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Physical Review A

Interference stabilization of Rydberg atoms in a strong laser field and phase locking of an array of cavities: Common properties of the phenomena

Victor V. Apollonov, Sergei I. Derzhavin, Victor I. Kislov, Vitaly V. Kuzminov, D A Mashkovskii, A M Prokhorov

Published Sep 1, 1998• 2 citations
Publisher

Abstract

A description of the common properties for different phenomena is presented: interference stabilization of Rydberg atoms in a strong electromagnetic field and phase locking of an array of cavities. A comparison of master equations is held for the discussed effects. Analytical expressions for basic parameters of the problems involved are used for quantitative analysis. The analogy established is exploited for the interpretation of a decrease in intracavity losses in the system of two coupled cavities with an increase of the extent of mutual coupling at a slight detuning of the cavity lengths. The expediency of the analogy establishment consists of existing difficulties in experimental confirmation of the principles of Rydberg-atom stabilization.

DOI
10.1103/physreva.58.2342

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A description of the common properties for different phenomena is presented: interference stabilization of Rydberg atoms in a strong electromagnetic field and phase locking of an array of cavities. A comparison of master equations is held for the discussed effects. Analytical expressions for basic parameters of the problems involved are used for quantitative analysis. The analogy established is exploited for the interpretation of a decrease in intracavity losses in the system of two coupled cavities with an increase of the extent of mutual coupling at a slight detuning of the cavity lengths. The expediency of the analogy establishment consists of existing difficulties in experimental confirmation of the principles of Rydberg-atom stabilization.
The main ideas and features of strong-field interference stabilization of Rydberg atoms are described. Both analytical and model calculations, as well as exact numerical solutions of the Schördinger equation are discussed and compared with each other. Experiments of the FOM Institute groups (The Netherlands) on stabilization of Ba and Ne atoms excited initially, correspondingly, to 27d and 5g levels are discussed. In both cases mechanisms of stabilization are argued in favor of different kinds of interference phenomena rather than adiabatic stabilization.
Photoionization of Rydberg atoms is considered in the framework of the quasiclassical (WKB) approach. Distribution of the photoelectron density in space and time is found and analyzed. This distribution is shown to consist of two main parts: the temporary population, which exists only as long as the light field is on; and the population corresponding to irreversible ionization. The irreversible-ionization wave packets are shown to experience the effect referred to as Coulomb narrowing. An origin of this effect and the conditions of its existence are discussed. In a strong field, rather simple analytical expressions are found for the partial probabilities of above-threshold ionization and for the total probability of ionization. In contrast to many earlier works, in the present theory neither the rotating-wave nor ``pole'' approximations are used, and the results are derived for an arbitrary pulse shape. Strong-field interference stabilization of Rydberg atoms is confirmed to occur at pulse durations shorter than the Kepler period. The arising regimes of interference stabilization are analyzed in comparison with the predictions of earlier works.
The coupling of an electric field to an atomic beam prepared in a phase-locked coherent superposition of energy eigenstates is examined for a ring-laser cavity. The active medium is assumed to be a collection of noninteracting homogeneously broadened two-level atoms whose transition is electric-dipole allowed. The atom-field interaction is treated semiclassically and the atomic coherence injected into the cavity is assumed to be phase matched to the unidirectional plane-wave cavity mode. The polarization is derived for the case in which the electric-field-mode envelope has at most linear phase variations in time and is applied to the problem of frequency locking in a cavity. The presence of the atomic coherence causes the active medium to possess an inherent polarization, i.e., a field-independent contribution. This enables an optical cavity to support laser oscillation over the entire range of relative excitations, in particular, even for strongly absorbing media. A simple linear stability analysis is performed on the electric-field envelope by describing the medium with a slowly varying polarization valid when the time scales of the atomic response are much smaller than those of the variations in the envelope. The stability of frequency-locked oscillation depends on the detuning of the cavity from line center and the strength of the injected coherence relative to that of the injected population difference.
The effect of interference stabilization is shown to exist in a system of two atomic levels coupled by a strong two-color laser field, the two frequencies of which are close to a two-photon Raman-type resonance between the chosen levels, with open channels of one-photon ionization from both of them. We suggest an experiment, in which a rather significant (up to 9090%90) suppression of ionization can take place and which demonstrates explicitly the interference origin of stabilization. Specific calculations are made for H and He atoms and optimal parameters of a two-color field are found. The physics of the effect and its relation with such well-known phenomena as light induced continuum structure and population trapping in a three-level system are discussed.
Integrating Rydberg-state control of atom-atom interactions with cavity control of atom-light interactions enables the combination of local entangling operations with photon-mediated long-range coupling, measurement, and communication. Such integration is challenging because electric fields generated by charges on cavity optics and by cavity-stabilizing actuators may disturb Rydberg-state coherence. Here, we couple a Rydberg tweezer array to a high-cooperativity optical cavity, suppressing the electric fields produced by cavity length actuation so that the residual field variation of about 3 mV/cm3~\mathrm{mV/cm}3 mV/cm rms does not limit Rydberg coherence. We demonstrate two capabilities that neither system provides alone. First, we use Purcell-enhanced fluorescence to read out atoms directly in the ground-Rydberg basis within 7.5 μs7.5~μ\mathrm{s}7.5 μs, well within the Rydberg-state lifetime, with ground- and Rydberg-state detection infidelities of 3%3\%3% and 5%5\%5%, respectively, and with low atom loss. Second, we use Rydberg-Rydberg interactions to control collective light-atom scattering into the cavity mode. Specifically, we drive blockaded Rabi oscillations between a state with two ground-state atoms, which scatter collectively with a superradiant or subradiant rate controlled by the atomic positions, and an entangled state with a single Rydberg excitation, which scatters like a single atom. These capabilities open routes toward networked Rydberg processors, mid-circuit measurements in analog quantum simulators, and many-body quantum optics with entangled emitters coupled collectively to light.