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Soviet Journal of Quantum Electronics

Spectral composition of stimulated radiation from a pulsed copper vapor laser

Anatoly A. Isaev

Published Mar 31, 1980• 25 citations
Publisher

Abstract

An investigation was made of the spectral composition of the spontaneous radiation, superradiance, and laser radiation emitted by a pulsed copper vapor laser. The time resolution was about 3 nsec. It was found that the observed spectral structure of the laser radiation and superradiance was governed by the hyperfine and isotopic splitting of the active levels of the copper atom. In the absence of saturation of the active medium a narrowing of the spectral line profiles was observed during a superradiance pulse. When saturation was achieved for superradiance and lasing, the line profiles broadened to the width of the spontaneous emission line during a radiation pulse. It was found that the temperature of the gas in the copper vapor laser did not exceed 2500°K.

DOI
10.1070/qe1980v010n03abeh009986

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An investigation was made of the spectral composition of the spontaneous radiation, superradiance, and laser radiation emitted by a pulsed copper vapor laser. The time resolution was about 3 nsec. It was found that the observed spectral structure of the laser radiation and superradiance was governed by the hyperfine and isotopic splitting of the active levels of the copper atom. In the absence of saturation of the active medium a narrowing of the spectral line profiles was observed during a superradiance pulse. When saturation was achieved for superradiance and lasing, the line profiles broadened to the width of the spontaneous emission line during a radiation pulse. It was found that the temperature of the gas in the copper vapor laser did not exceed 2500°K.
Since Karras et al. published a paper on the observation of optical cooperative emissions from copper vapor,1 no other convincing experimental evidence has been reported on this puzzling phenomenon. We reported an observation of a similar behavior of the stimulated emission from the copper-vapor laser in the context of Dicke superradiance.2 Subsequently we have carried out a detailed experimental investigation on this pulsing phenomenon in a transverse-discharge copper-vapor laser system. By means of a precision spectral analysis we can identify two principal mechanisms which are responsible for the multiple-pulsing phenomenon in a high-gain condition: (1) the superimposition of a few pulses corresponding to different regions of the spectrum of the laser line, and (2) superradiant ringing due to the coherent collective effect. The conditions in which one or the other of the two mechanisms is manifested are subtle and are not completely understood as yet. But the characteristics of the optical pulses resulting from each mechanism are quite distinct. We describe the difference between the two mechanisms and present the experimental results that exhibit an interesting spectral behavior of the laser pulses in each case.
We have observed, for the first time to our knowledge, stimulated emission in atomic-copper vapor that is excited by a resonant tunable laser beam. One of the important and interesting results obtained in this experiment is that excitation of the (2)P(1/2) level of the copper atoms generates strong amplified spontaneous emission (ASE) for both(2)P(1/2)-(2)D(3/2) and (2)P(3/2)-(2)D(5/2) transitions. This is the first reported direct experimental evidence observed for collisional mixing between the (2)P(1/2) and (2)P(3/2) levels in a copper-vapor laser. Excitation of the (2)P(3/2) level induces substantially weaker ASE for the (2)P(1/2)-(2)D(3/2) transition. In addition, we observed collision-induced ASE for both transitions over a wide range of detuning of the pump frequency. The preliminary results of the experiment are presented, and the implications of the results for high-pressure copper-vapor lasers are discussed.
Theoretical studies of standing and traveling wave lasers are presented. The spectral behavior of the amplified spontaneous emission (superradiance) in a pencil-shaped column is investigated theoretically and experimentally. Spectral narrowing followed by rebroadening has been observed as predicted by the theory. A geometrical representation of an interacting two-level atomic system has been developed and applied to an optical laser. A semi-classical model for a standing wave laser has been examined using the rotating wave approximation, and compared to the exact solution. Depth and width of the Lamb dip are determined theoretically and experimentally. The effect of radial profile of the laser field has been studied using the self-consistent-field approach, and the radius of the beam was measured at various positions from the window.
Our experimental studies of the optical emission from the Cu-vapor laser indicate a breakup of laser pulse into oscillatory structures in certain conditions. We believe this phenomenon is similar to the optical ringing reported earlier.1 We attribute this breakup of the pulse to cooperative effects involved in emission from the Cu-vapor laser.2 This effect is further enhanced by propagation through the system. We earlier explained the high gain of Cu-vapor due to radiation trapping and Rabi oscillation between the 2P and 2S states.3 This analysis further shows that a large percentage of Cu atoms in the lasing medium are in the excited state (2P) most of the time. Therefore, there is a very low probability for total depletion of this level. This implies that the phenomena like gain switching and relaxation oscillation may not play a significant role in the breakup of the laser pulse. The oscillatory structures for both the 510.6-nm and 578.2-nm lines were strongly dependent on the changes in operating temperature. We observed the breakup of the pulse mainly around the temperature of 1600°C.
1. Introduction 2. Review of Classical Electrodynamics 3. Review of Quantum Mechanics 4. The Spontaneous Emission of Radiation 5. Selection Rules for Electric Dipole Transitions 6. Measurement of Radiative Lifetimes of Atoms and Molecules 7. Forbidden Transitions and Metastable Atoms 8. The Width and Shape of Spectral Lines 9. The Absorption and Stimulated Emission of Radiation 10. Radiative Transfer and the Formation of Spectral Lines 11. Population Inversion Mechanisms in Gas Lasers 12. Resonant Modes of Optical Cavities 13. Saturation Characteristics and the Single-Frequency Operation of Gas Lasers 14. Turnable Dye Lasers and Atomic Spectroscopy 15. The Hanle Effect and the Theory of Resonance Flourescence Experiments 16. Optical Double Resonance Experiments 17. Optical Pumping Experiments 18. The Hyperfine Structure of Atoms and its Investigation by Magnetic Resonance Methods Appendix