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Journal of Physics Conference Series

Elimination of inhomogeneous broadening for a ground-state hyperfine transition in an optical trap

Jai Min Choi, D. Cho

Published Sep 1, 2007• 18 citations
Publisher

Abstract

We propose a way to eliminate the inhomogeneous broadening for a ground-state hyperfine transition of an alkali metal atom in an optical trap by using a properly polarized trapping field. The ac Stark shift contribution from the vector polarizability has opposite sign for a pair of ground hyperfine levels. It can be used to eliminate the inhomogeneous broadening from the difference in the scalar polarizbilities due to the hyperfine splitting. The size of the vector term is determined by the polarization state of the trapping field, and by controlling the polarization tightly one can achieve a very narrow linewidth. We estimate required tolerance in the polarization control to achieve 1-Hz linewidth for a specific case of a cesium atom. This proposal has significant implications for an electric dipole moment measurement using cesium atoms and quantum information processing using an optical lattice.

DOI
10.1088/1742-6596/80/1/012037

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The Inhomogeneous Light Shift in Alkali Atoms.

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We propose a way to eliminate the inhomogeneous broadening for a ground-state hyperfine transition of an alkali metal atom in an optical trap by using a properly polarized trapping field. The ac Stark shift contribution from the vector polarizability has opposite sign for a pair of ground hyperfine levels. It can be used to eliminate the inhomogeneous broadening from the difference in the scalar polarizbilities due to the hyperfine splitting. The size of the vector term is determined by the polarization state of the trapping field, and by controlling the polarization tightly one can achieve a very narrow linewidth. We estimate required tolerance in the polarization control to achieve 1-Hz linewidth for a specific case of a cesium atom. This proposal has significant implications for an electric dipole moment measurement using cesium atoms and quantum information processing using an optical lattice.
We demonstrate that the differential ac-Stark shift of a Zeeman-sensitive ground hyperfine transition in an optical trap can be eliminated by using properly polarized trapping light. We use the vector polarizability of an alkali-metal atom to produce a polarization-dependent ac-Stark shift that resembles a Zeeman shift. We study a transition from the $|2{S}_{1/2},F=2,{m}_{F}=\ensuremath{-}2⟩$ to the $|2{S}_{1/2},F=1,{m}_{F}=\ensuremath{-}1⟩$ state of 7Li^{7}\mathrm{Li}7Li to observe $0.59\ifmmode\pm\else\textpm\fi{}0.02\text{ }\text{ }\mathrm{Hz}$ linewidth with interrogation time of 2 s and $0.82\ifmmode\pm\else\textpm\fi{}0.06\text{ }\text{ }\mathrm{s}$ coherence time of a superposition state. Implications of the narrow linewidth and the long coherence time for precision spectroscopy and quantum information processing using atoms in an optical lattice are discussed.
We demonstrate that when laser light is circularly polarized and properly detuned, the ac Stark shift of an alkali-metal atom in its ground state takes the form of a pure Zeeman shift. The condition is satisfied when the laser frequency is between the D1D1D1 and D2D2D2 transition frequencies, with the size of the detuning from the D2D2D2 resonance twice that from the D1D1D1 resonance. The direction of the effective magnetic field is along the laser propagation axis, and its magnitude is proportional to the vector polarizability of the atom and to the laser intensity. We use stimulated Raman spectroscopy on an optically pumped slow atomic beam from a magneto-optical trap to measure the vector polarizability and saturated absorption spectroscopy to show that the scalar polarizability vanishes at the particular detuning.
Characterizing the trap-light-induced frequency shifts of optical Zeeman transitions is essential for the precise control of the interacting dynamics between optically trapped single atoms and external light fields. The closed hyperfine transition, for example, 6 S 1/2 | F = 4〉 → 6 P 3/2 | F ′ = 5〉 of the cesium (Cs) atom, is commonly used because of its high transition strength. However, within this hyperfine transition line, different Zeeman transitions experience distinct light shifts due to diverse susceptibilities to the light field, which are usually sorted as dynamic scalar, vector, and tensor polarizabilities. Here, we report an efficient method for measuring the light shifts of optical Zeeman transitions using single neutral atoms confined in an optical tweezer (OT). The method employs a weak probe beam together with an auxiliary optical pumping beam to manipulate the atomic population in ground states. In this way, population changes in a specific Zeeman state are mapped onto a different ground-state hyperfine manifold, allowing the optical spectrum of the Zeeman transition to be reconstructed through standard state-detection techniques. By using the method, we demonstrate the spectrum measurement of the open Zeeman transition 6 S 1/2 | F = 4, m F = 4〉 → 6 P 3/2 | F ′ = 5, m F ′ = 3〉 for a single Cs atom trapped in a π polarized OT. We further perform a systematic characterization of the tweezer-induced light shifts for both this open transition and the closed Zeeman transition 6 S 1/2 | F = 4, m F = 4〉 → 6 P 3/2 | F ′ = 5, m F ′ = 5〉 over a wide range of trap depths. The influence of the tensor polarizability in deep trap depths is experimentally observed.
The dynamic Stark shift of an inhomogeneously broadened spectral transition has been studied. Our measurements show a shift in the observed 87 Rb ground-state hyperfine transition, which has a nonlinear dependence on light intensity when the conditions for inhomogeneous broadening are met. The nonlinearity is the result of light-intensity gradients in the signal volume, which produce an inhomogeneously broadened asymmetric microwave transition. We show that our measurements are in full agreement with the second-order perturbation-theory treatment of light-induced energy-level shifts when the effects of inhomogeneities are properly taken into consideration. The effects of inhomogeneous broadening must be carefully considered when one extracts oscillator strengths from light-shift data, or performs high-precision laser spectroscopy. Originator-supplied keywords include: AC stark effect, Atomic clocks, Atomic line shapes, Light shifts.
We demonstrate the cancellation of the differential ac Stark shift of the microwave hyperfine clock transition in trapped 87Rb^{87}\mathrm{Rb}87Rb atoms. Recent progress in metrology exploits so-called magic wavelengths, whereby an atomic ensemble can be trapped with laser light whose wavelength is chosen so that both levels of an optical atomic transition experience identical ac Stark shifts. Similar magic-wavelength techniques are not possible for the microwave hyperfine transitions in the alkali metals due to their simple electronic structure. We show, however, that ac Stark shift cancellation is indeed achievable for certain values of wavelength, polarization, and magnetic field. The cancellation comes at the expense of a small magnetic-field sensitivity. The technique demonstrated here has implications for experiments involving the precise control of optically trapped neutral atoms.
The dynamic Stark shift of an inhomogeneously broadened spectral transition has been studied. Our measurements show a shift in the observed 87Rb^{87}\mathrm{Rb}87Rb ground-state hyperfine transition which has a nonlinear dependence on light intensity when the conditions for inhomogeneous broadening are met. The nonlinearity is the result of light-intensity gradients in the signal volume, which produce an inhomogeneously broadened asymmetric microwave transition. We show that our measurements are in full agreement with the second-order perturbation-theory treatment of light-induced energy-level shifts, when the effects of inhomogeneities are properly taken into consideration. The effects of inhomogeneous broadening must be carefully considered when extracting oscillator strengths from light-shift data, or when performing high-precision laser spectroscopy.