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arXiv:0801.1642 · Physical Review A

Vibrational Bloch-Siegert effect in trapped ions

Ion Lizuain, Juan Gonzalo Muga, Jürgen Eschner

Published May 19, 2008• 9 citations
arXivHTMLPDF

Abstract

When trapped atoms are illuminated by weak lasers, off-resonant transitions cause shifts in the frequencies of the vibrational-sideband resonances. These frequency shifts may be understood in terms of Stark shifts of the individual levels or, as proposed here, as a vibrational Bloch-Siegert shift, an effect closely related to the usual (radio-frequency or optical) Bloch-Siegert shift and associated with rapidly oscillating terms when the rotating wave approximation is not made. Explicit analytic expressions are derived and compared to numerical results, and the similarities and differences between the usual and the vibrational Bloch-Siegert shifts are also spelled out.

DOI
10.1103/physreva.77.053817

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When trapped atoms are illuminated by weak lasers, off-resonant transitions cause shifts in the frequencies of the vibrational-sideband resonances. These frequency shifts may be understood in terms of Stark shifts of the individual levels or, as proposed here, as a vibrational Bloch-Siegert shift, an effect closely related to the usual (radio-frequency or optical) Bloch-Siegert shift and associated with rapidly oscillating terms when the rotating wave approximation is not made. Explicit analytic expressions are derived and compared to numerical results, and the similarities and differences between the usual and the vibrational Bloch-Siegert shifts are also spelled out.
The two-level rotating wave approximation for two-photon excitations in dipolar molecules is modified to include the effects of the Bloch-Siegert shift in the two-photon resonance energy. The resulting analytical results are used to establish a criterion for when Bloch-Siegert effects are important and the relevance of these effects are compared for fixed laser-molecule configurations versus orientationally averaged results. Two-level model molecules, with parallel permanent and transition dipoles, are used in this work and the effects of Bloch-Siegert shifts are discussed for resonance profiles, time-dependent populations of the excited state, and time-averaged excitation rates. Bloch-Siegert shifts can have pronounced effects on resonance energies and the shape of resonance profiles and, for example, on the magnitudes and the temporal locations of the maxima in the temporal evolution of the time-dependent properties of the system.
We present investigations of radio-frequency (RF) resonances observed in an optically pumped rubidium vapor. By measuring the systematic shifts (the Bloch–Siegert shifts) of RF resonances in low magnetic fields, we demonstrate limitations of the rotating-wave approximation in the case of angular momentum F ≥ 1. The resonance shifts and deformations are characterized in a wide range of parameters and it is shown that the observed behavior is far more complex than in a standard two-level system. It is also demonstrated that the shifts can be controllably turned on or off by switching between the oscillating and rotating magnetic field. Experimental results are supported with numerical calculations, reproducing all features of the observed signals. Besides fundamental aspect of the research, application of rotating magnetic field helps to suppress/evaluate spectroscopic-measurement and precise-metrology systematic errors. The reported study has also important implications for quantum metrology and information processing beyond RWA and standard two-state qubit dynamics.
In a direct two-level qubit system, when the Rabi frequency is comparable to the resonance frequency, the rotating wave approximation is not appropriate. In this case, the Rabi oscillation is accompanied by another oscillation at twice the frequency of the driving field, the so called Bloch-Siegert oscillation (BSO), which depends on the initial phase of the driving field. This oscillation may restrict the precise rotation of a qubit made of direct two-level system. Here, we show that in case of an effectively two-level lambda system, the BSO is inherently negligible, implying a greater precision for rotation of a qubit made of such a lambda system when compared to a direct two-level qubit in a strong driving field.
This paper presents a theoretical study of the light-induced shift of the coherent population trapping resonance. An analytical model is proposed that describes the interaction of two radiation components with an atomic system using a ΛΛΛ scheme and takes into account an additional level of excited state. Both weak and strong coupling regimes with off-resonant transitions are considered. It is shown that, in addition to the conventional dynamic Stark shift, an extra shift arises due to the distortion of the resonance line shape when bichromatic laser radiation interacts with off-resonant atomic transitions. An analytical expression for this additional shift is derived in the weak-coupling limit, and its significant impact on the resonance shape and sensitivity to the intensities of the laser field components is demonstrated. It is found that under strong coupling conditions, the additional shift can deviate substantially from a linear dependence on light intensity, suggesting new opportunities for controlling light shifts in precision atomic devices such as quantum frequency standards.
The time evolution of the atomic dipole moment of a two-level atom damped by an off-resonance squeezed vacuum is studied. Our results are valid for arbitrary detuning between the carrier frequency of the squeezed vacuum and the atomic transition frequency and show that the atomic dipole moment can oscillate with two dominant frequencies. These frequencies are shifted from their central values by an amount which is proportional to the degree of squeezing. We show that this shift of the frequencies is the exact equivalent of the optical Bloch-Siegert shift in the case of the ordinary vacuum damping without the rotating-wave approximation.