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European Quantum Electronics Conference (EQEC)

Suppression of inhomogeneous broadening in rf spectroscopy of optically trapped atoms

Ariel Kaplan, Mikkel F. Andersen, Nir Davidson

Published Jan 1, 2003• 1 citation
Publisher

Abstract

A method for reducing the inhomogeneous broadening in the spectroscopic measurement of the hyperfine splitting of the ground state of optically trapped atoms is demonstrated. This reduction is achieved by the addition of a very weak light field (the "compensating beam"), whose frequency is tuned between the two hyperfine levels. The total shift is obtained by adding the shifts from the trap and the compensating beam, and a complete cancellation of the inhomogeneous broadening will occur for an intensity ratio of /spl sim/ (/spl Delta/HF/2/spl delta/)/sup 2/. With the suppression of inhomogeneous broadening, the atomic coherence time is next limited by the much smaller spontaneous scattering time. Finally, the introduction of the compensating beam provides with an experimental method to control the decoherence rate of the atomic ensemble, and thus to study the interesting interplay between dynamics and coherence in systems with a rich phase-space, for example in atom-optics billiards.

DOI
10.1109/eqec.2003.1314157

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A method for reducing the inhomogeneous broadening in the spectroscopic measurement of the hyperfine splitting of the ground state of optically trapped atoms is demonstrated. This reduction is achieved by the addition of a very weak light field (the "compensating beam"), whose frequency is tuned between the two hyperfine levels. The total shift is obtained by adding the shifts from the trap and the compensating beam, and a complete cancellation of the inhomogeneous broadening will occur for an intensity ratio of /spl sim/ (/spl Delta/HF/2/spl delta/)/sup 2/. With the suppression of inhomogeneous broadening, the atomic coherence time is next limited by the much smaller spontaneous scattering time. Finally, the introduction of the compensating beam provides with an experimental method to control the decoherence rate of the atomic ensemble, and thus to study the interesting interplay between dynamics and coherence in systems with a rich phase-space, for example in atom-optics billiards.
We present a method for reducing the inhomogeneous frequency broadening in the hyperfine splitting of the ground state of optically trapped atoms. This reduction is achieved by the addition of a weak light field, spatially mode matched with the trapping field and whose frequency is tuned in between the two hyperfine levels. We experimentally demonstrate the new scheme with 85Rb{}^{85}\mathrm{Rb}85Rb atoms, and report a 50-fold narrowing of the rf spectrum.
We perform spectroscopy on the hyperfine splitting of 85^{85}85Rb atoms trapped in far-off-resonance optical traps. The existence of a spatially dependent shift in the energy levels is shown to induce an inherent dephasing effect, which causes a broadening of the spectroscopic line and hence an inhomogeneous loss of atomic coherence at a much faster rate than the homogeneous one caused by spontaneous photon scattering. We present here a number of approaches for reducing this inhomogeneous broadening, based on trap geometry, additional laser fields, and novel microwave pulse sequences. We then show how hyperfine spectroscopy can be used to study quantum dynamics of optically trapped atoms.
Rb atoms optically trapped inside a hollow-core fiber. The differential light shift (DLS) for the clock transition caused by the trapping beam is reduced by one order of magnitude through the use of a weak compensation laser beam that is spatially mode-matched to the trapping beam. The coherence of the DLS-compensated system is characterized by microwave Ramsey interferometry, which shows Ramsey fringes with a contrast of over 0.6 at a separation time of 10 ms. The dephasing time, measured by Ramsey spectroscopy at different separation times, reaches tens of milliseconds after DLS cancellation, limited by the residual DLS caused by mode mismatching between the two laser beams. This work paves the way for compact and portable fiber-guided atom interferometers.
We report an investigation to establish the physical mechanisms responsible for decoherence in the generation of photon pairs from atomic ensembles, via the protocol of Duan et al. for long-distance quantum communication [Nature (London) 414, 413 (2001)] and present the experimental techniques necessary to properly control the process. We develop a theory to model in detail the decoherence process in experiments with magneto-optical traps. The inhomogeneous broadening of the ground state by the trap magnetic field is identified as the principal mechanism for decoherence. The theory includes the Zeeman structure of the atomic hyperfine levels used in the experiment, and the polarization of both excitation fields and detected photons. In conjunction with our theoretical analysis, we report a series of measurements to characterize and control the coherence time in our experimental setup. We use copropagating stimulated Raman spectroscopy to access directly the ground-state energy distribution of the ensemble. These spectroscopic measurements allow us to switch off the trap magnetic field in a controlled way, optimizing the repetition rate for single-photon measurements. With the magnetic field off, we then measure nonclassical correlations for pairs of photons generated by the ensemble as a function of the storage time of the single collective atomic excitation. We report coherence times longer than $10\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{s}$, corresponding to an increase of two orders of magnitude compared to previous results in cold ensembles. The coherence time is now two orders of magnitude longer than the duration of the excitation pulses. The comparison between these experimental results and the theory shows good agreement. Finally, we employ our theory to devise ways to improve the experiment by optical pumping to specific initial states.
We study a novel property of light scattering by Rb atoms confined in a far off-resonance optical dipole force trap. The trapping laser wavelength varies from 780 nm to 860 nm and its intensity is about 1 MW/cm{sup 2}. Spontaneous Raman scattering of photons from the trapping laser can change the ground-state hyperfine quantum number F of the atoms. We observe the relaxation time by measuring the population of the F=3 level after optically pumping the atoms into the F=2 level. Spontaneous photon scatter rates as low as 10{sup 3} s{sup -1} have been observed, corresponding to recoil heating rates below 1 mK/s. For detuning from resonance {Delta} greater than the excited-state fine-structure splitting the total scatter rate, including Rayleigh scattering, decreases as {Delta}{sup 2} while the spontaneous Raman scatter rate decreases as {Delta}{sup 4}. This is due to interference between the Raman scattering amplitudes from the two excited-state fine-structure levels in the Kramers-Heisenberg formula. Because Rayleigh scattering dominates, the atoms` F and M{sub F} quantum numbers are preserved even after many scattering events. This makes far off-resonance optical traps ideal for studies of state-selective collisions and collective phenomena.