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Physical Review A

Nonlinear Raman vibrational excitation of a trapped ion

Heping Zeng, Yuzhu Wang, Yusaburo Segawa

Published Mar 1, 1999• 10 citations
Publisher

Abstract

Raman sideband excitations driven by counterpropagating Raman beams are analyzed for the trapped ion under the localization conditions in and beyond the Lamb-Dicke regime. Multiquantum vibrational couplings are demonstrated to produce significant effects on the Raman sideband transitions and the relevant Raman excitations of the trapped ion beyond the Lamb-Dicke regime. The quantum features of the vibrational states attained by exciting the motional ground state are closely associated with the nonlinear vibronic couplings, Raman excitation, and localization conditions. Quantum entanglement and quantum interference are discussed for the trapped ion under various Raman excitation and localization conditions. The results are compared with the recent experiments. Further experimental attempts are proposed to use the single trapped ${}^{25}{\mathrm{Mg}}^{+}$ ion in a linear ion trap.

DOI
10.1103/physreva.59.2174

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Raman sideband excitations driven by counterpropagating Raman beams are analyzed for the trapped ion under the localization conditions in and beyond the Lamb-Dicke regime. Multiquantum vibrational couplings are demonstrated to produce significant effects on the Raman sideband transitions and the relevant Raman excitations of the trapped ion beyond the Lamb-Dicke regime. The quantum features of the vibrational states attained by exciting the motional ground state are closely associated with the nonlinear vibronic couplings, Raman excitation, and localization conditions. Quantum entanglement and quantum interference are discussed for the trapped ion under various Raman excitation and localization conditions. The results are compared with the recent experiments. Further experimental attempts are proposed to use the single trapped 25Mg+{}^{25}{\mathrm{Mg}}^{+}25Mg+ ion in a linear ion trap.
The first sideband Raman excitations driven by counter-propagating Raman beams are analysed for the trapped ion under the localization condition in or beyond the Lamb-Dicke regime. It is demonstrated that multiquantum processes in the vibrational couplings produce significant effects on the the first sideband Raman transitions and the relevant Raman displacements for the trapped ion beyond the Lamb-Dicke regime. The quantum features of the vibrational states attained by displacing the motional ground state are demonstrated to be closely associated with the nonlinear vibronic couplings. Quantum entanglement, and quantum interference as well, are discussed for ion traps with various Raman excitation and localization conditions. The results are compared with the recent experiment reported by Monroe C et al in 1996 Science 272 1131-5.
We consider the first-sideband Raman excitations of a trapped ion in the strong Raman coupling regime on the basis of the splitting approximation. It is demonstrated that not only weak but strong Raman excitations can be used to displace the motional ground state to some well-localized motional states under appropriate conditions. Nonlinear and nonresonant effects are taken into account for the Raman sideband transitions. The condition and limitation for the Raman vibrational excitations to be used for preparing Schr\"odinger cat motional states are analyzed. Quantum interference between the displaced motional states is discussed.
Raman interaction between two internal levels and its sideband cooling of a trapped ion or atom are investigated in copropagating traveling-wave light fields for localization beyond the Lamb-Dicke limit. Under certain conditions, only the first-order sideband excitations (\ensuremath{\Vert}n〉\ensuremath{\rightarrow}\ensuremath{\Vert}n\ifmmode\pm\else\textpm\fi{}1〉 with \ensuremath{\Vert}n〉 being a Fock state) may play a significant role. This provides an experimental realization of the Jaynes-Cummings model with quantized center-of-mass motion beyond the Lamb-Dicke regime, which can be used to measure the statistics of the quantized motion, and thus to detect nonclassical states of motion. Moreover, the multichromatic two-photon Raman excitations of the trapped particle can be used for the preparation of coherent squeezed states of motion.
It is well known that electronic transitions driven by nearly resonant travelling- or standing- wave lasers are often accompanied with vibrational sideband transitions of a single trapped ion undergoing quantized center-of-mass motion [1], Our previous studies showed that quantum statistics of radiation fields can be used to manipulate the vibronic motion of a trapped ion localised within the Lamb-Dicke limit (LDL) [2]. The present paper addresses quantum manipulating vibronic motion of an ion trapped far beyond the LDL.
The nonlinear interaction of three ions in a linear trap with laser light is studied by taking into account the three vibrational modes within a rotating-wave approximation. It is demonstrated that, for localization conditions far from the Lamb-Dicke limit, all three modes have a significant impact on the dynamics of the system. Preparations of vibrational Fock states can be used to realize two different regimes with an exactly solvable three-atom dynamics. The first one corresponds to a nonlinear version of the Tavis-Cummings coupling, whereas the Tavis-Cummings type interactions are suppressed in the second one.
Efficient cooling of trapped ions is a prerequisite for various applications of the ions in precision spectroscopy, quantum information, and coherence control. Raman sideband cooling is an effective method to cool the ions to their motional ground state. We investigate both numerically and experimentally the optimization of Raman sideband cooling strategies and propose an efficient one, which can simplify the experimental setup as well as reduce the number of cooling pulses. Several cooling schemes are tested and compared through numerical simulations. The simulation result shows that the fixed-width pulses and varied-width pulses have almost the same efficiency for both the first-order and the second-order Raman sideband cooling. The optimized strategy is verified experimentally. A single 25Mg+{^{25}\mathrm{Mg}}^{+}25Mg+ ion is trapped in a linear Paul trap and Raman sideband cooled, and the achieved average vibrational quantum numbers under different cooling strategies are evaluated. A good agreement between the experimental result and the simulation result is obtained.