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Journal of Physics B Atomic and Molecular Physics

Quantum beats in superradiance in sodium vapours

J Marek, M. Ryschka

Published Aug 28, 1980• 4 citations
Publisher

Abstract

Intensity modulations have been observed in the superradiant signals on the 4 2 P 1/2 -4 2 S 1/2 transitions obtained by pulsed dye laser beam excitation of the 4 2 P 1/2 level in Na vapour. The modulations were interpreted as beats among the frequencies of the electric dipole transitions resulting from the different HFS levels. The HFS splitting both of the upper and the lower levels must be taken into consideration in explaining the observed signals. Preliminary results of the study are reported, in particular the characteristics of the time development and polarisation of the superradiance.

DOI
10.1088/0022-3700/13/16/002

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Intensity modulations have been observed in the superradiant signals on the 4 2 P 1/2 -4 2 S 1/2 transitions obtained by pulsed dye laser beam excitation of the 4 2 P 1/2 level in Na vapour. The modulations were interpreted as beats among the frequencies of the electric dipole transitions resulting from the different HFS levels. The HFS splitting both of the upper and the lower levels must be taken into consideration in explaining the observed signals. Preliminary results of the study are reported, in particular the characteristics of the time development and polarisation of the superradiance.
Using laser excitation of the 6 2 P levels in the natural isotopic mixture of Rb atoms, modulation of superradiance intensity from some transitions to the lower levels was observed. On the transition 6 2 P 1/2 -6 2 S 1/2 this effect is interpreted as a quantum beat between the hyperfine-structure transitions of the Rb 85 and Rb 87 isotopes. A nearly 'single-pulse' superradiant signal was obtained on the 6 2 P-4 2 D transitions. When a magnetic field was applied transverse to the direction of the laser beam, the pulses obtained showed the properties forecast by two-level superradiance theory. Preliminary results are reported.
The method of Synchronized Quantum Beat Spectroscopy has been improved by introducing the amplitude modulation on the excitation pulse train. By using an amplitude-modulated train of picosecond pulses from a cw mode-locked dye laser, we obtain resonance enhancement of the substate coherence (quantum beat) at f 0 = n f p + n ' f m ( n , n ' : integer, f 0 : sublevel splitting, f p : pulse repetition frequency, f m : modulation frequency), which can be detected by monitoring the optical anisotropy due to the substate coherence. Resonances can be obtained in the frequency domain by sweeping f m . Pressure shift coefficients of the hyperfine splitting in Na 3 2 S 1/2 are measured to be 82, 61, -1 and -47 Hz/Torr for He, N 2 , Ar and Kr, respectively, within an accuracy of ±3 Hz/Torr.
Pulsed dye lasers are used to excite sodium atoms into a coherent superposition of high Rydberg nd(2D32,2D52)\mathrm{nd} (^{2}\mathrm{D}_{\frac{3}{2}},^{2}D_{\frac{5}{2}})nd(2D23​​,2D25​​) states. Analysis of the field ionization behavior of these atoms reveals the time evolution of the superposition state. Rapid application of a weak electric field projects different components of the superposition state onto states having identifiably different field ionization behavior. Analysis of the signal from subsequent field ionization as a function of the time of weak-field application reveals fine-structure quantum beats. These beats result from the time development of the original superposition state. Measurements of the fine-structure quantum beat frequency are presented for the principal quantum numbers n=32,34,35,36,38,and40n=32, 34, 35, 36, 38, \mathrm{and} 40n=32,34,35,36,38,and40.
The population gratings were created by two intersecting resonant light pulses in the ground state 3 2 S 1/2 and the excited state 3 2 P 1/2 in sodium vapor, and their developements in a static magnetic field were monitored by the diffraction of the resonant probe pulse. Intensity modulations of the diffraction signals at the Zeeman frequencies (Zeeman beats) were observed, which are due to the oscillation of the LIPG's. The detailed analysis of the creation, detection and the time development of the LIPG was made in a simple model system with total angular momentum J =1/2 in both the ground and the excited states. The observed beat patterns were compared with the theoretical calculations including the effects of hyperfine interaction in both states. Polarization characteristics were also examined. The agreement between theoretical predictions and experimental results was quite satisfactory.
Pressure shifts of the hyperfine splitting in Na 3(2)S((1/2)) that are due to buffer gases have been measured for the first time to our knowledge by all-optical means using the method of synchronized-quantum-beat spectroscopy reported previously [Y. Fukuda et al., Opt. Commun. 38, 357 (1981)]. The substate coherence is excited and detected with amplitude-modulated mode-locked laser pulses tuned to the D(1) line (pulse-repetition frequency, f(p); modulation frequency, f(m)), and the resonances observed at f(0) = nf(p) + ńf(m), (n and n' are integers) are used for the measurement. The pressure-shift coefficients obtained at 210 degrees C are 82, 61, -1, and -47 Hz/Torr for He, N(2), Ar, and Kr, respectively, within an accuracy of +/-3 Hz/Torr.
We report observation of hyperfine quantum beats in the light emitted by the 72P327{^{2}P}_{\frac{3}{2}}72P23​​ level of Cs133{\mathrm{Cs}}^{133}Cs133 after excitation by a short resonant dye laser pulse. Frequency analysis of the beats provides a measurement of the hyperfine splittings in agreement with previous work. The usefulness of quantum-beat detection as a new method of laser spectroscopy without complications from the Doppler effect is discussed.