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physica status solidi (b)

Resonatorless Optical Bistability of CdS Reconsideration of Transient Effects Due to Lattice Heating

H. Rossmann, F. Henneberger

Published Sep 1, 1985• 12 citations
Publisher

Abstract

Abstract Results of laser pulse transmission measurements are presented. Introducing a variable optical delay between exciting and probing pulse the relaxation behaviour of induced optical nonlinearities in the spectral region around the An = 1‐exciton resonance is investigated. Optical bistability reported earlier is supported. Crystal lattice heating and nonstationarity due to long‐living extrinsic effects are observed, too, but are of minor importance.

DOI
10.1002/pssb.2221310118

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physica status solidi (b)•May 1, 1990•2 citations
Abstract Results of laser pulse transmission measurements are presented. Introducing a variable optical delay between exciting and probing pulse the relaxation behaviour of induced optical nonlinearities in the spectral region around the An = 1‐exciton resonance is investigated. Optical bistability reported earlier is supported. Crystal lattice heating and nonstationarity due to long‐living extrinsic effects are observed, too, but are of minor importance.
Abstract Under high excitation conditions thick CdS samples show pronounced broad‐band nonlinear transmission in the bound exciton region and up to a wavelength of about 515 nm at cryo‐temperatures. This behavior is only explainable in a model based on impurity neutralization and bound exciton creation. The suitability of these nonlinearities to yield optical bistability will be shown. Bistable operation is investigated in dependence of crystal thickness, impurity concentration, excitation density, wavelength, and temperature. A strong correlation to acceptor‐bound exciton generation is obtained, and the explanation of this bistable operation fits well with that of the above mentioned transmission behavior.
Abstract A new type of optical bistability is presented. Instead of a resonator the intrinsic feedback between the optical excitation of carriers and their recombination is used. Optical bistability appears, if the absorption coefficient increases with growing carrier density. Both propagation effects and carrier diffusion are considered. Analytical model calculations are carried out for an abrupt behaviour of the absorption coefficient. The results explain the hysteresis in the transmittivity of CdS, recently observed.
Optical bistability in the presence of an optically induced absorption is observed when a thin 13-μm CdS sample is inserted between two mirrors of 90 % reflectivity, in our experiment, a modulated cw laser of ~15-mW peak power is tuned on each side of the free exciton resonance in CdS, and the transmission characteristics are studied. A theoretical calculation including both absorptive and dispersive effects is presented and good agreement is obtained. The absorption coefficient and the index of refraction of the material are connected by Kramers-Kronig relations. Propagation effects are taken into account. Sufficiently long pulses (40 ms) are considered to allow the thermally induced absorption to occur. For detunings above the free exciton resonance, we predict that counterclockwise hysteresis loops will first be observed as the intensity rises; for detunings below the free exciton resonance, only clockwise hysteresis loops are predicted. These predictions were experimentally verified. Power levels of the order of 5–10 mW were sufficient to observe bistability. Cavity effects were also observed.
Optical bistability (ob) is investigated in CdS in a wide range of intensities. Under pulsed excitation (total pulse width 20 nsec) we find at 5K for ħωexc ≈ 2.550 eV on the flank of the AΓ5 exciton ob of the induced absorption type for incident intensities of Iexc ≈ 1kW/cm2. The nonlinearity is in this case a collision-broadening of the free exciton resonance [1]. The commutation times τ↓ and τ↑ are about 1 nsec and 5 nsec, respectively. For ħωexc ≈ 2.546 eV we observe absorptive ob due to the formation of an electron-hole plasma [2] for Iexc ≈ 1MW/cm2. Single shot experiments show τ↓ ≲ 500 psec being thus to our knowledge one of the shortest commutation times reported for single beam ob so far. The observed hysteresis loops are compared to model calculations with variable pulse lengths. The comparison indicates true ob in our experiments.
Abstract Thermally induced dispersive and absorptive optical bistability of CdS is investigated in a temperature range of 20 K to RT. The influence of the geometry of the crystals, e. g., thickness, surface area size, and resonator structure, on the hysteresis feature and switching behavior is investigated. The quality of the thermal contact between the sample and the heat sink strongly influences switch‐back times. Further, starting temperature, light spot diameter, and pulse intensity are varied in order to find a set of optimization criteria for this kind of optical bistability. Experimental results are in good agreement with model calculations.