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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Angular polarization anisotropy of nonlinear resonance in two-photon scattering of acoustic vibrations in gas

G. N. Alferov, Gennady I. Smirnov, Yu. S. Chesnokov

Published Oct 21, 1998• 0 citations
Publisher

Abstract

The dependence of nonlinear resonances of two-photon scattering on acoustic vibrations in gases is investigated on the polarization of the laser radiation, the angular moment of the energetic levels and magnetic field.
DOI
10.1117/12.328273

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The effect of different populations of the magnetic sublevels of the ground state on the propagation of polarized radiation through resonant media is studied theoretically. The nonlinear refractive indices for circularly and linearly polarized waves in media with arbitrary angular momenta j 1 and j 2 are found. The influence of the coherence between the magnetic sublevels on multiphoton effects is analyzed. It is shown that, as a result of elastic Rayleigh scattering, energy transfer from one component of the wave polarization to the other takes place. The picture of induced four-photon parametric scattering of a weak wave in the presence of a strong wave also changes.
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New resonances are predicted in the interaction of a two-level system (TLS) with laser radiation. These resonances are related to the nonlinear coupling between the TLS and Brillouin enhanced acoustic waves driven by the laser radiation. Resonances in phase conjugation by four-wave mixing driven by stimulated Brillouin scattering (SBS) of laser radiation in fluids have been studied elsewhere.1,2 The coupling of such resonances to the TLS interaction with laser radiation influences the spectral behavior of the TLS. Such resonances appear in addition to the Rabi sidebands. The inclusion of these resonances should have important practical implications in processes that depend on accurate spectral behavior such as in the fields of laser spectroscopy, four-wave mixing, and phase conjugation. Here the new resonances are demonstrated for two mutually detuned counterpropagating laser beams interacting with a TLS at frequencies that may be detuned from the TLS spectral line center. The nonlinear Maxwell Bloch equations coupled to the acoustic wave equation are solved numerically. Damping due to viscosity is taken into account. Wave depletion is included and no perturbation theory approximations are assumed in the numerical solution of these equations.
A theoretical analysis is made of the resonant interaction between a traveling monochromatic light wave of arbitrary intensity and polarization and the 1/21/2 and 10 transitions in gas atoms in a magnetic field. An analysis is made of the influence of atomic collisions and coherence of the Zeeman sublevels of the terms on the structure of nonlinear magnetooptic resonances in the amplitude and polarization characteristics of the wave. Some features of nonlinear magnetooptic resonances for laser excitation of atoms from the ground state are noted. A study is made of the Faraday rotation and self-rotation of the polarization ellipse of the radiation as a function of the detuning of the wave frequency, the saturation parameter, and the optical density of the gas. The stability of the polarization of light in the medium is discussed. It is noted that these laws may be used to analyze and control the radiation characteristics of lasers and amplifiers when the level of saturation of a resonant gaseous medium in a magnetic field is high.