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Physical Review A

Short-time behavior of the correlation functions for the quantum Langevin equation

Raffaella Blasi, Saverio Pascazio

Published Apr 1, 1996• 13 citations
Publisher

Abstract

We analyze the quantum Langevin equation obtained for the Ford-Kac-Mazur and related models. We study an explicit expression for the correlation function of the noise, obtained by making use of the normal-ordered product of operators. Such an expression is divergence-free, does not require any frequency cutoff, and yields the classical (Markoffian) case in the limit of vanishing \ensuremath{\Elzxh}. We also bring to light and discuss two different regimes for the momentum autocorrelation. The high-temperature and weak-coupling limits are considered, and the latter is shown to be related to van Hove's ``${\ensuremath{\lambda}}^{2}$T'' limit. \textcopyright{} 1996 The American Physical Society.

DOI
10.1103/physreva.53.2033

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We analyze the quantum Langevin equation obtained for the Ford-Kac-Mazur and related models. We study an explicit expression for the correlation function of the noise, obtained by making use of the normal-ordered product of operators. Such an expression is divergence-free, does not require any frequency cutoff, and yields the classical (Markoffian) case in the limit of vanishing \ensuremath{\Elzxh}. We also bring to light and discuss two different regimes for the momentum autocorrelation. The high-temperature and weak-coupling limits are considered, and the latter is shown to be related to van Hove's ``\ensuremathλ2{\ensuremath{\lambda}}^{2}\ensuremathλ2T'' limit. \textcopyright{} 1996 The American Physical Society.
A quantum mechanical form of the Langevin equation is derived from an explicit consideration of the molecule-medium interaction, as advocated by Simons in 1978, and by using two identities in the interaction picture. This can be easily reduced to the classical regime, and further simplified to the macroscopic Langevin equation by considering the stochastic Langevin force autocorrelation function. One of the so-called Einstein relations appears as a byproduct. By following the methodology proposed by Simons, an exact expression for the momentum autocorrelation function is obtained. The latter can be used to calculate the zero-frequency macroscopic diffusion coefficient that is observed to satisfy the second Einstein relation. The formalism described above gives rise to the possibility of explicitly computing the transport characteristics such as friction constant and diffusion coefficient from the corresponding quantum statistical mechanical expressions. A discussion on the Langevin equation becomes complete only when the corresponding Fokker-Planck equation is obtained. Therefore, the probability of the evolution of states with a particular absolute magnitude of linear momentum from those of another momentum eigenvalue is quantum mechanically defined. This probability appears as a special average value of a projection operator and as a special projection operator correlation function. A classical identity is introduced that is shown to be valid also for the quantum mechanically defined probability function. By using this identity, the so-called Fokker-Planck equation for the evolution probability is easily established.
Abstract A phenomenological construction of quantum Langevin equations, based on the physical criteria of (i) the canonical equal-time commutators, (ii) the Kubo formula, (iii) the virial theorem and (iv) the quantum fluctuation–dissipation theorem is presented. The case of a single harmonic oscillator coupled to a large external bath is analysed in detail. This allows to distinguish a Markovian semi-classical approach, due to Bedeaux and Mazur, from a non-Markovian full quantum approach, due to to Ford, Kac and Mazur. The quantum-fluctuation–dissipation theorem is seen to be incompatible with a Markovian dynamics. Possible applications to the quantum spherical model are discussed.
Equations for correlation functions in nonequilibrium systems are derived using a generalization of the diagrammatic Keldysh method. The four field operators of the correlation function are ordered on a time contour that consists of four axes extending from -\ensuremath{\infty} to +\ensuremath{\infty} and from +\ensuremath{\infty} to -\ensuremath{\infty} (doubled Keldysh contour). For those correlation functions that may be considered as correlation functions of one-particle Green-functions' fluctuations, a closed system of equations is obtained in the case of weak interaction of the particles with the scattering system. Its structure may be related to the Langevin approach: on the left-hand side a linear operator acts on each of two pairs of the correlation-function arguments, each of these two operators being just the operator of the linearized quantum kinetic equation. The expression for the right-hand side of this equation is derived. It has the meaning of the correlation function of extraneous Langevin sources, and the equation may be called the quantum Boltzmann-Langevin equation. In the quasi-classical limit it reduces to the usual Boltzmann-Langevin equation for the particles' distribution-function fluctuations. Possible applications of the method are discussed.
Quantum diffusion equations featuring explicitly time-dependent transport coefficients are derived from generalized non-Markovian Langevin equations. Generalized fluctuation-dissipation relations and analytic expressions for calculating the friction and diffusion coefficients in nuclear processes are obtained. The asymptotic behavior of the transport coefficients and correlation functions for a damped harmonic oscillator that is linearly coupled in momentum to a heat bath is studied. The coupling to a heat bath in momentum is responsible for the appearance of the diffusion coefficient in coordinate. The problem of regression of correlations in quantum dissipative systems is analyzed.