Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physical Review A

Coherent population trapping and electromagnetically induced transparency in multi-Zeeman-sublevel atoms

Hong Yuan Ling, Yongqing Li, Min Xiao

Published Feb 1, 1996• 95 citations
Publisher

Abstract

We present a general formalism for studying the interaction between laser fields and degenerate-Zeeman-sublevel atoms correct up to the first order in the weak probe field. We derive from this theory the equations of motion for a \ensuremath{\Lambda}-type system involving ${\mathit{S}}_{1/2}$, F=2\ensuremath{\leftrightarrows}${\mathit{P}}_{1/2}$, F\ensuremath{'}=1\ensuremath{\leftrightarrows}${\mathit{S}}_{1/2}$, F=1 transitions in $^{87}\mathrm{Rb}$ atoms. These equations are used to numerically investigate the coherent population trapping (CPT) schemes in the ${\mathit{S}}_{1/2}$, F=2\ensuremath{\leftrightarrows}${\mathit{P}}_{1/2}$, F\ensuremath{'}=1 transition induced by a linearly polarized pumping field and the electromagnetically induced transparency exhibited in the weak probe spectrum in the ${\mathit{S}}_{1/2}$, F=1\ensuremath{\leftrightarrows}${\mathit{P}}_{1/2}$, F\ensuremath{'}=1 transition. We discuss the effects of the CPT on the probe spectrum with and without the Doppler broadenings by comparing the probe spectrum derived from the real system with that derived from an ideal \ensuremath{\Lambda}-type system. We show that the atoms in the CPT states are shielded from interacting with the probe field while those in the absorbent states make contributions to the weak probe by the Raman anti-Stokes process, and the effect of the real system on the probe field becomes equivalent to the ideal \ensuremath{\Lambda} system only in the strong CPT parameter regime. \textcopyright{} 1996 The American Physical Society.

DOI
10.1103/physreva.53.1014

Related papers

Coherent population trapping: its physics and historical roots

Anatolii M. Shalagin

There presented basic information on coherent population trapping (CPT) and related phenomenon of electromagnetically induced transparence, ‘dark’ and ‘bright’ (anomalous absorption) states is presented. Spectrum transformation is considered in probe field spectroscopy for Λ-scheme in various settings. The close relation is revealed between the effect of CPT in the manifold of magnetic sublevels and the phenomenon of optical pumping (optical orientation and optical alignment). CPT is shown to be generalized to the case of several transitions with a common upper level and with the corresponding number of light fields each being in quasiresonance with its ‘own’ transition.

EPJ Web of Conferences•Dec 13, 2016•0 citations

Pump-probe spectroscopy in degenerate two-level atoms with arbitrarily strong fields

T. Zigdon, A. D. Wilson‐Gordon, Chana Goren +2 more

We review our previous work on pump-probe spectroscopy in realistic degenerate two-level systems and model systems. In particular, we discuss the role of transfer of coherence (TOC) between the ground and excited hyperfine states in producing electromagnetically-induced transparency (EIA) peaks in the probe spectrum, when an Fg goes to Fe = Fg +1 transition in an alkali-metal atom interacts with a strong pump and weak probe that have perpendicular polarizations. When the pump is rho+ polarized and the probe pi polarized, this system can be modelled by an N system. We also discuss the role of transfer of population (TOP) between the Zeeman levels of the ground hyperfine state in producing EIA peaks when the pump and probe have the same polarization. This system can be modelled using a double two-level system. The role of Doppler broadening and phase-changing collisions in modifying the EIA-TOC and EIA-TOP absorption and refraction spectra is also discussed. All these spectra were calculated using MATLAB programs that both construct and solve the relevant Bloch equations. In our recent work, we consider the effect of a strong probe on the pump absorption and refraction spectra when the pump and probe polarizations are linear and perpendicular. It is difficult to solve this problem numerically due to the large number frequencies involved. In order to simplify the problem, we considered two cases: (i) rho+ polarized pump and pi polarized probe, and (ii) rho+ polarized pump and rho- polarized probe, and investigated a series of transitions in both Rb and Cs, using modified versions of the MATLAB programs devised for the weakprobe case. A number of interesting differences from the weak-probe case were found. For example, when the probe is sufficiently strong, we found the pump and probe spectra to show complementary behavior. In addition, as the number of Zeeman levels increase, the EIA peaks become progressively sharper, and are accompanied by steeper dispersion.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Mar 2, 2007•2 citations

