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Physical Review A

Optical nonlinear waves in semiconductor quantum dots: Solitons and breathers

Guram T. Adamashvili, Carsten Weber, Andreas Knorr, Nugzar T. Adamashvili

Published Jun 11, 2007• 30 citations
Publisher

Abstract

A general theory of optical resonance solitons and breathers in the presence of single-excitonic and biexcitonic transitions in an ensemble of inhomogeneously broadened semiconductor quantum dots is constructed. Optical plane wave solitons ($2\ensuremath{\pi}$ pulses) are formed in stacked layer structures (many-layered systems) of semiconductor quantum dots. Optical small-amplitude bright breathers ($0\ensuremath{\pi}$ pulses) in semiconductor quantum dot waveguides are considered. Explicit analytical expressions for the shape and parameters of the solitons and breathers in the regime of self-induced transparency are obtained as well as simulations of the space-time dynamics of two-dimensional breathers presented with realistic parameters which can be reached in current experiments. It is shown that, unlike for plane wave breathers, the parameters additionally depend on the waveguide mode. In the special case of plane wave breathers in semiconductor quantum dots, known analytical results are recovered.

DOI
10.1103/physreva.75.063808

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•Jan 1, 2008•1 citation
A general theory of optical resonance solitons and breathers in the presence of single-excitonic and biexcitonic transitions in an ensemble of inhomogeneously broadened semiconductor quantum dots is constructed. Optical plane wave solitons (2\ensuremathπ2\ensuremath{\pi}2\ensuremathπ pulses) are formed in stacked layer structures (many-layered systems) of semiconductor quantum dots. Optical small-amplitude bright breathers (0\ensuremathπ0\ensuremath{\pi}0\ensuremathπ pulses) in semiconductor quantum dot waveguides are considered. Explicit analytical expressions for the shape and parameters of the solitons and breathers in the regime of self-induced transparency are obtained as well as simulations of the space-time dynamics of two-dimensional breathers presented with realistic parameters which can be reached in current experiments. It is shown that, unlike for plane wave breathers, the parameters additionally depend on the waveguide mode. In the special case of plane wave breathers in semiconductor quantum dots, known analytical results are recovered.
We discover and theoretically explore self-induced transparency quadratic solitons (SIT-QS) supported by the media with quadratic optical nonlinearities, doped with resonant impurities. The fundamental frequency of input pulses is assumed to be close to the impurity resonance. We envision an ensemble of inhomogeneously broadened semiconductor quantum dots (QD) in the strong confinement regime grown on a substrate with a quadratic nonlinearity to be a promising candidate for the laboratory realization of SIT-QS. We also examine the influence of inhomogeneous broadening as well as wave number and group-velocity mismatches on the salient properties of the introduced solitons.
Considering the exciton-biexciton coherence, we analytically study the linear absorption and nonlinear propagation properties of the probe and signal field in a semiconductor quantum dot. It is found that in the linear case, in the system takes place an electromagnetically induced transparency phenomenon. Furthermore, we obtain that in the system there occurs one- or two-transparency window, or optical gain, which is controlled by adjusting the coupling control field. For the nonlinear case, the weak probe field, which is induced by a signal field, splits into two parts. When their excited self-Kerr and cross-Kerr nonlinear effects balance the refractive effect of the beam, the system exhibits bright-bright, bright-dark, dark-bright, dark-dark soliton pairs.
The nonlinear optical response of an ensemble of semiconductor quantum dots is analyzed by wave-mixing processes, where we focus on four-wave mixing with two incident pulses. Wave-mixing experiments are often described with semiclassical models, where the light is modeled classically and the material quantum mechanically. Here, however, we use a fully quantized model, where the light is given by a quantum state of light. Quantum light involves more degrees of freedom than classical light as e.g., its photon statistics and quantum correlations, which is a promising resource for quantum devices, such as quantum memories. The light-matter interaction is treated with a Jaynes-Cummings type model and the quantum field is given by a single mode since the quantum dots are embedded in a microcavity. We present numerical simulations of the four-wave-mixing response of a homogeneous system for pulse sequences and find a significant dependence of the result on the photon statistics of the incident pulses. The model constitutes a problem with a large state space which arises from the frequency distribution of the transition energies of the inhomogeneously broadened quantum dot ensemble that is coupled with a quantum light mode. Here we approximate the dynamics by summing over individual quantum dot-microcavity systems. Photon echoes arising from the excitation with different quantum states of light are simulated and compared.
This work is focused on the optical dynamics of mesoscopic semiconductor heterostructures, using as prototypes zero-dimensional quantum dots and quantum cascade lasers which consist of quasitwo-dimensional quantum wells. Within a density matrix theory, a microscopic many-particle theory is applied to study scattering effects in these structures: the coupling to external as well as local fields, electron-phonon coupling, coupling to impurities, and Coulomb coupling. For both systems, the investigated effects are compared to experimentally observed results obtained during the past years. In quantum dots, the three-dimensional spatial confinement leads to the necessity to consider a quantum kinetic description of the dynamics, resulting in non-Markovian electron-phonon effects. This can be seen in the spectral phonon sidebands due to interaction with acoustic phonons as well as a damping of nonlinear Rabi oscillations which shows a nonmonotonous intensity and pulse duration dependence. An analysis of the inclusion of the self-interaction of the quantum dot shows that no dynamical local field terms appear for the simple two-level model. Considering local fields which have their origin in many quantum dots, consequences for a two-level quantum dot such as a zero-phonon line broadening and an increasing signal in photon echo experiments are found. For the use of quantum dots in an optical spin control scheme, it is found that the dephasing due to the electron-phonon interaction can be dominant in certain regimes. Furthermore, soliton and breather solutions are studied analytically in nonlinear quantum dot ensembles. Generalizing to quasi-two-dimensional structures, the intersubband dynamics of quantum cascade laser structures is investigated. A dynamical theory is considered in which the temporal evolution of the subband populations and the current density as well as the influence of scattering effects is studied. In the nonlinear regime, the scattering dependence and the importance of coherence for Rabi oscillations is investigated. The optically induced charge dynamics is discussed with respect to coherent effects. Calculations of the electronic density and pump-probe signals within a microscopic theory of dephasing show coherent transport effects such as gain oscillations, in agreement with recent experimental results.