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Japanese Journal of Applied Physics

Fabrication of Magnetic Barrier NbN Tunnel Junctions with the Gap Voltage over 5 mV

Ryo Terajima, Joe Sakai, Akira Kawakami, Syozo Imai

Published Mar 1, 2008• 0 citations
Publisher

Abstract

Superconductor–insulator–superconductor (SIS) tunnel junctions including magnetic barriers, with structures NbN/AlNiN/NbN or NbN/MgO/NiO/MgO/NbN, were fabricated. The junctions with upper NbN layers of good crystallinity showed a gap voltage ( V g ) higher than 5 mV. In an NbN/Al 0.942 Ni 0.058 N/NbN junction, its Josephson current I c was suppressed to approximately a third of a theoretical value under no magnetic field. Therefore, it would be possible to avoid Josephson noise in magnetic barrier junctions with a much smaller magnetic field than junctions with conventional barriers. The Ni ion area density dependence of I c suppression ratio was identical for both types of junction, suggesting that the area density of magnetic ions is the factor that determines the I c suppression ratio. On the other hand, the extents of degradation of V g and increase in leakage current caused by the increase in Ni ion area density were smaller in MgO/NiO/MgO barrier junctions than in AlNiN barrier junctions. This suggests that the proximity effect of magnetic ions was weakened owing to the separation of Ni ions and NbN layers by the inserted thin MgO layers.

DOI
10.1143/jjap.47.1563

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Superconductor–insulator–superconductor (SIS) tunnel junctions including magnetic barriers, with structures NbN/AlNiN/NbN or NbN/MgO/NiO/MgO/NbN, were fabricated. The junctions with upper NbN layers of good crystallinity showed a gap voltage ( V g ) higher than 5 mV. In an NbN/Al 0.942 Ni 0.058 N/NbN junction, its Josephson current I c was suppressed to approximately a third of a theoretical value under no magnetic field. Therefore, it would be possible to avoid Josephson noise in magnetic barrier junctions with a much smaller magnetic field than junctions with conventional barriers. The Ni ion area density dependence of I c suppression ratio was identical for both types of junction, suggesting that the area density of magnetic ions is the factor that determines the I c suppression ratio. On the other hand, the extents of degradation of V g and increase in leakage current caused by the increase in Ni ion area density were smaller in MgO/NiO/MgO barrier junctions than in AlNiN barrier junctions. This suggests that the proximity effect of magnetic ions was weakened owing to the separation of Ni ions and NbN layers by the inserted thin MgO layers.
All-NbN Josephson tunnel junctions with sputter-deposited magnesium oxide barriers have been fabricated using single-crystal NbN films for the base electrodes. Fabricated Josephson junctions have shown good tunneling characteristics with large gap voltages (5.6-5.8 mV), narrow gap widths (0.1-0.2 mV, from 30 to 70%), and small subgap leakage currents (V/sub m/=20-30 mV, measured at 3 mV). The results of a measurement of a subgap structure for a fabricated junction suggest that the excess leakage currents of fabricated junctions are due to multiparticle tunneling through locally thin areas in the MgO barriers.
Niobium nitride-niobium nitride Josephson tunnel junctions have been fabricated using amorphous magnesium oxide (a-MgO) films as barriers. These junctions have excellent tunneling characteristics. For example, a large gap voltage (Vg=5.1 mV), a large product of the maximum critical current and the normal tunneling resistance (IcRn=3.25 mV), and a small subgap leakage current (Vm=45 mV, measured at 3 mV) have been obtained for a NbN/a-MgO/NbN junction. The critical current of this junction remains finite up to 14.5 K.
We report the electrical properties of all niobium nitride(NbN) Josephson tunnel junctions with magnesium oxide(MgO) films as barriers in the temperature range 4.2-15 K. NbN/MgO/NbN Josephson tunnel junctions have large gap voltages(Vg=4.8-5.4 mV), large products of the maximum critical currents and the normal tunneling resistances(IcRn=3.15-3.35 mV), and small subgap leakage currents(Vm=13-138 mV) at 4.2 K. The junction parameters decreased with increase in temperature, but reasonably large junction parameters(for example, Vg=4.9 mV, IcRn=2.67 mV, and Vm=22 mV) have been obtained even at 9 K. The magnetic penetration depth in NbN electrodes has been measured up to 15 K using two-junction interferometers which consist of NbN/MgO/NbN junctions, NbN ground planes, and NbN control lines.
We have evaluated the electrical characteristics of NbN/Al-AlNx/NbN tunnel junctions fabricated on sapphire-C or fused-silica substrates. NbN/Al-AlNx/NbN multilayers were prepared by reactive dc-magnetron sputtering deposition of lower and upper NbN layers, and rf-magnetron sputtering deposition of the Al layer, followed by radical-nitridation. The junctions showed low sub-gap leakage currents in the current-voltage characteristics at 4.2 K. The quality parameter, Rsg/Rn, where respective Rsgand Rnare the sub-gap resistance at 2 mV and junction resistance at 5 mV, was above 15. The gap voltage (Vg) was around 3.3 mV, which was reduced in comparison with Vgvalues of ~4.3 mV for junctions on MgO substrates. The reduced Vgwas caused by superconducting properties of lower NbN layers deposited on the sapphire or fused-silica substrates. Uniformity in critical current (Ic) was relatively good, and the maximum-to-minimum spread in Icwas ±1.7% for 200 junctions on a sapphire substrate and ±2.0% for the junctions on a fused-silica substrate.
Within the past few years all-refractory superconductor-insulator-superconductor (SIS) tunnel junctions based on Nb/Al/AlO/sub x//Nb technology have displaced lead alloy devices as the preferred junctions for SIS mixers. There is growing interest in materials with higher superconducting energy gaps. NbN has a high gap ( approximately 3 meV) and higher critical temperature than Nb. Its main drawback, apart from the greater complexity of the material itself, stems from its short superconducting coherence length which results in a decrease in the measured gap voltage in proximity barrier structures, as generally used for Nb-based junctions. For this reason, most recent work has concentrated on the direct deposition of MgO as a tunnel barrier. The authors summarise work on Nb devices for MM-wave mixers and then report recent work performed at Cambridge on the fabrication of high quality NbN device structures.
A description of the fabrication technology of high-quality tunnel SIS junctions is presented, with following characteristics: energy gap in superconductors Vg=3.2-3.4 mV, tunnel current density up to J 35 kA/cm2, quality factor Rj/Rn (ratio of subgap resistance to normal-state resistance) up to 30, junction area up to 1 μm2. The SIS junctions are integrated into the NbTiN|SiO2|Al microstrip line. Keywords: superconducting devices, superconductor--insulator--superconductor tunnel junction, plasma etching.