Coherent population trapping in a Λ configuration coupled by magnetic dipole interactions

Huidong Kim, Hyok Sang Han, Tai Hyun Yoon +1 more

We report our study on coherent population trapping (CPT) in a $\ensuremath{\Lambda}$ configuration coupled by magnetic dipole interactions. The $\ensuremath{\Lambda}$ configuration is formed by bichromatic radio-frequency fields coupling a pair of Zeeman sublevels in one hyperfine level of an alkali-metal atom to another sublevel in the other hyperfine level. The Zeeman sublevel at the apex is coupled to a state in the $nP$ manifold via an optical transition on one of the spectroscopic $D$ lines to induce optical pumping to a dark state. The configuration is closed without leakage to other Zeeman sublevels. We use lithium atoms in an optical trap for our experimental study. The system allows independent control of the main parameters characterizing CPT, which include the upper-state decay rate and the decoherence rate as well as the Rabi frequencies. By turning off the applied fields, the system is frozen so that its quantum state can be measured precisely. We studied the line shapes and dynamics of the CPT system, and measured the phase relation of the dark superposition state to find excellent agreement with theory. The possible application of the scheme as a method to cool optically trapped atoms below the recoil limit in a manner analogous to velocity-selective coherent population trapping is discussed.

Physical Review A•Mar 10, 2014•7 citations

Electromagnetically induced transparency in a thin film

David Petrosyan, Yu. P. Malakyan

Summary form only given. We have developed a formalism for rendering the (near)resonant interaction of two electromagnetic fields with an inhomogeneously broadened system consisting of three-level /spl Lambda/-atoms confined in an ultrathin cell of thickness 10 /spl mu/m or less. The peculiar features of this model stem from the fact that the free interaction time of atoms with two laser fields is solely determined by the wall-to-wall time of atomic flight. Unusual absorptive and dispersive properties of this system have been found. Thus, we show that the absorption spectrum of the probe field and the fluorescence signal from the upper atomic level contain two sub-Doppler dips. One of them is originated from the optical pumping due to the leak of atomic population from the upper atomic level, white the other much narrower dip corresponds to the electromagnetically induced transparency (EIT) effect established in the medium due to the coherent population trapping of the atoms. When the coupling field is tuned into the exact resonance with the corresponding atomic transition, the locations of the two dips on the frequency scale coincide, whereas in the case of nonzero detuning of the coupling field, the two dips are shifted from each other by the amount of this detuning. This is because the EIT is very sensitive to the Raman resonance condition, while the OP is most efficient in the vicinity of the resonance of the probe field with the atomic transition frequency.

Conference on Lasers and Electro-Optics•Aug 29, 2005•2 citations

Electromagnetically Induced Transparency in Λ-Type Zeeman Sublevels of Cesium Atoms

Tiancai Zhang

Employing two lasers as the coupling and probe fields which have opposite circular polarization (σ + and σ -), electromagnetically induced transparency (EIT) in Λ-type Zeeman sublevels of cesium 6 2S 1/2F=3-6 2P 3/2F′=2 degenerate two-level system has been demonstrated via probe absorption spectra. The effect of the intensity and detuning of different coupling. Laser on EII was also investigated in experiments. Within the Doppler background, optical pumping among Zeeman sub-levels and the population of different Zeeman sub-levels can dominate the intensity of EIT effect. And the physical reason of the rugged spectra are presented qualitatively.

Chinese Journal of Lasers•Jan 1, 2005•0 citations

Multilevel dark states in an inhomogeneously broadened open atomic system

Yifu Zhu, Shijun Wang, Neil Mulchan

We report an experimental observation of coherent population trapping in multilevel dark states prepared in the ground hyperfine states of ${}^{87}\mathrm{Rb}$ atoms confined in a room-temperature vapor cell. The dark states are created by a linearly polarized coupling laser that is tuned to the ${}^{87}\mathrm{Rb}$ ${D}_{1}$ $F=2\ensuremath{\leftrightarrow}{F}^{\ensuremath{'}}=1$ or 2 transition and establishes \ensuremath{\Lambda}-type transition chains. The Doppler shift for the \ensuremath{\Lambda}-type transition chains is compensated by the left and right circularly polarized components of the coupling laser. The multilevel dark states that consist of three or two magnetic sublevels among the five degenerate magnetic sublevels in the $F=2$ ground hyperfine state are probed by a weak probe laser scanned across the same ${D}_{1}$ transition and their existence is manifested by a strong dependence of the probe excitation on the probe polarization. Our experiment demonstrates the importance of coherent population trapping in a laser coupled degenerate multilevel open atomic system, which may play an important role in diverse physical phenomena such as atom cooling and trapping, optical pumping, and multiple laser excitation and ionization of atoms and molecules.

