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Physical Review A

Effect of light pressure on transitions from excited states of the Ne atom

А. А. Черненко, I. A. Kartashov, A. V. Shishaev

Published May 16, 2005• 1 citation
Publisher

Abstract

Anomalous behavior of the saturated absorption resonance line shape on the $1\phantom{\rule{0.2em}{0ex}}{s}_{5}\ensuremath{-}2\phantom{\rule{0.2em}{0ex}}{p}_{8}(J=2\ensuremath{-}J=2)$ transition in the Ne atom is experimentally observed. The shape of the saturation resonance on transitions with degenerate excited states of atoms is numerically analyzed. The reasons and conditions for the anomalous behavior of the resonance line shape and the formation of its doublet spectral structure are established. The influence of the resonant light pressure force on the amplitude and the frequency properties of the saturated resonance is investigated. It is shown, that the asymmetry of the doublet splitting of the resonance is caused by the effect of resonant light pressure.

DOI
10.1103/physreva.71.053405

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Anomalous behavior of the saturated absorption resonance line shape on the 1s5\ensuremath−2p8(J=2\ensuremath−J=2)1\phantom{\rule{0.2em}{0ex}}{s}_{5}\ensuremath{-}2\phantom{\rule{0.2em}{0ex}}{p}_{8}(J=2\ensuremath{-}J=2)1s5​\ensuremath−2p8​(J=2\ensuremath−J=2) transition in the Ne atom is experimentally observed. The shape of the saturation resonance on transitions with degenerate excited states of atoms is numerically analyzed. The reasons and conditions for the anomalous behavior of the resonance line shape and the formation of its doublet spectral structure are established. The influence of the resonant light pressure force on the amplitude and the frequency properties of the saturated resonance is investigated. It is shown, that the asymmetry of the doublet splitting of the resonance is caused by the effect of resonant light pressure.
Anomalous behavior of the shape of saturated absorption resonance on the transition 1 s 5 → 2 p 8 ( J =2→ J =2) in the Ne atom is experimentally observed. The shape of the saturation resonance on transitions with degenerate excited states of atoms is analyzed numerically and the reasons for the anomalous behavior of the resonance shape and the formation of its doublet spectral structure are established. The effect of the resonance light pressure on the amplitude and frequency properties of resonance is investigated. It is shown that the asymmetry of the doublet splitting of the resonance is associated with the effect of resonance light pressure.
The effect of a force of resonance pressure of light on the amplitude and frequency properties of saturated-absorption resonance in a gas of two-level atoms was studied. On the basis of numerical solutions of the Liouville and Fokker-Planck equations, dynamics of changes in the velocity-distribution function of an ensemble of atomic particles, depending on the saturation parameter and time of their interaction with a strong field of light, was evaluated. The shape of a resonance line, related to saturated absorption, and its location relative to the frequency of the atomic transition were determined taking into account the dynamics of the distribution function. The results of the calculations are compared with the experimental data.
We report the results of studying the effect of the resonant light pressure force on the amplitude and frequency properties of the nonlinear susceptibility and well known absorption resonance dip occurring in optical saturation spectroscopy of two level atomic gas. On the basis of numerical solutions of the Liouville and Fokker-Plank equations the behaviour pattern of the velocity distribution function of a two-level atomic gas in relation to the saturation intensity and time of interaction with a strong resonant optical field was obtained. Time course of the velocity distribution function due to the action of spontaneous light pressure force leads to modification of the nonlinear susceptibility, absorption saturation resonant line form and to change of frequency dip relative to the atomic resonant frequency transition. The represented numerical modeling results explained qualitatively a number ofexperimental facts, that could not be explained before.
We report on the observation of a light-pressure-induced asymmetry of the well-known absorption dip occurring in optical saturation spectroscopy. This asymmetry is due to the small modification of the atomic velocity distribution that is caused by the spontaneous scattering force of the saturating light field. Our measurements were performed on the \ensuremath{\lambda}=555.65 nm 1S0^{1}\mathrm{S}_{0}1S0​${\mathrm{\ensuremath{-}}}^{3}$P1{\mathrm{P}}_{1}P1​ transition in atomic ytterbium vapor by the use of a frequency-modulated test field propagating collinearly with the scattering field. The experimental results clearly confirm theoretical predictions and demonstrate the significance of the phenomenon for high-resolution laser spectroscopy.
We have studied the effects of optical pumping and near-resonant radiation pressure that compete with the saturation effect on the formation of the line shapes of Doppler-free saturation absorption spectra of alkali atoms. We have measured the reverse of the sign of F g =3 to F e =4 saturated absorption of the rubidium D 2 line and the change in its asymmetry as the optical pumping effect is gradually turned on compared with the saturation effect. The experimentally observed behaviors of optically pumped Lamb dips and crossover resonances in rubidium show good agreement with the calculation using the phenomenological model previously introduced for cesium.
Degenerate four-wave mixing (DFWM) in excited atoms is investigated as a probe of the excited-state density produced by collision-assisted transitions. Sodium atoms are excited to the 3P state by absorption of light in the extreme blue wing of the D lines in the presence of He, Ne and Ar perturbers. The rare-gas pressure dependence of the DFWM signals, resonantly enhanced by the 3P-4D transition, is studied to determine the regime where the signals give an unambiguous measure of the excited-state (3P) density. The observed behaviour is compared with a simple model of DFWM in absorbing media. Good qualitative agreement is obtained and the results illustrate the role of absorption, saturation and finite laser bandwidth. The technique allows small excited-state densities ( approximately 10 9 cm -3 ) to be detected with good temporal and spatial resolution.