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Applied Physics Letters

Efficient infrared imaging upconversion via quantum coherence

Robert W. Boyd, Marlan O. Scully

Published Nov 27, 2000• 23 citations
Publisher

Abstract

We show that quantum coherence can be used to achieve marked improvement in the efficiency of the process of infrared upconversion. In one particular example which we analyze in detail, we show that it is possible to convert infrared radiation at a wavelength of 100 μm to the visible with essentially 100% efficiency while maintaining diffraction-limited imaging of the infrared field.

DOI
10.1063/1.1329160

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We show that quantum coherence can be used to achieve marked improvement in the efficiency of the process of infrared upconversion. In one particular example which we analyze in detail, we show that it is possible to convert infrared radiation at a wavelength of 100 μm to the visible with essentially 100% efficiency while maintaining diffraction-limited imaging of the infrared field.
We have demonstrated experimentally that infrared light at 1529.4 nm can be converted into the visible at 780 nm with 54% efficiency through a ladder-type atomic configuration in 85Rb. Specifically we theoretically analyze that high efficiency is due to the large nonlinear dispersion of the index of refraction from the off-resonant enhancement in a four-wave mixing (FWM) process. By using two perpendicular polarized pump fields, the coherence of two FWM processes in this configuration is verified.
Single-photon frequency upconversion is an effective method of infrared single-photon detection and imaging by converting the long-wavelength photons to shorter wavelengths to match the detector’s spectral response. We realized few-photon level 2D infrared imaging with a coincidence frequency upconversion system in a bulk periodically poled lithium niobate crystal. Moreover, the infrared photons carrying orbital angular momentum were converted to the visible regime with high efficiency, while the orbital angular momentum of the photons was well conserved during the frequency upconversion process. The single-photon frequency upconversion method was also used for mid-infrared imaging at 3.39 µm with high efficiency and low noise.
Single-photon frequency upconversion is a nonlinear process where the frequency of the signal photon is translated to the higher frequency with the complete preservation of all the quantum characteristics of the “flying” qubits [1,2]. One promising application of the singlephoton frequency upconversion is converting the infrared photons to the desired spectral regime (usually visible regime) where the high performance detectors are available for sensitive detections [3-6]. The infrared single-photon frequency upconversion detection technique has been successfully used in a variety of applications, including infrared imaging [7] and infrared ultra-sensitive spectroscopy [8,9]. Additionally, such upconversion detector has greatly benefited the applications stringently requiring efficient photon detection in optical quantum computation and communication [10-12]. Furthermore, due to the phase-matching requirement in the frequency upconversion process, the upconversion detectors have some unique features, such as narrow-band wavelength acceptance [13] and polarization sensitivity [14], both of which render them very useful for fiber based quantum systems [15]. In the recent decade, experiments bear that the photon correlation, entanglement, and photon statistics are all well preserved in the coherent frequency upconversion [16-18].
Mid-infrared (MIR) imaging plays a pivotal role in chemical sensing, biomedicine, and material analysis, yet its further development is fundamentally constrained by limited room-temperature sensitivity and the lack of efficient multidimensional light-field control. In recent years, frequency upconversion imaging has emerged as a rapidly advancing approach that translates MIR signals to the visible or near-infrared domain, enabling high-sensitivity detection with mature, low-noise photonic platforms. More importantly, by engineering the pump field in nonlinear frequency conversion processes, a multidimensional imaging framework has been established, enabling indirect, all-optical encoding and retrieval of multiple degrees of freedom—including amplitude, phase, spectrum, time, and polarization—of MIR light fields. This paradigm shifts complex light-field manipulation from the MIR to technologically mature short-wavelength regimes, overcoming intrinsic limitations of conventional approaches. In this review, we systematically summarize the principles, architectures, and representative methodologies of MIR upconversion multidimensional imaging, and outline future directions toward high-sensitivity, high-dimensional, and integrated imaging systems, with implications extending to broader photonic and information processing domains.
The process of up-conversion is shown to enable superior single-photon detectors in the infrared, compared to InGaAs and germanium Avalanche Photodiodes (APDs) (normally used for IR single photon detection). After up-converting an infrared photon to a visible one in a non-linear crystal-Periodically Poled Lithium Niobate (PPLN)-we use a silicon APD to efficiently detect the frequency up-shifted IR photon. We have demonstrated this process at the "high-intensity" level and at the single-photon level, where the up-converted state is effectively a superposition of the single photon Fock state and the vacuum state. We achieve an 80% conversion efficiency over the width of the pulse, and show that this process is coherent, a necessary ingredient for many applications.