exciton-phonon coupling constant and the vacuum Rabi frequency. Even at absolute zero temperature and in the vacuum cavity, the exciton-phonon interaction and exciton-photon interaction still cause excitonic decoherence. We also predict that under strong control fields the collapse and revival of excitonic Rabi oscillation may be observed for the quantum dots with small exciton-phonon coupling in the $T\ensuremath{\rightarrow}0$ limit.