Physical Review A•May 1, 1999•16 citations
We present a general formalism for studying the interaction between laser fields and degenerate-Zeeman-sublevel atoms correct up to the first order in the weak probe field. We derive from this theory the equations of motion for a \ensuremath{\Lambda}-type system involving S1/2{\mathit{S}}_{1/2}S1/2​, F=2\ensuremath{\leftrightarrows}P1/2{\mathit{P}}_{1/2}P1/2​, F\ensuremath{'}=1\ensuremath{\leftrightarrows}S1/2{\mathit{S}}_{1/2}S1/2​, F=1 transitions in 87Rb^{87}\mathrm{Rb}87Rb atoms. These equations are used to numerically investigate the coherent population trapping (CPT) schemes in the S1/2{\mathit{S}}_{1/2}S1/2​, F=2\ensuremath{\leftrightarrows}P1/2{\mathit{P}}_{1/2}P1/2​, F\ensuremath{'}=1 transition induced by a linearly polarized pumping field and the electromagnetically induced transparency exhibited in the weak probe spectrum in the S1/2{\mathit{S}}_{1/2}S1/2​, F=1\ensuremath{\leftrightarrows}P1/2{\mathit{P}}_{1/2}P1/2​, F\ensuremath{'}=1 transition. We discuss the effects of the CPT on the probe spectrum with and without the Doppler broadenings by comparing the probe spectrum derived from the real system with that derived from an ideal \ensuremath{\Lambda}-type system. We show that the atoms in the CPT states are shielded from interacting with the probe field while those in the absorbent states make contributions to the weak probe by the Raman anti-Stokes process, and the effect of the real system on the probe field becomes equivalent to the ideal \ensuremath{\Lambda} system only in the strong CPT parameter regime. \textcopyright{} 1996 The American Physical Society.
There presented basic information on coherent population trapping (CPT) and related phenomenon of electromagnetically induced transparence, ‘dark’ and ‘bright’ (anomalous absorption) states is presented. Spectrum transformation is considered in probe field spectroscopy for Λ-scheme in various settings. The close relation is revealed between the effect of CPT in the manifold of magnetic sublevels and the phenomenon of optical pumping (optical orientation and optical alignment). CPT is shown to be generalized to the case of several transitions with a common upper level and with the corresponding number of light fields each being in quasiresonance with its ‘own’ transition.
We review our previous work on pump-probe spectroscopy in realistic degenerate two-level systems and model systems. In particular, we discuss the role of transfer of coherence (TOC) between the ground and excited hyperfine states in producing electromagnetically-induced transparency (EIA) peaks in the probe spectrum, when an Fg goes to Fe = Fg +1 transition in an alkali-metal atom interacts with a strong pump and weak probe that have perpendicular polarizations. When the pump is rho+ polarized and the probe pi polarized, this system can be modelled by an N system. We also discuss the role of transfer of population (TOP) between the Zeeman levels of the ground hyperfine state in producing EIA peaks when the pump and probe have the same polarization. This system can be modelled using a double two-level system. The role of Doppler broadening and phase-changing collisions in modifying the EIA-TOC and EIA-TOP absorption and refraction spectra is also discussed. All these spectra were calculated using MATLAB programs that both construct and solve the relevant Bloch equations. In our recent work, we consider the effect of a strong probe on the pump absorption and refraction spectra when the pump and probe polarizations are linear and perpendicular. It is difficult to solve this problem numerically due to the large number frequencies involved. In order to simplify the problem, we considered two cases: (i) rho+ polarized pump and pi polarized probe, and (ii) rho+ polarized pump and rho- polarized probe, and investigated a series of transitions in both Rb and Cs, using modified versions of the MATLAB programs devised for the weakprobe case. A number of interesting differences from the weak-probe case were found. For example, when the probe is sufficiently strong, we found the pump and probe spectra to show complementary behavior. In addition, as the number of Zeeman levels increase, the EIA peaks become progressively sharper, and are accompanied by steeper dispersion.
