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Journal of Physics B Atomic and Molecular Physics

Observation of Bloch-Siegert shifts in the 22S1/2-22P1/2microwave resonance in atomic hydrogen

David A. Andrews, G Newton

Published Jun 21, 1975• 8 citations
Publisher

Abstract

Radio-frequency power shifts in the 2 2 S 1/2 -2 2 P 1/2 microwave resonance in atomic hydrogen have been measured and compared with the results of a numerical integration for the two- and three-level situations. Effects due to the initial phase of the RF field, the finite size of the atomic beam and its trajectory have been included in the numerical integration.

DOI
10.1088/0022-3700/8/9/008

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Radio-frequency power shifts in the 2 2 S 1/2 -2 2 P 1/2 microwave resonance in atomic hydrogen have been measured and compared with the results of a numerical integration for the two- and three-level situations. Effects due to the initial phase of the RF field, the finite size of the atomic beam and its trajectory have been included in the numerical integration.
Observation of Bloch--Siegert shifts in the 2sup2sup 2sup2S/sub 1/2/ - 2sup2sup 2sup2P/ sub 1/2/ microwave resonance in atomic hydrogen
The Bloch-Siegert-type shifts and multiple-quantum resonance shifts of a spin-one system subjected to an oscillating radio-frequency applied at right angles to a DC field have been calculated to sixth order in V, the amplitude of the oscillating field, for the single-quantum resonance, and to fourth order in V for the higher resonances. The level crossing criterion appropriate to two-level systems cannot be used here, and a resonance condition based on a previously derived analogue of Shirley's equation for spin-one systems is used instead. The calculation uses degenerate continued-fraction perturbation theory. Numerical calculations were performed in order to obtain the shape of the resonances, and partially check the analytic results. The atomic levels were assumed to be completely stable; the corrections due to finite atomic lifetimes are expected to be small.
We present investigations of radio-frequency (RF) resonances observed in an optically pumped rubidium vapor. By measuring the systematic shifts (the Bloch–Siegert shifts) of RF resonances in low magnetic fields, we demonstrate limitations of the rotating-wave approximation in the case of angular momentum F ≥ 1. The resonance shifts and deformations are characterized in a wide range of parameters and it is shown that the observed behavior is far more complex than in a standard two-level system. It is also demonstrated that the shifts can be controllably turned on or off by switching between the oscillating and rotating magnetic field. Experimental results are supported with numerical calculations, reproducing all features of the observed signals. Besides fundamental aspect of the research, application of rotating magnetic field helps to suppress/evaluate spectroscopic-measurement and precise-metrology systematic errors. The reported study has also important implications for quantum metrology and information processing beyond RWA and standard two-state qubit dynamics.
When trapped atoms are illuminated by weak lasers, off-resonant transitions cause shifts in the frequencies of the vibrational-sideband resonances. These frequency shifts may be understood in terms of Stark shifts of the individual levels or, as proposed here, as a vibrational Bloch-Siegert shift, an effect closely related to the usual (radio-frequency or optical) Bloch-Siegert shift and associated with rapidly oscillating terms when the rotating wave approximation is not made. Explicit analytic expressions are derived and compared to numerical results, and the similarities and differences between the usual and the vibrational Bloch-Siegert shifts are also spelled out.
Using electron paramagnetic resonance (EPR) at Rabi frequencies, we study the Bloch-Siegert effect in the coherent dynamics of electron spin states driven by a bichromatic radiation consisting of a transverse microwave (MW) and longitudinal radio frequency (RF) fields. The Rabi oscillations on the electron spin states dressed by the MW field are observed at the double resonance, when the MW frequency equals the Larmor frequency of the spin system and the frequency ωrf of the RF field is close to the Rabi frequency ω1 in the MW field. The dispersive (|ωrf - ω1| ~ ωrf, ω1) and near-resonant (ωrf ≈ ω1) regimes are investigated. We demonstrate that the Bloch-Siegert shift increases with increas- ing RF amplitude and at the fixed RF amplitude it has the largest values in the low-frequency (ωrf < ω1) range of the dispersive regime. Experimental results were obtained in the time-resolved EPR for E' centres in quartz.