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Physical Review A

Measurement of the Zeeman-like ac Stark shift

Chang Yong Park, Heeso Noh, Chungmok Lee, D. Cho

Published Feb 9, 2001• 28 citations
Publisher

Abstract

We demonstrate that when laser light is circularly polarized and properly detuned, the ac Stark shift of an alkali-metal atom in its ground state takes the form of a pure Zeeman shift. The condition is satisfied when the laser frequency is between the $D1$ and $D2$ transition frequencies, with the size of the detuning from the $D2$ resonance twice that from the $D1$ resonance. The direction of the effective magnetic field is along the laser propagation axis, and its magnitude is proportional to the vector polarizability of the atom and to the laser intensity. We use stimulated Raman spectroscopy on an optically pumped slow atomic beam from a magneto-optical trap to measure the vector polarizability and saturated absorption spectroscopy to show that the scalar polarizability vanishes at the particular detuning.

DOI
10.1103/physreva.63.032512

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We demonstrate that when laser light is circularly polarized and properly detuned, the ac Stark shift of an alkali-metal atom in its ground state takes the form of a pure Zeeman shift. The condition is satisfied when the laser frequency is between the D1D1D1 and D2D2D2 transition frequencies, with the size of the detuning from the D2D2D2 resonance twice that from the D1D1D1 resonance. The direction of the effective magnetic field is along the laser propagation axis, and its magnitude is proportional to the vector polarizability of the atom and to the laser intensity. We use stimulated Raman spectroscopy on an optically pumped slow atomic beam from a magneto-optical trap to measure the vector polarizability and saturated absorption spectroscopy to show that the scalar polarizability vanishes at the particular detuning.
The energy shift of an atom due to its interaction with the oscillating electric field of an electromagnetic wave, or a laser light, is called the ac Stark shift. It has been studied both in the field of precision spectroscopy and atom optics. When the laser intensity is not constant spatially, its gradient gives rise to a dipole force. The force was used either to trap atoms in an optical trap or to reflect or guide atoms. We studied the ac Stark effect taking into account the fine structure of an alkali atom. We found that when the laser light is circularly polarized and properly detuned between the D1 and D2 transitions, the ac Stark shift can take the form of a pure Zeeman shift, hence the name analogous Zeeman shift.
We report a different type of optical Stern-Gerlach effect, where a magnetic-field gradient is replaced with a light-intensity gradient and a paramagnetic atom is deflected according to its magnetic quantum number. The laser light is detuned between the D1D1D1 and D2D2D2 frequencies, with the size of the detuning from the D2D2D2 resonance being twice that from the D1D1D1 resonance, and it is circularly polarized to produce an ac Stark shift that takes the form of a pure Zeeman shift. Slow rubidium atoms are extracted from a magneto-optical trap and then spin polarized. The atoms traversing the laser-intensity gradient on one side of the Gaussian beam profile show deflections that depend on the atomic spin state and the laser polarization. When the laser-beam axis is aligned with the slit that defines the atomic beam, we observe focusing and defocusing of the atomic beam.
We demonstrate that the differential ac-Stark shift of a Zeeman-sensitive ground hyperfine transition in an optical trap can be eliminated by using properly polarized trapping light. We use the vector polarizability of an alkali-metal atom to produce a polarization-dependent ac-Stark shift that resembles a Zeeman shift. We study a transition from the $|2{S}_{1/2},F=2,{m}_{F}=\ensuremath{-}2⟩$ to the $|2{S}_{1/2},F=1,{m}_{F}=\ensuremath{-}1⟩$ state of 7Li^{7}\mathrm{Li}7Li to observe $0.59\ifmmode\pm\else\textpm\fi{}0.02\text{ }\text{ }\mathrm{Hz}$ linewidth with interrogation time of 2 s and $0.82\ifmmode\pm\else\textpm\fi{}0.06\text{ }\text{ }\mathrm{s}$ coherence time of a superposition state. Implications of the narrow linewidth and the long coherence time for precision spectroscopy and quantum information processing using atoms in an optical lattice are discussed.
We have measured light shifts, also known as AC Stark shifts, as a function of laser intensity in cold Rubidium atoms by observing sub-natural linewidth gain and loss features in the transmission spectrum of a weak probe beam passing through the atomic sample. The observed energy-level shifts for atoms in a magneto-optical trap (MOT) are found to be consistently higher than that obtained in optical molasses (i.e., when the magnetic field gradient in the MOT is turned off). Using a simple model of a multilevel Rubidium atom interacting with pump and probe beams, we have calculated the theoretical light shift as a function of intensity. A comparison of these calculated values with the light shift data obtained for molasses reveals good agreement between experiment and theory. Further, our model elucidates the role of the Zeeman shifts arising from the magnetic field gradient in the observed probe transmission spectrum for the MOT.