We report our study on coherent population trapping (CPT) in a $\ensuremath{\Lambda}$ configuration coupled by magnetic dipole interactions. The $\ensuremath{\Lambda}$ configuration is formed by bichromatic radio-frequency fields coupling a pair of Zeeman sublevels in one hyperfine level of an alkali-metal atom to another sublevel in the other hyperfine level. The Zeeman sublevel at the apex is coupled to a state in the nPnPnP manifold via an optical transition on one of the spectroscopic DDD lines to induce optical pumping to a dark state. The configuration is closed without leakage to other Zeeman sublevels. We use lithium atoms in an optical trap for our experimental study. The system allows independent control of the main parameters characterizing CPT, which include the upper-state decay rate and the decoherence rate as well as the Rabi frequencies. By turning off the applied fields, the system is frozen so that its quantum state can be measured precisely. We studied the line shapes and dynamics of the CPT system, and measured the phase relation of the dark superposition state to find excellent agreement with theory. The possible application of the scheme as a method to cool optically trapped atoms below the recoil limit in a manner analogous to velocity-selective coherent population trapping is discussed.
Summary form only given. We have developed a formalism for rendering the (near)resonant interaction of two electromagnetic fields with an inhomogeneously broadened system consisting of three-level /spl Lambda/-atoms confined in an ultrathin cell of thickness 10 /spl mu/m or less. The peculiar features of this model stem from the fact that the free interaction time of atoms with two laser fields is solely determined by the wall-to-wall time of atomic flight. Unusual absorptive and dispersive properties of this system have been found. Thus, we show that the absorption spectrum of the probe field and the fluorescence signal from the upper atomic level contain two sub-Doppler dips. One of them is originated from the optical pumping due to the leak of atomic population from the upper atomic level, white the other much narrower dip corresponds to the electromagnetically induced transparency (EIT) effect established in the medium due to the coherent population trapping of the atoms. When the coupling field is tuned into the exact resonance with the corresponding atomic transition, the locations of the two dips on the frequency scale coincide, whereas in the case of nonzero detuning of the coupling field, the two dips are shifted from each other by the amount of this detuning. This is because the EIT is very sensitive to the Raman resonance condition, while the OP is most efficient in the vicinity of the resonance of the probe field with the atomic transition frequency.
Employing two lasers as the coupling and probe fields which have opposite circular polarization (σ + and σ -), electromagnetically induced transparency (EIT) in Λ-type Zeeman sublevels of cesium 6 2S 1/2F=3-6 2P 3/2F′=2 degenerate two-level system has been demonstrated via probe absorption spectra. The effect of the intensity and detuning of different coupling. Laser on EII was also investigated in experiments. Within the Doppler background, optical pumping among Zeeman sub-levels and the population of different Zeeman sub-levels can dominate the intensity of EIT effect. And the physical reason of the rugged spectra are presented qualitatively.
We report an experimental observation of coherent population trapping in multilevel dark states prepared in the ground hyperfine states of 87Rb{}^{87}\mathrm{Rb}87Rb atoms confined in a room-temperature vapor cell. The dark states are created by a linearly polarized coupling laser that is tuned to the 87Rb{}^{87}\mathrm{Rb}87Rb D1{D}_{1}D1​ $F=2\ensuremath{\leftrightarrow}{F}^{\ensuremath{'}}=1$ or 2 transition and establishes \ensuremath{\Lambda}-type transition chains. The Doppler shift for the \ensuremath{\Lambda}-type transition chains is compensated by the left and right circularly polarized components of the coupling laser. The multilevel dark states that consist of three or two magnetic sublevels among the five degenerate magnetic sublevels in the F=2F=2F=2 ground hyperfine state are probed by a weak probe laser scanned across the same D1{D}_{1}D1​ transition and their existence is manifested by a strong dependence of the probe excitation on the probe polarization. Our experiment demonstrates the importance of coherent population trapping in a laser coupled degenerate multilevel open atomic system, which may play an important role in diverse physical phenomena such as atom cooling and trapping, optical pumping, and multiple laser excitation and ionization of atoms and molecules.